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Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

The electronic band structure-controlled ultrafast demagnetization mechanism in Co2FexMn1-xSi Heusler alloy is underpinned by systematic variation of composition. We find the spin-flip scattering rate controlled by spin density of states at…

Materials Science · Physics 2020-07-01 Santanu Pan , Takeshi Seki , Koki Takanashi , Anjan Barman

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the…

The direct manipulation of spins via light may provide a path toward ultrafast energy-efficient devices. However, distinguishing the microscopic processes that can occur during ultrafast laser excitation in magnetic alloys is challenging.…

Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

The discovery of femtosecond laser-induced ultrafast demagnetization in 1996 opened a new field, femtomagnetism, in which magnetic order can be quenched on timescales shorter than a picosecond. This seminal observation revealed that angular…

Materials Science · Physics 2026-04-29 Quentin Remy , Stéphane Mangin

The dynamics of ultrafast demagnetisation in 3$d$ magnets is complicated by the presence of both spin ${\v S}$ and orbital ${\v L}$ angular momentum, with the microscopic mechanism by which the magnetic moment is redistributed to the…

Materials Science · Physics 2021-09-01 J. K. Dewhurst , S. Shallcross , P. Elliott , S. Eisebitt , C. v. Korff Schmising , Sangeeta Sharma

When a laser pulse excites a ferromagnet, its spin undergoes a dramatic change. The initial demagnetization process is very fast. Experimentally, it is found that the demagnetization time is related to the spin moment in the sample. In this…

Materials Science · Physics 2016-11-11 G. P. Zhang , M. S. Si , Thomas F. George

Induced by an ultra-short laser pulse, the electronic structure of a material undergoes strong modifications leading to a fast demagnetization in magnetic materials. Induced spin-flip transitions are one of the reasons for demagnetization,…

Materials Science · Physics 2024-04-29 Sergiy Mankovsky , Svitlana Polesya , Hubert Ebert

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

The microscopic origin of laser-induced ultrafast demagnetization remains an open question, to which the non-thermal electronic distribution plays a vital role at the initial stage. Herein, we investigate the connection between the…

Materials Science · Physics 2025-12-25 Yu-Hui Song , Huan-Cheng Yang , Kai Liu , Zhong-Yi Lu

Engineering and controlling heat and spin transport on the femtosecond time-scale in spintronic devices opens up new ways to manipulate magnetization with unprecedented speed. Yet the underlying reversal mechanisms remain poorly understood…

Mesoscale and Nanoscale Physics · Physics 2026-02-04 Harjinder Singh , Alberto Anadón , Junta Igarashi , Quentin Remy , Stéphane Mangin , Michel Hehn , Jon Gorchon , Gregory Malinowski

Electronic excitations in a ferromagnet can trigger ultrafast spin dynamics with potential applications in a speed increase in magnetic recording. The project investigates ultrafast magnetization dynamics, which is driven in metallic layers…

Materials Science · Physics 2010-07-06 Adrian Glaubitz

Laser induced ultrafast demagnetization is the process whereby the magnetic moment of a ferromagnetic material is seen to drop significantly on a timescale of $10-100$s of femtoseconds due to the application of a strong laser pulse. If this…

Materials Science · Physics 2016-01-20 P. Elliott , K. Krieger , J. K. Dewhurst , S. Sharma , E. K. U. Gross

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific…

Engineering of magnetic materials for developing better spintronic applications relies on the control of two key parameters: the spin polarization and the Gilbert damping responsible for the spin angular momentum dissipation. Both of them…

With density functional theory, studied are the local magnetic moments in Fe-Al alloys depending on concentration and Fe nearest environment. At zero temperature, the system can be in different states: ferromagnetic, antiferromagnetic and…

Materials Science · Physics 2009-11-13 A. K. Arzhnikov , L. V. Dobysheva , M. A. Timirgazin

It is now well established that a few femtosecond laser pulse will induce an ultrafast loss of moment in a magnetic material. Here we show that the opposite effect can also occur: an ultrafast increase in moment. Employing both…

The ultimate control of magnetic states of matter at femtosecond (or even faster) timescales defines one of the most pursued paradigm shifts for future information technology. In this context, ultrafast laser pulses developed into extremely…

Mesoscale and Nanoscale Physics · Physics 2022-03-15 Hanan Hamamera , Filipe Souza Mendes Guimarães , Manuel dos Santos Dias , Samir Lounis

A systematic investigation of spin injection behavior in Au/FM (FM = Fe and Ni) multilayers is performed using the superdiffusive spin transport theory. By exciting the nonmagnetic layer, the laser-induced hot electrons may transfer spin…

Mesoscale and Nanoscale Physics · Physics 2023-11-20 Wen-Tian Lu , Zhe Yuan , Xiaohong Xu
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