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The discovery of pressure-induced superconductivity in two- and three-layer Ruddlesden-Popper nickelates has generated significant interest in these materials as a platform for unconventional superconductivity. While their ground state…

The synthesis, structure, and elementary magnetic and electronic properties are reported for layered compounds of the type Na3-xMIr2O6 and Na3-xM2IrO6, where M is a transition metal from the 3d series (M=Zn, Cu, Ni, Co, Fe and Mn). The…

The pyrochlore insulator Yb2Ti2O7 has attracted the attention of experimentalists and theoreticians alike for about 15 years. Conflicting neutron diffraction data on the possible existence of magnetic Bragg reflections at low temperature…

Strongly Correlated Electrons · Physics 2016-08-26 A. Yaouanc , P. Dalmas de Reotier , L. Keller , B. Roessli , A. Forget

An archetypical layered topological insulator Bi$_2$Se$_3$ becomes superconductive upon doping with Sr, Nb or Cu. Superconducting properties of these materials in the presence of in-plane magnetic field demonstrate spontaneous symmetry…

We explore the relative strengths of spin orbit coupling and crystal field splitting in the Ir5+ compounds Ba2-xSrxYIrO6. In the case of strong spin orbit coupling and regular Ir5+ octahedra, one expects a nonmagnetic J = 0 state; in the…

Strongly Correlated Electrons · Physics 2016-03-29 Brendan F. Phelan , Elizabeth M. Seibel , Daniel Badoe , Weiwei Xie , R. J. Cava

Competition and cooperation between electron correlation and relativistic spin-orbit coupling give rise to diverse exotic quantum phenomena in solids. An illustrative example is spin-orbit entangled quantum liquids, which exhibit remarkable…

Strongly Correlated Electrons · Physics 2024-03-15 Yi-Feng Zhao , Seong-Hoon Jang , Yukitoshi Motome

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

Sr$_{2}$IrO$_{4}$ has often been described via a simple, one-band pseudo-spin 1/2 model, subject to electron-electron interactions, on a square lattice, fostering analogies with cuprate superconductors, believed to be well described by a…

We employ reactive molecular-beam epitaxy to synthesize the metastable perovskite SrIrO$_{3}$ and utilize {\it in situ} angle-resolved photoemission to reveal its electronic structure as an exotic narrow-band semimetal. We discover…

Strongly Correlated Electrons · Physics 2015-01-13 Y. F. Nie , P. D. C. King , C. H. Kim , M. Uchida , H. I. Wei , B. D. Faeth , J. P. Ruf , J. P. C. Ruff , L. Xie , X. Pan , C. J. Fennie , D. G. Schlom , K. M. Shen

The ground state properties and neutron structure factor for the two-dimensional antiferromagnet on the triangular lattice, with uni-directional anisotropy in the nearest-neighbor exchange couplings and a weak Dzyaloshinskii-Moriya (DM)…

Strongly Correlated Electrons · Physics 2009-11-11 Denis Dalidovich , Rastko Sknepnek , A. John Berlinsky , Junhua Zhang , Catherine Kallin

Iridium-based 5d transition-metal oxides are attractive candidates for the study of correlated electronic states due to the interplay of enhanced crystal-field, Coulomb and spin-orbit interaction energies. At ambient pressure, these…

Strongly Correlated Electrons · Physics 2014-06-05 D. A. Zocco , J. J. Hamlin , B. D. White , B. J. Kim , J. R. Jeffries , S. T. Weir , Y. K. Vohra , J. W. Allen , M. B. Maple

Correlated oxides can exhibit complex magnetic patterns, characterized by domains with vastly different size, shape and magnetic moment spanning the material. Understanding how magnetic domains form in the presence of chemical disorder and…

Strongly Correlated Electrons · Physics 2021-11-12 He Zhao , Zach Porter , Xiang Chen , Stephen D. Wilson , Ziqiang Wang , Ilija Zeljkovic

We report time-of-flight neutron scattering measurements of the magnetic spectrum of Tb3+ in Tb2Ti2O7. The data, which extend up to 120 meV and have calibrated intensity, enable us to consolidate and extend previous studies of the…

Strongly Correlated Electrons · Physics 2015-09-04 A. J. Princep , H. C. Walker , D. T. Adroja , D. Prabhakaran , A. T. Boothroyd

For the Sr2-xIrO4 system, recent work pointed out the abnormal electronic and magnetic properties around the critical point. Here, to understand Sr-vacancy effect on spin-orbit coupled Mott insulator Sr2IrO4, the electronic structure and…

Strongly Correlated Electrons · Physics 2019-01-07 Jie Cheng , Shengli Liu , Bin Li , Haiyun Wang , Yu Wang , Wei Xu

We probe the spectrum of elementary excitations in SrIrO$_3$ by using heterostructured [(SrIrO$_3$)$_m$/(SrTiO$_3$)$_l$] samples to approach the bulk limit. Our resonant inelastic x-ray scattering (RIXS) measurements at the Ir $L_3$-edge…

We report the single crystal study of the bulk magnetization and neutron scattering measurements on a quantum S=1/2 spin ladders system IPA-Cu(Cl0.95Br0.05)3with quenched disorder. In zero field, the disordered spin liquid phase is…

Strongly Correlated Electrons · Physics 2010-02-19 Tao Hong , A. Zheludev , H. Manaka , L. -P. Regnault

We investigate the bilayer Ruddlesden-Popper iridate Sr$_3$Ir$_2$O$_7$ by temperature-dependent angle-resolved photoemission. We find a narrow-gap correlated insulator, with spectral features indicative of a polaronic ground state,…

Strongly Correlated Electrons · Physics 2013-07-01 P. D. C. King , T. Takayama , A. Tamai , E. Rozbicki , S. McKeown Walker , M. Shi , L. Patthey , R. G. Moore , D. Lu , K. M. Shen , H. Takagi , F. Baumberger

The crystal structure of the candidate topological superconductor Cu$_x$Bi$_2$Se$_3$ was studied by single-crystal neutron diffraction using samples obtained by inserting the Cu dopant electrochemically. Neither structural refinements nor…

Superconductivity · Physics 2022-03-24 Tobias Fröhlich , Zhiwei Wang , Mahasweta Bagchi , Anne Stunault , Yoichi Ando , Markus Braden

The spin structure function of the neutron is traditionally determined by measuring the spin asymmetry of inclusive electron deep inelastic scattering (DIS) off polarized3He nuclei. In such experiments, nuclear effects can lead to large…

The monoclinic double-perovskite Sr2YRuO6 has recently gained a renewed interest in order to get a deeper insight into the exotic magnetic ground states associated with geometric frustration. Striking discrepancies between the spin order…

Materials Science · Physics 2016-04-19 P. L. Bernardo , L. Ghivelder , H. S. Amorim , J. J. Neumeier , S. Garcia