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We develop a quantum master equation (QME) approach to investigate the electroluminesence (EL) of molecules confined between metallic electrodes and coupled to quantum plasmonic modes. Within our general state-based framework, we describe…

Mesoscale and Nanoscale Physics · Physics 2018-03-06 Justin P. Bergfield , Joshua R. Hendrickson

A numerically exact solution to the many emitter -- cavity problem as an open many body system is presented. The solution gives access to the full, nonperturbative density matrix and thus the full quantum statistics and quantum…

Mesoscale and Nanoscale Physics · Physics 2015-01-15 Marten Richter , Michael Gegg , T. Sverre Theuerholz , Andreas Knorr

A new method to calculate level densities for non-interacting Fermions within the constant-spacing model with a finite number of states is developed. We show that asymptotically (for large numbers of particles or holes) the densities have…

Nuclear Theory · Physics 2013-01-08 Adriana Pálffy , Hans A. Weidenmüller

This paper is concerned with efficient representations and approximations of the solution to the scattering problem by a system of strongly coupled plasmonic particles. Three schemes are developed: the first is the resonant expansion which…

Numerical Analysis · Mathematics 2017-09-26 Habib Ammari , Matias Ruiz , Sanghyeon Yu , Hai Zhang

For atoms embedded in dense plasma, the plasma screening effects will greatly alter their structure and dynamics, and then determine the radiation transport properties of the plasma. In the present work, a new statistical model is proposed…

Plasma Physics · Physics 2020-11-25 Fuyang Zhou , Yizhi Qu , Junwen Gao , Yulong Ma , Yong Wu , Jianguo Wang

We present a unified approach to describe spasing in plasmonic systems modeled by quantum emitters interacting with resonant plasmon mode. We show that spaser threshold implies detailed energy transfer balance between the gain and plasmon…

Mesoscale and Nanoscale Physics · Physics 2019-04-15 Tigran V. Shahbazyan

Plasmon-emitter interactions are of paramount importance in modern nanoplasmonics and are generally maximal at short emitter-surface separations. However, when the separation falls below 10-20 nm, the classical theory progressively…

Mesoscale and Nanoscale Physics · Physics 2020-01-20 P. A. D. Gonçalves , Thomas Christensen , Nicholas Rivera , Antti-Pekka Jauho , N. Asger Mortensen , Marin Soljačić

We study theoretically the emission and lasing properties of a single nanoshell spaser nanoparticle, or plasmonic nanolaser, made of an active core (gain material) and a plasmonic metal shell. Based on an analytical framework coupling…

Energetic electromagnetic fields produce a variety of elementary excitations in solids that can strongly modify their primary photoemission spectra. Such is the plasmon excitation or pumping mechanism which, although indirect, is very…

Materials Science · Physics 2025-04-11 Branko Gumhalter

We obtain the local density of states (LDOS) for any nanoplasmonic system in the frequency range dominated by a localized surface plasmon. By including the Ohmic losses in a consistent way, we show that the plasmon LDOS is proportional to…

Mesoscale and Nanoscale Physics · Physics 2016-11-10 Tigran V. Shahbazyan

The accurate calculation of excited state properties of interacting electrons in the condensed phase is an immense challenge in computational physics. Here, we use state-of-the-art equation-of-motion coupled-cluster theory with single and…

Chemical Physics · Physics 2019-07-10 Alan M. Lewis , Timothy C. Berkelbach

Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is…

A theory of lasing in a two-dimensional array of metal nanoparticles (MNPs) covered with a thin layer of fluorescent molecules is developed from first principles. The approach is based on a rigorous account of the local field in a close…

Mesoscale and Nanoscale Physics · Physics 2021-11-24 V. G. Bordo

The collective excitation of the conduction electrons in subwavelength structures gives rise to the Localized Surface Plasmon(LSP). The system consisting of two such LSPs, known as the dimer system,is of fundamental interest and is being…

Mesoscale and Nanoscale Physics · Physics 2014-03-19 Bo Liu , Eric J. Heller

Versatile quantum modes emerge for plasmon describing the collective oscillations of free electrons in metallic nanoparticles when the particle sizes are greatly reduced. Rather than traditional nanoscale study, the understanding of quantum…

We study a class of random processes on $N$ particles which can be interpreted as stochastic model of luminescence. Each particle can stay in one of two states: Excited state or ground state. Any particle at ground state is excited with a…

Probability · Mathematics 2018-10-31 E. Pechersky , S. Pirogov , G. M. Schütz , A. Vladimirov , A. Yambartsev

In this paper the influence of large-scale decreasing and increasing gradients of the density of magnetized plasma on the relaxation process of a continuously injected relativistic electron beam with an energy of 611 keV ($v_b=0.9c$) and a…

Plasma Physics · Physics 2022-08-30 Vladimir Annenkov , Evgeniia Volchok

Strong coupling of plasmonic excitations and dipolar emitters, such as organic molecules, have been studied extensively in the last years. The questions whether strong coupling can be achieved with a single molecule only and how this is…

Plasmonic nanocavities enable the confinement of molecules and electromagnetic fields within nano-metric volumes. As a consequence, the molecules experience a remarkably strong interaction with the electromagnetic field, to such an extent…

Chemical Physics · Physics 2021-09-01 Jacopo Fregoni , Tor S. Haugland , Silvio Pipolo , Tommaso Giovannini , Henrik Koch , Stefano Corni

Rapid progress in electrically-controlled plasmonics in solids poses a question about effects of electronic reservoirs on the properties of plasmons. We find that plasmons in electronically open systems [i.e. in (semi)conductors connected…

Mesoscale and Nanoscale Physics · Physics 2020-12-03 Kirill Kapralov , Dmitry Svintsov