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Related papers: \textit{Ab initio} study of reactive collisions be…

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We performed calculations of the optimized structure, harmonic vibrational frequencies and dissociation energies of RbOH and its anion, and investigate the interactions between Rb and OH$^-$ leading to possible associative detachment…

Chemical Physics · Physics 2015-06-16 Jason N. Byrd , H. Harvey Michels , John A. Montgomery , Robin Côté

Reaction rate constants and cross sections are computed for the radiative association of carbon cations ($\text{C}^+$) and fluorine atoms ($\text{F}$) in their ground states. We consider reactions through the electronic transition $1^1\Pi…

Chemical Physics · Physics 2015-10-01 Jonatan Öström , Dmitry S. Bezrukov , Gunnar Nyman , Magnus Gustafsson

Light-assisted reactive collisions between laser-cooled Ba+ ions and Rb atoms were studied in an ion-atom hybrid trap. The reaction rate was found to strongly depend on the electronic state of the reaction partners with the largest rate…

Atomic Physics · Physics 2015-06-12 Felix H. J. Hall , Mireille Aymar , Maurice Raoult , Olivier Dulieu , Stefan Willitsch

We have computed ab inito cross sections for cold collisions of Rb atoms with OH radicals. We predict collision rate constants of order 10^{-11} cm^3/s at temperatures in the range 10-100 mK at which molecules have already been produced…

Atomic Physics · Physics 2009-11-13 M. Lara , J. L. Bohn , D. Potter , P. Soldan , J. Hutson

Using a merged beams apparatus we have measured the associative detachment (AD) reaction of ${\rm H}^- + {\rm H} \to {\rm H}_2 + e^-$ for relative collision energies up to \textit{E}$_{\rm{r}} \leq 4.83$ eV. These data extend above the 1 eV…

Atomic Physics · Physics 2015-05-30 K. A. Miller , H. Bruhns , J. Eliášek , M. Čížek , H. Kreckel , X. Urbain , D. W. Savin

The dynamics of the reaction H + OH $\to$ O (3P) + H2 have been studied in a series of quasi-classical trajectory (QCT) calculations and transition state theory (TST) methods using high quality 3A' and 3A'' potential energy surfaces (PESs).…

Solar and Stellar Astrophysics · Physics 2014-02-27 Xiaohu Li , Carina Arasa , Marc C. van Hemert , Ewine F. van Dishoeck

We use quantum and classical adiabatic capture theories to study the chemical reaction Li + CaH -> LiH + Ca. Using a recently developed ab initio potential energy surface, which provides an accurate representation of long-range interactions…

Atomic Physics · Physics 2015-06-23 Timur V. Tscherbul , Alexei A. Buchachenko

We analyze reactive collisions of a single Ba$^+$ ion in contact with an ultracold gas of Rb atoms at low three-body collision energies of 2.2(9) mK$\times k_{\mathrm{B}}$. Mapping out the Ba$^+$ loss rate dependence on the Rb atom density…

Atomic Physics · Physics 2016-09-14 Artjom Krükow , Amir Mohammadi , Arne Härter , Johannes Hecker Denschlag

The reaction dynamics of O(3P) + O2(3Sigma_g-) collisions in the O3(1A') electronic ground state is characterized on a high-level MRCI+Q/aug-cc-pVQZ potential energy surface represented as a reproducing kernel. For the atom exchange…

Chemical Physics · Physics 2026-03-12 Raidel Martin-Barrios , Abhirami Vijayakumar , Jingchun Wang , Markus Meuwly

We present a theoretical investigation of cold reactive and non-reactive collisions of Li and Rb atoms with C$_{2}^{-}$. The potential energy surfaces for the singlet and triplet states of the Li--C$_{2}^{-}$ and Rb--C$_{2}^{-}$ systems…

Atomic Physics · Physics 2019-04-17 Milaim Kas , Jérôme Loreau , Jacques Liévin , Nathalie Vaeck

OH radicals play a key role as an intermediate in the water formation chemistry of the interstellar medium. For example the reaction of OH radicals with H$_2$ molecules is among the final steps in the astrochemical reaction network starting…

Astrophysics of Galaxies · Physics 2017-08-21 Jan Meisner , Thanja Lamberts , Johannes Kästner

A theoretical method for the estimation of cross sections and rates for excitation and charge transfer processes in low-energy hydrogen atom collisions with neutral atoms, based on an asymptotic two-electron model of ionic-covalent…

Atomic Physics · Physics 2016-05-04 Paul S. Barklem

We present a theoretical investigation of reactive and non-reactive collisions of Li and Rb atoms with C$_{2}^{-}$ molecular anions at low temperatures in the context of sympathetic cooling in hybrid trap experiments. Based on recently…

Chemical Physics · Physics 2020-08-26 M. Kas , J. Liévin , N. Vaeck , J. Loreau

The energy dependence of the rate coefficient of the H$_2^+\ + {\rm H}_2 \rightarrow {\rm H}_3^+ + {\rm H}$ reaction has been measured in the range of collision energies between $k_\mathrm{B}\cdot 10$ K and $k_\mathrm{B}\cdot 300$ mK. A…

We present a theoretical investigation of the hydrated hydroxide anion clusters OH(H$_{2}$O)$_{n}^{-}$ and of the collisional complexes H-OH(H$_{2}$O)$_{n}^{-}$ and Rb-OH(H$_{2}$O)$_{n}^{-}$ (with n$=1-4$). The MP2 and CCSD(T) methods are…

Chemical Physics · Physics 2019-10-16 Milaim Kas , Jérôme Loreau , Jacques Liévin , Nathalie Vaeck

We calculated reaction rate constants including atom tunneling of the reaction of dihydrogen with the hydroxy radical down to a temperature of 50 K. Instanton theory and canonical variational theory with microcanonical optimized…

Chemical Physics · Physics 2016-05-31 Jan Meisner , Johannes Kästner

We employ an accurate, ab initio potential energy surface (PES) which describes the electronic interaction energy between the molecular anion OH$^-$ ($^1\Sigma^+$) and the neutral rubidium atom Rb ($^2S$), to evaluate the elastic and…

Atomic Physics · Physics 2018-07-31 L. González-Sánchez , F. Carelli , F. A. Gianturco , R. Wester

The gas-phase reaction of $\mathrm{O}+\mathrm{H}_3^+$ has two exothermic product channels, $\mathrm{OH}^+ +\mathrm{H}_2$ and $\mathrm{H}_2\mathrm{O}^+ +\mathrm{H}$. In the present study, we analyze experimental data from a merged-beams…

Instrumentation and Methods for Astrophysics · Physics 2022-03-04 Pierre-Michel Hillenbrand , Nathalie de Ruette , Xavier Urbain , Daniel Wolf Savin

The tunneling reaction H$_2$ + D$^-$ $\rightarrow$ HD + H$^-$ was studied in a recent experimental work at low temperatures (10, 19, and 23~K) by Endres {\it et al.}, Phys. Rev. A {\bf 95}, 022706 (2017). An upper limit of the rate…

We present calculated cross sections and rate coefficients for the formation of the dicarbon cation (C$_2^+$) by the radiative association process in collisions of a C$(^3P)$ atom and a C$^+(^2P^o)$ ion. Molecular structure calculations for…

Atomic Physics · Physics 2019-10-24 James F. Babb , R. T. Smyth , B. M. McLaughlin
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