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Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

We investigate the performance of entangled coherent state for quantum enhanced phase estimation. An exact analytical expression of quantum Fisher information is derived to show the role of photon losses on the ultimate phase sensitivity.…

Quantum Physics · Physics 2014-04-07 Y. M. Zhang , X. W. Li , W. Yang , G. R. Jin

Quantum phenomena such as entanglement can improve fundamental limits on the sensitivity of a measurement probe. In optical interferometry, a probe consisting of $N$ entangled photons provides up to a $\sqrt{N}$ enhancement in phase…

We propose a novel quantum diffraction imaging technique whereby one photon of an entangled pair is diffracted off a sample and detected in coincidence with its twin. The image is obtained by scanning the photon that did not interact with…

Quantum Physics · Physics 2019-09-04 Shahaf Asban , Konstantin E. Dorfman , Shaul Mukamel

Phase measurement using a lossless Mach-Zehnder interferometer with certain entangled $N$-photon states can lead to a phase sensitivity of the order of 1/N, the Heisenberg limit. However, previously considered output measurement schemes are…

Quantum Physics · Physics 2009-11-13 Yang Gao , Hwang Lee

Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission…

Quantum Physics · Physics 2020-08-10 Akihito Ishizaki

We optimize two-mode, entangled, number states of light in the presence of loss in order to maximize the extraction of the available phase information in an interferometer. Our approach optimizes over the entire available input Hilbert…

Precise measurements are the key to advances in all fields of science. Quantum entanglement shows higher sensitivity than achievable by classical methods. Most physical quantities including position, displacement, distance, angle, and…

Quantum Physics · Physics 2017-07-05 Zhi-Yuan Zhou , Shi-Long Liu , Shi-Kai Liu , Yin-Hai Li , Dong-Sheng Ding , Guang-Can Guo , Bao-Sen Shi

Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…

We investigate the phase enhancement of quantum states subject to non-linear phase shifts. The optimal phase estimation of even entangled coherent states (ECSs) is shown to be better than that of NOON states and of odd ECS states with the…

Quantum Physics · Physics 2012-10-25 Jaewoo Joo , Kimin Park , Hyunseok Jeong , William J. Munro , Kae Nemoto , Timothy P. Spiller

Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

The high-precision interferometric measurement of an unknown phase is the basis for metrology in many areas of science and technology. Quantum entanglement provides an increase in sensitivity, but present techniques have only surpassed the…

Quantum Physics · Physics 2011-01-25 G. Y. Xiang , B. L. Higgins , D. W. Berry , H. M. Wiseman , G. J. Pryde

Quantum entanglement and squeezing have significantly improved phase estimation and imaging in interferometric settings beyond the classical limits. However, for a wide class of non-interferometric phase imaging/retrieval methods vastly…

In virtual-state spectroscopy, information about the energy-level structure of an arbitrary sample is retrieved by Fourier transforming sets of measured two-photon absorption probabilities of entangled photon pairs where the degree of…

Quantum Physics · Physics 2021-08-04 Lutz Mertenskötter , Kurt Busch , Roberto de J. León-Montiel

We describe two-photon absorption processes excited by entangled pairs, but not by non-entangled pairs of the same energy and polarization. Photon states are selected for destructive interference in the non-entangled process between…

Quantum Physics · Physics 2010-12-21 Keith Kastella , Ralph S. Conti

We experimentally demonstrate a general criterion to identify entangled states useful for the estimation of an unknown phase shift with a sensitivity higher than the shot-noise limit. We show how to exploit this entanglement on the examples…

Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…

Entangled multi-photon states have the potential to provide improved measurement accuracy, but are sensitive to photon loss. It is possible to calculate ideal loss-resistant states that maximize the Fisher information, but it is unclear how…

Quantum Physics · Physics 2014-09-04 Hossein T. Dinani , Dominic W. Berry

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen
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