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EuRhAl4Si2, crystallizes in tetragonal crystal structure and orders antiferromagnetically at ~12 K. The isothermal magnetization along the two principle directions is highly anisotropic despite Eu2+ being an S-state ion. The variation of…

Strongly Correlated Electrons · Physics 2017-05-18 Arvind Maurya , A. Thamizhavel , P. Bonville , S. K. Dhar

We report the ferroelectric property in Tb2Ti2O7 pyrochlore, prepared by a two-step solid-state reaction method. A concave P-E (polarisation vs electric field) loop observed from 382 K confirms ferroelectricity, below which the loop remains…

Materials Science · Physics 2021-02-03 B. Santhosh Kumar , Rajesh Narayana Perumal , C. Venkateswaran

We present a detailed theoretical overview of the thermodynamic properties of the dipolar spin ice model, which has been shown to be an excellent quantitative descriptor of the Ising pyrochlore materials Dy_2Ti_2O_7 and Ho_2Ti_2O_7. We show…

Disordered Systems and Neural Networks · Physics 2015-06-24 Roger G. Melko , Matthew Enjalran , Byron C. den Hertog , Michel. J. P. Gingras

We report an extensive study on the zero field ground state of a powder sample of the pyrochlore $\mathrm{Yb_2Ti_2O_7}$. A sharp heat capacity anomaly that labels a low temperature phase transition in this material is observed at 280 mK.…

Pyrochlore iridates and pyrochlore ices are two families of materials where novel quantum phenomena are intertwined with strong spin-orbit coupling, substantial electron correlation and geometrical frustration. Motivated by the puzzling…

Strongly Correlated Electrons · Physics 2016-11-09 Gang Chen

Layered 5$d$ transition iridium oxides, Sr$_2$(Ir,Rh)O$_4$, are described as unconventional Mott insulators with strong spin-orbit coupling. The undoped compound, Sr$_2$IrO$_4$, is a nearly ideal two-dimensional pseudospin-$1/2$ Heisenberg…

Strongly Correlated Electrons · Physics 2017-05-02 Jaehong Jeong , Yvan Sidis , Alex Louat , Véronique Brouet , Philippe Bourges

Strong electronic interactions and spin orbit coupling can be conducive for realizing novel broken symmetry phases supporting quasiparticles with nontrivial band topology. 227 pyrochlore iridates provide a suitable material platform for…

Strongly Correlated Electrons · Physics 2017-02-22 Pallab Goswami , Bitan Roy , Sankar Das Sarma

The rich phase diagrams of magnetically frustrated pyrochlores have maintained a high level of interest over the past 20 years. To experimentally explore these phase diagrams requires a means of tuning the relevant interactions. One…

Strongly Correlated Electrons · Physics 2015-03-24 A. M. Hallas , A. M. Arevalo-Lopez , A. Z. Sharma , T. Munsie , J. P. Attfield , C. R. Wiebe , G. M. Luke

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond…

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

We have studied the effect of nonmagnetic Ti substitution Eu2(Ir1-xTix)2O7 with the help of electrical transport and magnetic measurement. The minor structural modification enhances the orbital overlapping and favours its electrical…

Strongly Correlated Electrons · Physics 2024-07-09 Sampad Mondal , B. Maji , M. Modak , Swapan K. Mandal , S. Banerjee

Electron spin resonance study of frustrated pyrochlore Gd2Ti2O7 is performed in a wide frequency band for a temperature range 0.4-30 K, which covers paramagnetic and magnetically ordered phases. The paramagnetic resonance reveals the…

Strongly Correlated Electrons · Physics 2012-02-02 S. S. Sosin , A. I. Smirnov , L. A. Prozorova , G. Balakrishnan , M. E. Zhitomirsky

We study the finite temperature and magnetic field phase diagram of electrons on the pyrochlore lattice subject to a local repulsion as a model for the pyrochlore iridates. We provide the most general symmetry-allowed Hamiltonian, including…

Strongly Correlated Electrons · Physics 2013-04-02 William Witczak-Krempa , Ara Go , Yong Baek Kim

We theoretically study the magnetic properties of pyrochlore iridate bilayer and trilayer thin films grown along the $[111]$ direction using a strong coupling approach. We find the ground state magnetic configurations on a mean field level…

Strongly Correlated Electrons · Physics 2018-09-19 Pontus Laurell , Gregory A. Fiete

The pyrochlore iridate In$_2$Ir$_2$O$_7$ is a strong $J_{\mathrm{eff}} = 1/2$ Mott insulator with frustrated magnetism. Despite the large trigonal crystal field, a small admixture of $J_{\mathrm{eff}} = 3/2$ component in the…

Strongly Correlated Electrons · Physics 2020-03-11 A. Krajewska , T. Takayama , R. Dinnebier , A. Yaresko , K. Ishii , M. Isobe , H. Takagi

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron…

Strongly Correlated Electrons · Physics 2014-04-11 J. Oitmaa , R. R. P. Singh , A. G. R. Day , B. V. Bagheri , M. J. P. Gingras

A comprehensive study of the structural properties of the heavily investigated rare-earth A2Ir2O7 series under extreme conditions is presented. The series is covered by studying iridates with A = Pr, Sm, Dy-Lu. Temperature- and…

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic…

Strongly Correlated Electrons · Physics 2017-04-25 H. Chu , L. Zhao , A. de la Torre , T. Hogan , S. D. Wilson , D. Hsieh

We study the prototype 5d pyrochlore iridate Y2Ir2O7 from first principles using the local density approximation and dynamical mean-field theory (LDA+DMFT). We map out the phase diagram in the space of temperature, onsite Coulomb repulsion…

Strongly Correlated Electrons · Physics 2015-10-14 Hiroshi Shinaoka , Shintaro Hoshino , Matthias Troyer , Philipp Werner

The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at…