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The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

Multi-photon emitters are a sought-after resource in quantum photonics. Nonlinear interactions between a multi-level atomic system and a coherent drive can lead to resonant two-photon emission, but harvesting light from this process has…

Two-photon absorption in molecules, of significance for high-resolution imaging applications, is typically characterised with low cross sections. To enhance the TPA signal, one effective approach exploits plasmonic enhancement. For this…

Optics · Physics 2024-08-28 Saeid Izadshenas , Karolina Słowik

We propose a novel scheme of photon upconversion based on harnessing the energy of plasmonic hot carriers. Low-energy photons excite hot electrons and hot holes in a plasmonic nanoparticle, which are then injected into an adjacent…

Optics · Physics 2015-11-17 Gururaj V. Naik , Jennifer A. Dionne

We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with conventional absorption peak at frequency close to intersubband…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Dai , M. E. Raikh , T. V. Shahbazyan

The light-matter quantum interface that can create quantum-correlations or entanglement between a photon and one atomic collective excitation is a fundamental building block for a quantum repeater. The intrinsic limit is that the…

Quantum Physics · Physics 2017-10-04 Long Tian , Zhongxiao Xu , Lirong Chen , Wei Ge , Haoxiang Yuan , Yafei Wen , Shengzhi Wang , Shujing Li , Hai Wang

We investigate the photon statistics, entanglement and squeezing of a pn-junction sandwiched between two superconducting leads, and show that such an electrically-driven photon pump generates correlated and entangled pairs of photons. In…

Mesoscale and Nanoscale Physics · Physics 2014-03-14 Paul Baireuther , Peter P. Orth , Ilya Vekhter , Jörg Schmalian

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky

A new type of artificial molecule is proposed, which consists of coupled defect atoms in photonic crystals, named as photonic molecule. Within the major band gap, the photonic molecule confines the resonant modes that are closely analogous…

Optics · Physics 2007-05-23 Bin-Shei Lin

The rotating-wave approximation to light-matter interactions is widely used in the quantum electrodynamics Hamiltonian; however, its validity has long been a matter of debate. In this article, we explore the impact of the rotating-wave…

Quantum Physics · Physics 2024-03-04 Yi-Ting Chuang , Liang-Yan Hsu

In this work, we provide an overview of how well-established concepts in the fields of quantum chemistry and material sciences have to be adapted when the quantum nature of light becomes important in correlated matter-photon problems.…

Quantum Physics · Physics 2017-04-12 Johannes Flick , Michael Ruggenthaler , Heiko Appel , Angel Rubio

We consider ramifications of the use of high speed light modulators to questions of correlation and measurement of time-energy entangled photons. Using phase modulators, we find that temporal modulation of one photon of an entangled pair,…

Quantum Physics · Physics 2009-11-13 S. E. Harris

By using a quantized input light, we theoretically revisit the coherent two-color photo-association process in an atomic Bose-Einstein condensate. Under the single-mode approximations, we show two interesting regimes of the light…

Quantum Physics · Physics 2007-05-23 Hui Jing , Ming-Sheng Zhan

We discuss two-photon correlations from the side peaks that are formed when a two-level system emitter is driven coherently, with a detuning between the driving source and the emitter (quasi-resonance fluorescence). We do so in the context…

Quantum Physics · Physics 2023-05-03 Eduardo Zubizarreta Casalengua , Elena del Valle , Fabrice P. Laussy

We present a detailed theoretical analysis of a weakly driven multimode optomechanical system, in which two optical modes are strongly and near-resonantly coupled to a single mechanical mode via a three-wave mixing interaction. We calculate…

Quantum Physics · Physics 2013-04-12 P. Kómár , S. D. Bennett , K. Stannigel , S. J. M. Habraken , P. Rabl , P. Zoller , M. D. Lukin

Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

The time-energy entanglement of down-converted photon pairs is particularly difficult to characterize because direct measurements of photon arrival times are limited by the temporal resolution of photon detection. Here, we explore an…

Quantum Physics · Physics 2013-04-12 Changliang Ren , Holger F. Hofmann

High-dimensional entanglement in the form of transverse spatial correlation between a pair of photons generated via spontaneous parametric downconversion is not only a valuable resource in many academic and real-life applications but also…

Quantum Physics · Physics 2025-08-18 Rounak Chatterjee , Vikas S Bhat , Kiran Bajar , Sushil Mujumdar

Directing indistinguishable photons from one input port into separate output ports is a fundamental operation in quantum information processing. The simplest scheme for achieving routing beyond random chance uses the photon blockade effect…

Quantum Physics · Physics 2023-05-03 Harjot Singh , Jasvith Raj Basani , Edo Waks

Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

Atomic and Molecular Clusters · Physics 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost