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We demonstrate a quasi optical cycling for the $X(v=0)\to A(v'=0)$ transition and a radiative force induced deflection on the buffer-gas cooled BaF molecular beam. The laser induced fluorescence enhancement with additional sidebands and a…

Atomic Physics · Physics 2017-11-15 Tao Chen , Wenhao Bu , Bo Yan

We present experimental results from a new scheme for magneto-optically trapping strontium monofluoride (SrF) molecules, which provides increased confinement compared to our original work. The improved trap employs a new approach to…

Atomic Physics · Physics 2015-06-23 D. J. McCarron , E. B. Norrgard , M. H. Steinecker , D. DeMille

Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the…

Atomic Physics · Physics 2020-12-18 Konrad Wenz , Ivan Kozyryev , Rees L. McNally , Leland Aldridge , Tanya Zelevinsky

Today, it is well known that light possesses a linear momentum which is along the propagation direction. Besides, scientists also discovered that light can possess an angular momentum (AM), a spin angular momentum (SAM) associated with…

Optics · Physics 2020-07-15 Andy Chong , Chenhao Wan , Jian Chen , Qiwen Zhan

We demonstrate a scheme for magneto-optically trapping strontium monofluoride (SrF) molecules at temperatures one order of magnitude lower and phase space densities three orders of magnitude higher than obtained previously with laser-cooled…

Atomic Physics · Physics 2016-02-17 E. B. Norrgard , D. J. McCarron , M. H. Steinecker , M. R. Tarbutt , D. DeMille

We demonstrate that a bichromatic standing-wave laser field can exert a significantly larger force on a molecule than ordinary radiation pressure. Our experiment measures the deflection of a pulsed supersonic beam of CaF molecules by a…

Atomic Physics · Physics 2018-08-22 S. E. Galica , L. Aldridge , D. J. McCarron , E. E. Eyler , P. L Gould

The vibrational branching ratios of SrOH for radiative decay to the ground electronic state, $X^{2}\Sigma^{+}$, from the first two electronically excited states, $A^{2}\Pi$ and $B^{2}\Sigma^{+}$, are determined experimentally at the…

Atomic Physics · Physics 2022-08-17 Zack Lasner , Annika Lunstad , Chaoqun Zhang , Lan Cheng , John M. Doyle

We propose and demonstrate a novel technique that combines Raman scattering and optical cycling in molecules with diagonal Franck-Condon factors. This resonance Raman optical cycling manipulates molecules to behave like efficient…

Atomic Physics · Physics 2021-08-26 J. C. Shaw , J. C. Schnaubelt , D. J. McCarron

We demonstrate production of cold atomic strontium (Sr) and strontium-containing molecules (SrOH) in a cryogenic buffer gas beam source via direct heating of strontium oxide (SrO) with 30 mJ laser pulses several milliseconds long.…

Atomic Physics · Physics 2024-07-23 Andrew Winnicki , Zack D. Lasner , John M. Doyle

In cavity optomechanics, radiation pressure and photothermal forces are widely utilized to cool and control micromechanical motion, with applications ranging from precision sensing and quantum information to fundamental science. Here, we…

Quantum Physics · Physics 2016-05-04 D. L. McAuslan , G. I. Harris , C. Baker , Y. Sachkou , X. He , E. Sheridan , W. P. Bowen

Photodetachment spectroscopy of OH- and H3O2- anions has been performed in a cryogenic 22-pole radiofrequency multipole trap. Measurements of the detachment cross section as a function of laser frequency near threshold have been analysed.…

Chemical Physics · Physics 2014-08-22 R. Otto , A. von Zastrow , T. Best , R. Wester

We investigated the optical cycling effect of the $\mathrm{X}^2\Sigma(v=0,\ N=1^-) - \mathrm{A}^2\Pi_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in…

Atomic and Molecular Clusters · Physics 2025-07-08 Kikyeong Kwon , Seunghwan Roh , Youngju Cho , Yongwoong Lee , Eunmi Chae

A new scheme of three-dimensional (3D) all-optical (nonmagnetic) cooling and trapping of resonant atoms, based on using of so-called rectified radiation forces in non-monochromatic light fields is presented. It can be applied to the atoms…

Optics · Physics 2010-09-17 I. V. Krasnov

Recently a number of diatomic and polyatomics molecules has been identified as a prospective systems for Doppler/Sisyphus cooling. Doppler/Sisyphus cooling allows to decrease the kinetic energy of molecules down to microkelvin temperatures…

Chemical Physics · Physics 2017-11-22 T. A. Isaev , A. V. Zaitsevskii , E. Eliav

A full density-matrix simulation is performed for optical deflection of a barium monofluoride ($^{138}$Ba$^{19}$F) beam using the bichromatic force, which employs pairs of counter-propagating laser beams that are offset in frequency. We…

Atomic Physics · Physics 2023-07-26 A. Marsman , M. Horbatsch , E. A. Hessels

We report a study on light force on a beam of neutral two-level atoms superimposed upon a few-cycle pulsed Gaussian laser field under both resonant and off-resonant condition. The phenomena of focusing, defocusing and steering of the…

Atomic Physics · Physics 2013-05-29 Parvendra Kumar , Amarendra K. Sarma

We consider high energy electron scattering by hydrogen atoms in the presence of a laser field of moderate power and higher frequencies. If the field is a superposition of a linearly and a circularly polarized laser beam in a particular…

Atomic Physics · Physics 2013-03-07 Aurelia Cionga , Fritz Ehlotzky , Gabriela Zloh

We consider deflection of rotating symmetric molecules by inhomogeneous optical and static electric fields, compare results with the case of linear molecules, and find new singularities in the distribution of the scattering angle.…

Chemical Physics · Physics 2015-05-28 Erez Gershnabel , Ilya Sh. Averbukh

We examine the prospects for utilizing the optical bichromatic force (BCF) to greatly enhance laser deceleration and cooling for near-cycling transitions in small molecules. We discuss the expected behavior of the BCF in near-cycling…

Atomic Physics · Physics 2015-05-30 M. A. Chieda , E. E. Eyler

We propose a scheme to transfer molecules from a slow beam into an optical trap using only a single photon absorption and emission cycle. The efficiency of such a scheme is numerically explored for BaF using realistic experimental…