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We provide conclusive demonstration of vibrational pumping under Surface Enhanced Raman Scattering (SERS) conditions by performing anti-Stokes/Stokes ratio measurements down to 10 K using dried silver colloids, the dye rhodamine 6G and 676…

Chemical Physics · Physics 2007-05-23 R. C. Maher , P. G. Etchegoin , E. C. Le Ru , L. F. Cohen

We demonstrate gold coated polymer surface enhanced Raman scattering (SERS) substrates with a pair of complementary structures--positive and inverted pyramids array structures fabricated by multiple-step molding and replication process. The…

Optics · Physics 2014-02-10 Zhida Xu , Logan Liu

Superconducting MgB(2) films with Tc = 38.6 K were prepared using a precursor-deposition, ex-situ post-processing approach. Precursor films of boron, ~0.5 micrometer thick, were deposited onto Al(2)O(3) (102) substrates by e-beam…

We apply interferometric picometrology to measure the complex refractive index and dielectric properties of ultra-thin gold films as a continuous function of thickness from 0.2 nm to 10 nm deposited on thermal oxide on silicon. Three…

Materials Science · Physics 2009-03-17 Xuefeng Wang , Ming Zhao , David D Nolte

Using density functional theory, we carried out systematic calculations for a series of ultrathin iron layers with thicknesses ranging from one atomic monolayer to eleven monolayers (up to about 1.5 nm). We considered three cases: (1) iron…

In this paper Al doped ZnO (AZO) thin films with 0, 3, 6 and 12 at. % Al concentration were prepared by sol-gel method on glass substrates. The deposited films were annealed at different temperatures of 300, 350, 400, 450 and 500 {\deg}C…

Mesoscale and Nanoscale Physics · Physics 2014-12-30 F. Eskandari , M. Ranjbar , P. Kameli , H. Salamati

The results of characterization of TiAlSiON hard coatings deposited on ferric-chromium AISI 430 stainless steel by plasma enhanced magnetron sputtering are presented. The coating with maximum hardness (of 45 GPa) was obtained at the…

Thin-film nanocomposites, consisting of silver nanoparticles embedded in a dielectric Teflon\textregistered AF matrix, were synthesized using vapor phase co-deposition. The electrical conductivity of these composites was measured in-situ as…

Materials Science · Physics 2011-06-21 Haoyan Wei , Hergen Eilers

We present a modeling of the nonlinear optical response of a metal surface in order to account for recent experimental results from two-color Sum-Frequency Generation experiments on gold. The model allows calculating the surface and bulk…

Chemical Physics · Physics 2019-05-16 Bertrand Busson , Laetitia Dalstein

While classical percolation is well understood, percolation effects in randomly packed or jammed structures are much less explored. Here we investigate both experimentally and theoretically the electrical percolation in a binary composite…

Materials Science · Physics 2021-04-20 Shiva Pokhrel , Brendon Waters , Solveig Felton , Zhi-Feng Huang , Boris Nadgorny

Continuous films of metals like gold and silver with a thickness of a few tens of nm have poor optical transmission in the visible and infrared. However, the same films become largely transparent when the transmission is mediated by coupled…

Optics · Physics 2010-04-06 Arvind S. Vengurlekar

Transition Edge Sensor (TES) spectrometers for hard X-ray beamline science will enable improved X-ray emission and absorption spectroscopy in the information-rich 2 to 20 keV energy range. We are building a TES-based instrument for the…

Instrumentation and Detectors · Physics 2020-08-26 Tejas Guruswamy , Lisa M. Gades , Antonino Miceli , Umeshkumar M. Patel , John T. Weizeorick , Orlando Quaranta

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

Strongly Correlated Electrons · Physics 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

Atomically thin boron nitride (BN) nanosheets have many properties desirable for surface enhanced Raman spectroscopy (SERS). BN nanosheets have a strong surface adsorption capability towards airborne hydrocarbon and aromatic molecules. For…

Mesoscale and Nanoscale Physics · Physics 2016-06-24 Qiran Cai , Srikanth Mateti , Kenji Watanabe , Takashi Taniguchi , Shaoming Huang , Ying Chen , Lu Hua Li

A sample-based stochastic model is presented to investigate the effects of uncertainties of various input parameters, including laser fluence, laser pulse duration, thermal conductivity constants for electron, and electron-lattice coupling…

Computational Physics · Physics 2016-04-28 Nazia Afrin , Yuwen Zhang , J. K. Chen

In this letter, we report a chemical route for synthesizing SiO2@Au core-shell nanoparticles. The process includes four steps: i) preparation of the silica cores, ii) grafting gold nanoparticles over SiO2 cores, iii) priming of the…

The spreading of a bilayer gold film propagating outward from gold clusters, which are pinned to clean Si(111), is imaged in real time by low energy electron microscopy. By monitoring the evolution of the boundary of the gold film at fixed…

Mesoscale and Nanoscale Physics · Physics 2009-12-18 Nicola Ferralis , Farid El Gabaly , Andreas K. Schmid , Roya Maboudian , Carlo Carraro

We present simulations of an efficient high numerical aperture solid immersion metalens concept for fluorescence microscopy. The technique exploits the preferential emission of interfacial dipoles into a high refractive index substrate…

Optics · Physics 2022-01-12 Zhiheng Li , Zequan Chen , Rupert F. Oulton , Ming Fu

We present SERS-active metal holographic metasurfaces fabricated from metal periodical nanograting deposited on a dielectric substrate. The metasurface consists of a modulated dielectric, which is covered by a thin silver layer. The…

We investigate the growth conditions for thin (less than 200 nm) sputtered aluminum (Al) films. These coatings are needed for various applications, e.g. for advanced manufacturing processes in the aerospace industry or for nanostructures…

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