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Related papers: Short-Lived Electron Transfer in Donor-Bridge-Acce…

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We consider the time-dependent electron transport through a quantum dot connected to multiple leads in the presence of the additional over-dot (bridge) tunnelling channels by using the evolution operator technique. Each terminal and quantum…

Mesoscale and Nanoscale Physics · Physics 2007-06-13 R. Taranko , T. Kwapinski , E. Taranko

We investigate the time an electronic excitation travels in a supermolecular setup using a measurement process in an open quantum-system framework. The approach is based on the stochastic Schr\"odinger equation and uses a Hamiltonian from…

Materials Science · Physics 2013-12-09 Dirk Hofmann , Heiko Appel , Massimiliano Di Ventra , Stephan Kümmel

Electron transmission through molecules and molecular interfaces has been a subject of intensive research due to recent interest in electron transfer phenomena underlying the operation of the scanning tunneling microscope (STM) on one hand,…

Condensed Matter · Physics 2015-06-24 Abraham Nitzan

Electron transfer (ET) across molecular chains including an impurity is studied based on a recently improved real-time path integral Monte Carlo (PIMC) approach [J. Chem. Phys. {\bf 121}, 12696 (2004)]. The reduced electronic dynamics is…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Lothar Muehlbacher , Joachim Ankerhold

An asymptotic scaling theory is presented using the conceptual basis of trapping-free subspace (i.e., orthogonal subspace) to establish the generic mechanism of optimal efficiency of excitation energy transfer (EET) in light-harvesting…

Quantum Physics · Physics 2013-05-16 Jianlan Wu , Jianshu Cao , Robert J. Silbey

It is proposed two models describing transport and absorbtion processes that occur in nanoscale fragments of electrical circuits, pulled adsorbed molecules, atomic or molecular chains connecting electrodes. Discrete chain model of a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 V. N. Evteev , M. V. Moiseenko , E. V. Zhuravel , E. Ya. Glushko

Here we study incoherent transport through molecular wire treated as a linear chain of absorbers, where the phase-breaking processes are modeled by the use of imaginary point-like potentials. The calculations are performed within a…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 Kamil Walczak

Using large-scale, real-time quantum dynamics calculations, we present a detailed analysis of electronic excitation transfer (EET) mechanisms in a multi-particle plasmonic nanoantenna system. Specifically, we utilize real-time,…

Mesoscale and Nanoscale Physics · Physics 2018-03-06 Niranjan V. Ilawe , M. Belén Oviedo , Bryan M. Wong

The scattering phase shift of an electron transferred through a quantum dot is studied within a model Hamiltonian, accounting for both the electron--electron interaction in the dot and a finite temperature. It is shown that, unlike in an…

Condensed Matter · Physics 2009-10-28 Yuval Oreg , Yuval Gefen

We develop a new approach to electron transport in mesoscopic systems by using a particular single-particle basis. Although this basis generates redundant many-particle amplitudes, it greatly simplifies the treatment. By using our method…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Shmuel Gurvitz

We propose a series of dissipation-assisted entanglement generation protocols that can be implemented on a trapped-ion quantum simulator. Our approach builds on the single-site molecular electron transfer (ET) model recently realized in the…

Quantum Physics · Physics 2025-07-10 Mingjian Zhu , Visal So , Guido Pagano , Han Pu

It is well known that the electron transfer (ET) reaction in donor-bridge-acceptor systems is much influenced by the bridge conformational changes. However, the importance of the dynamical contribution to the ET rate is still under debate.…

Chemical Physics · Physics 2009-03-31 Kazuhiro Tsusaka

Charge transfer is a fundamental process that underlies a multitude of phenomena in chemistry and biology. Recent advances in observing and manipulating charge and heat transport at the nanoscale, and recently developed techniques for…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Galen T. Craven , Abraham Nitzan

We present the formalism of Time-dependent Exchange Perturbation Theory (TDEPT) built to all orders of perturbation, for the arbitrary time dependency of perturbation. The theory takes into account the rearrangement of electrons among…

Quantum Physics · Physics 2015-04-13 Elena V. Orlenko , Tatiana Latychevskaia , Alexandr V. Evstafev , Fedor E. Orlenko

In this work we theoretically study steady state thermoelectric transport through a single-molecule junction with a long chain-like bridge. Electron transmission through the system is computed using a tight-binding model for the bridge. We…

Mesoscale and Nanoscale Physics · Physics 2018-03-02 Natalya A. Zimbovskaya , Abraham Nitzan

Electron transport characteristics are investigated through some molecular chains attached to two non-superconducting electrodes by the use of Green's function method. Here we do parametric calculations based on the tight-binding…

Mesoscale and Nanoscale Physics · Physics 2009-07-31 Santanu K. Maiti

We present a model of electron transport through a random distribution of interacting quantum dots embedded in a dielectric matrix to simulate realistic devices. The method underlying the model depends only on fundamental parameters of the…

Mesoscale and Nanoscale Physics · Physics 2012-07-25 S. Illera , J. D. Prades , A. Cirera , A. Cornet

Electron Transfer (ET) reactions are modeled by the dynamics of a quantum two-level system (representing the electronic state) coupled to a thermalized bath of classical harmonic oscillators (representing the nuclei degrees of freedom).…

Chemical Physics · Physics 2014-11-24 Serge Aubry

The multilayer multiconfiguration time-dependent Hartree theory within second quantization representation of the Fock space is applied to study correlated electron transport in models of single-molecule junctions. Extending previous work,…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Haobin Wang , Michael Thoss

We introduce a model of a nonlinear double-barrier structure, to describe in a simple way the effects of electron-electron scattering while remaining analytically tractable. The model is based on a generalized effective-mass equation where…

Condensed Matter · Physics 2009-10-28 Enrique Diez , Angel Sanchez , Francisco Dominguez-Adame