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Observing nonlinear optical quantum effects or implementing quantum information protocols using nonlinear optics requires moving to ever-smaller input light intensities. However, low light intensities generally mean weak optical…

Quantum Physics · Physics 2014-10-15 Audrey Dot , Evan Meyer-Scott , Raja Ahmad , Martin Rochette , Thomas Jennewein

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

Atomic Physics · Physics 2015-05-27 C. Müller , A. B. Voitkiv

We demonstrate the formation of a single RbCs molecule during the merging of two optical tweezers, one containing a single Rb atom and the other a single Cs atom. Both atoms are initially predominantly in the motional ground states of their…

The energetic positions of molecular electronic states at molecule/electrode interfaces are crucial factors for determining the transport and optoelectronic properties of molecular junctions. Strong light--matter coupling offers a potential…

Mesoscale and Nanoscale Physics · Physics 2023-05-10 Kuniyuki Miwa , Souichi Sakamoto , Akihito Ishizaki

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency…

The junction of a scanning tunneling microscope (STM) operating in the tunneling regime was irradiated with femtosecond laser pulses. A photo-excited hot electron in the STM tip resonantly tunnels into an excited state of a single molecule…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shiwei Wu , Wilson Ho

Single--photon which is initially uncorrelated with atom, will evolve to be entangled with the atom on their continuous kinetic variables in the process of resonant scattering. We find the relations between the entanglement and their…

Quantum Physics · Physics 2007-05-23 Rui Guo , Hong Guo

We study the collective phenomenon in the scattering of a single-photon by one or two layers of two-level atoms. By modeling the photon dispersion with a two-dimensional (2D) coupled cavity array, we analytically derive the scattering…

Quantum Physics · Physics 2013-07-23 D. Z. Xu , Yong Li , C. P. Sun , Peng Zhang

Multi-photon absorption is a well-known phenomenon. With atom lasers a similar process could take place for massive particles, the ionization of an atom or molecule by the successive interaction with various particles. This process would…

Quantum Physics · Physics 2009-11-13 Pedro Sancho

We show that the two-photon transition rates of quantum dots coupled to nanocavities are enhanced by up to 8 orders of magnitude relative to quantum dots in bulk host. We then propose how to take advantage of this enhancement to implement…

Quantum Physics · Physics 2009-07-02 Ziliang Lin , Jelena Vuckovic

It depends. For a single molecule interacting with one mode of a biphoton probe, we show that the spectroscopic information has three contributions, only one of which is a genuine two-photon contribution. When all the scattered light can be…

Quantum Physics · Physics 2024-04-16 Aiman Khan , Francesco Albarelli , Animesh Datta

We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction…

Quantum Physics · Physics 2010-04-12 Hao You , S. M. Hendrickson , J. D. Franson

By combining genetic algorithm and a spatial light modulator we theoretically analyse how to improve a two-photon cascade absorption in atomic ensembles, inspecting the impact of various configurations and parameters in the optimized phase…

Atomic Physics · Physics 2026-02-24 L. B. A. Mélo , Daniel Felinto , Marcio H. G. de Miranda

We demonstrate two-photon interference using two remote single molecules as bright solid-state sources of indistinguishable photons. By varying the transition frequency and spectral width of one molecule, we tune and explore the effect of…

Quantum Physics · Physics 2015-05-14 R. Lettow , Y. L. A. Rezus , A. Renn , G. Zumofen , E. Ikonen , S. Goetzinger , V. Sandoghdar

Photoionization of an atom $A$, in the presence of a neighboring atom $B$, can proceed via resonant excitation of $B$ with subsequent energy transfer to $A$ through two-center electron-electron correlation. We demonstrate that this…

Atomic Physics · Physics 2015-05-19 B. Najjari , A. B. Voitkiv , C. Müller

We study the two-photon scattering processes in a one-dimensional waveguide coupled to a two- or three-level giant atom, respectively. The accumulated phase shift between the two coupling points can be utilized to alter the scattering…

Quantum Physics · Physics 2023-11-30 Wenju Gu , He Huang , Zhen Yi , Lei Chen , Lihui Sun , Huatang Tan

Optical emitters strongly coupled to photons propagating in one-dimensional waveguides are a promising platform for optical quantum information processing. Here, we present a theoretical study of the scattering of two indistinguishable…

Quantum Physics · Physics 2016-03-24 Alexandre Roulet , Huy Nguyen Le , Valerio Scarani

The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…

Chemical Physics · Physics 2015-06-15 C T L Smeenk , L Arissian , A V Sokolov , M Spanner , K F Lee , A Staudte , D M Villeneuve , P B Corkum

We investigate the intrinsic microscopic mechanism of photon upconversion in air-suspended single-walled carbon nanotubes through photoluminescence and upconversion photoluminescence spectroscopy. Nearly linear excitation power dependence…

Mesoscale and Nanoscale Physics · Physics 2024-10-14 Daichi Kozawa , Shun Fujii , Yuichiro K. Kato

We theoretically examine photoassociation of a non-ideal Bose-Einstein condensate, focusing on evidence for a macroscopic superposition of atoms and molecules. This problem raises an interest because, rather than two states of a given…

Soft Condensed Matter · Physics 2009-11-07 John Calsamiglia , Matt Mackie , Kalle-Antti Suominen