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Magnetism induced by external pressure ($p$) was studied in a FeSe crystal sample by means of muon-spin rotation. The magnetic transition changes from second-order to first-order for pressures exceeding the critical value $p_{{\rm…

Elucidating the microscopic origin of nematic order in iron-based superconducting materials is important because the interactions that drive nematic order may also mediate the Cooper pairing. Nematic order breaks fourfold rotational…

A hallmark of the iron-based superconductors is the strong coupling between magnetic, structural and electronic degrees of freedom. However, a universal picture of the normal state properties of these compounds has been confounded by recent…

Since its discovery, iron-based superconductivity has been known to develop near an antiferromagnetic order, but this paradigm fails in the iron chalcogenide FeSe, whose single-layer version holds the record for the highest superconducting…

Strongly Correlated Electrons · Physics 2020-06-22 Wen-Jun Hu , Hsin-Hua Lai , Shou-Shu Gong , Rong Yu , Elbio Dagotto , Qimiao Si

FeSe, despite being the structurally simplest compound in the family of iron-based superconductors, shows an astoundingly rich interplay of physical phenomena including nematicity and pressure-induced magnetism. Here, we present a…

We present $^{77}$Se-NMR measurements on single-crystalline FeSe under pressures up to 2 GPa. Based on the observation of the splitting and broadening of the NMR spectrum due to structural twin domains, we discovered that static, local…

Strongly Correlated Electrons · Physics 2017-12-13 P. Wiecki , M. Nandi , A. E. Böhmer , S. L. Bud'ko , P. C. Canfield , Y. Furukawa

The sulfur-substituted FeSe, FeSe$_{1-x}$S$_{x} $, is one of the unique systems that provides an independent tunability of nematicity, antiferromagnetism and superconductivity under pressure ($p$). Recently Rana et al. [Phys. Rev. B 101,…

Superconductivity · Physics 2023-04-28 K. Rana , D. V. Ambika , S. L. Bud'ko , A. E. Böhmer , P. C. Canfield , Y. Furukawa

We report high-pressure $^{77}$Se NMR studies on FeSe single crystals that reveal a prominent inhomogeneous NMR linewidth broadening upon cooling, with the magnetic field applied along the tetragonal [110] direction. The data indicate the…

Superconductivity · Physics 2017-09-29 P. S. Wang , P. Zhou , S. S. Sun , Y. Cui , T. R. Li , Hechang Lei , Ziqiang Wang , Weiqiang Yu

The sulfur substituted FeSe system, FeSe$_{1-x}$S$_{x}$, provides a versatile platform for studying the relationship between nematicity, antiferromagnetism, and superconductivity. Here, by nuclear magnetic resonance (NMR) and resistivity…

Strongly Correlated Electrons · Physics 2020-05-20 K. Rana , Li. Xiang , P. Wiecki , R. A. Ribeiro , G. G. Lesseux , A. E. Böhmer , S. L. Bud'ko , P. C. Canfield , Y. Furukawa

We report pressure-dependent neutron diffraction and muon spin relaxation/rotation measurements combined with first-principles calculations to investigate the structural, magnetic, and electronic properties of BaFe$_2$S$_3$ under pressure.…

Elucidating the nature of the magnetism of a high-temperature superconductor is crucial for establishing its pairing mechanism. The parent compounds of the cuprate and iron-pnictide superconductors exhibit N\'eel and stripe magnetic order,…

The angular-dependent magnetoresistance (AMR) of the ab plane is measured on the single crystals of FeSe1-xSx (x = 0, 0.07, 0.13 and 1) and FeSe1-yTey (y = 0.06, 0.61 and 1) at various temperatures under fields up to 9 T. A pronounced…

We report measurements of resistance and ac magnetic susceptibility on FeSe single crystals under high pressure up to 27.2 kbar. The structural phase transition is quickly suppressed with pressure, and the associated anomaly is not seen…

To elucidate the origin of nematic order in FeSe, we performed field-dependent 77Se-NMR measurements on single crystals of FeSe. We observed orbital ordering from the splitting of the NMR spectra and Knight shift and a suppression of it…

Temperature dependence of resistivity under high pressures with magnetic fields parallel and perpendicular to the FeSe planes are measured in FeSe single crystals. It is found that the structural transition (nematic) temperature is…

Superconductivity · Physics 2019-03-06 Guan-Yu Chen , Enyu Wang , Xiyu Zhu , Hai-Hu Wen

A fundamental issue concerning iron-based superconductivity is the roles of electronic nematicity and magnetism in realising high transition temperature ($T_{\rm c}$). To address this issue, FeSe is a key material, as it exhibits a unique…

The recent study of $^{77}$Se nuclear magnetic resonance (NMR) in a $\beta$-FeSe single crystal proposed that ferro-orbital order breaks the $90^\circ$ $C_4$ rotational symmetry, driving nematic ordering. Here, we report an NMR study of the…

Superconductivity · Physics 2016-05-18 S. -H. Baek , D. V. Efremov , J. M. Ok , J. S. Kim , Jeroen van den Brink , B. Büchner

The unusual quantum-disordered magnetic ground state intertwined with superconductivity and electronic nematicity in FeSe has been a research focus in iron-based superconductors. However, the intrinsic spin excitations across the entire…

Iron-based superconductors are well known for their complex interplay between structure, magnetism and superconductivity. FeSe offers a particularly fascinating example. This material has been intensely discussed because of its extended…

Superconductivity · Physics 2018-01-04 Anna E. Böhmer , Andreas Kreisel

The interplay between the nematic order and magnetism in FeSe is not yet well understood. There is a controversy concerning the relationship between orbital and spin degrees of freedom in FeSe and their relevance for superconductivity. Here…

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