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Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J$_{eff}=1/2$ Mott insulating iridate Sr$_2$IrO$_4$. Comparisons are drawn between the correlated magnetism in this single…

Strongly Correlated Electrons · Physics 2013-04-09 Chetan Dhital , Tom Hogan , Z. Yamani , Clarina de la Cruz , Xiang Chen , Sovit Khadka , Zhensong Ren , Stephen D. Wilson

Neutron single crystal diffraction and rotational anisotropy optical second harmonic generation data are presented resolving the nature of the structural distortion realized in electron-doped (Sr$_{1-x}$La$_x$)$_3$Ir$_2$O$_7$ with $x=0.035$…

Strongly Correlated Electrons · Physics 2017-06-28 Tom Hogan , Xiaoping Wang , H. Chu , David Hsieh , Stephen D. Wilson

We use the bilayer twisted Hubbard model to study the low energy electronic structure of Sr3Ir2O7. Sr3Ir2O7 is suggested as a Mott insulator and described by the bilayer twisted pseudospin-1/2 model. The bilayer twists in Sr3Ir2O7 bring the…

Strongly Correlated Electrons · Physics 2012-10-09 Jia-Wei Mei

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

Strongly Correlated Electrons · Physics 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

This report presents azimuthal dependent and polarisation dependent x-ray resonant magnetic scattering at the Ir L3 edge for the bilayered iridate compound, Sr3Ir2O7. Two magnetic wave vectors, k1=(1/2,1/2,0) and k2=(1/2,-1/2,0), result in…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R Springell , H C Walker , A T Boothroyd , D Prabhakaran , S P Collins , D F McMorrow

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

We have carried out detailed bulk and local probe studies on the hexagonal oxides Ba3MIr2O9 (M=Sc,Y) where Ir is expected to have a fractional oxidation state of +4.5. In the structure, Ir-Ir dimers are arranged in an edge shared triangular…

Strongly Correlated Electrons · Physics 2014-05-06 Tusharkanti Dey , R. Kumar , A. V. Mahajan , S. D. Kaushik , V. Siruguri

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

We use single-crystal neutron diffraction to determine the crystal structure symmetry and the magnetic evolution in the rhodium doped iridates $\rm Sr_2Ir_{1-x}Rh_{x}O_4$ ($0\leq x \leq 0.16$). Throughout this doping range, the crystal…

The bilayered rhodium oxide Sr3Rh2O7 was synthesized by high-pressure and high-temperature heating techniques. The single-phase polycrystalline sample of Sr3Rh2O7 was characterized by measurements of magnetic susceptibility, electrical…

Superconductivity · Physics 2009-11-07 K. Yamaura , Q. Huang , D. P. Young , Y. Noguchi , E. Takayama-Muromachi

We report on the spin structure of the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ that could be directly determined by means of powder neutron diffraction. Our magnetic structure refinement unravels a so-called all-in/all-out magnetic structure…

Strongly Correlated Electrons · Physics 2016-10-14 H. Guo , C. Ritter , A. C. Komarek

This article reports a detailed x-ray resonant scattering study of the bilayer iridate compound, Sr3Ir2O7, at the Ir L2 and L3 edges. Resonant scattering at the Ir L3 edge has been used to determine that Sr3Ir2O7 is a long-range ordered…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R. Springell , H. C. Walker , A. T. Boothroyd , D. Prabhakaran , D. Wermeille , L. Bouchenoire , S. P. Collins , D. F. McMorrow

The low-energy electronic structure of the J_{eff}=1/2 spin-orbit insulator Sr3Ir2O7 has been studied by means of angle-resolved photoemission spectroscopy. A comparison of the results for bilayer Sr3Ir2O7 with available literature data for…

Strongly Correlated Electrons · Physics 2012-09-27 B. M. Wojek , M. H. Berntsen , S. Boseggia , A. T. Boothroyd , D. Prabhakaran , D. F. McMorrow , H. M. Rønnow , J. Chang , O. Tjernberg

The spin-orbit Mott insulator Sr3Ir2O7 provides a fascinating playground to explore insulator-metal transition driven by intertwined charge, spin, and lattice degrees of freedom. Here, we report high pressure electric resistance and…

Magnetic structures of the noncentrosymmetric magnet Sr$_2$MnSi$_2$O$_7$ were examined through neutron diffraction for powder and single-crystalline samples, as well as magnetometry measurements. All allowed magnetic structures under the…

Strongly Correlated Electrons · Physics 2024-10-08 Y. Nambu , M. Kawamata , X. Pang , H. Murakawa , M. Avdeev , H. Kimura , H. Masuda , N. Hanasaki , Y. Onose

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

Strongly Correlated Electrons · Physics 2013-05-30 Jean-Michel Carter , Hae-Young Kee

We report the first observation of two-dimensional incommensurate magnetic fluctuations in the layered metallic perovskite Sr3Ru2O7. The wavevectors where the magnetic fluctuations are strongest are different from those observed in the…

Strongly Correlated Electrons · Physics 2007-05-23 L. Capogna , E. M. Forgan , S. M. Hayden , A. Wildes , J. A. Duffy , A. P. Mackenzie , R. S. Perry , S. Ikeda , Y. Maeno , S. P. Brown

We have investigated the structural, electronic, and magnetic properties of the pyrochlore iridates Eu2Ir2O7 and Pr2Ir2O7 using a combination of resonant elastic x-ray scattering, x-ray powder diffraction, and resonant inelastic x-ray…

In spin ice research, small variations in structure or interactions drive a multitude of different behaviors, yet the collection of known materials relies heavily on the `227' pyrochlore structure. Here, we present thermodynamic, structural…

Disordered Systems and Neural Networks · Physics 2019-04-30 D. Reig-i-Plessis , S. V. Geldern , A. A. Aczel , D. Kochkov , B. K. Clark , G. J. MacDougall
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