Related papers: Attosecond pulse characterization with coherent Ry…
Applying a magnetic field as a method for tuning the frequency of Autler-Townes splitting for Rydberg electrometry has recently been demonstrated. In this paper we provide a theoretical understanding of EIT signals in the presence of a…
We investigate the quantum dynamics of ultra-long-range trilobite molecules exposed to homogeneous electric fields. A trilobite molecule consists of a Rydberg atom and a ground-state atom, which is trapped at large internuclear distances in…
An autoionizing resonance in molecular N$_2$ is excited by an ultrashort XUV pulse and probed by a subsequent weak IR pulse, which ionizes the contributing Rydberg states. Time- and angular-resolved photoelectron spectra recorded with a…
Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…
Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of…
We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.
Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…
A detection scheme for characterizing high-energy $\gamma$-ray pulses down to the zeptosecond timescale is proposed. In contrast to existing attosecond metrology techniques, our method is not limited by atomic shell physics and therefore…
Attosecond ionization time-delays at photoelectron energies above typically 10 eV are usually interpreted using the so called asymptotic approximation as a sum of the atomic or molecular delays with a universal laser-induced contribution.…
Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…
The anisotropic Dicke model reveals the important role that counter-rotating wave terms play in the coupling between light and two level atoms. It is intriguing to generate the model to the strongly correlated many body case, where the…
We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…
We demonstrate a multiphoton Rydberg dark resonance where a Lambda-system is coupled to a Rydberg state. This N-type level scheme combines the ability to slow and store light pulses associated with long lived ground state superpositions,…
The quest to realize topological band structures in artificial matter is strongly focused on lattice systems, and only quantum Hall physics is known to appear naturally also in the continuum. In this letter, we present a proposal based on a…
Temporal pulse characterization methods can often not be applied to UV pulses due to the lack of suitable nonlinear crystals and very low pulse energies. Here, a method is introduced for the characterization of two unknown and independent…
Controlling strongly interacting many-body systems enables the creation of tailored quantum matter, with properties transcending those based solely on single particle physics. Atomic ensembles which are optically driven to a Rydberg state…
Relativistic surface high harmonics have been considered a unique source for the generation of intense isolated attosecond pulses in the extreme ultra-violet (XUV) and X-ray spectral range. However, its experimental realization is still a…
We present measurements on pulsed four-wave mixing involving a Rydberg state in an atomic vapor cell. The excitation to the Rydberg state is conducted by a pulsed two-photon excitation on the nanosecond timescale that is combined with a…
The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…
We present an ab initio approach to solve the time-dependent Schr\"odinger equation to treat electron and photon impact multiple ionization of atoms or molecules. It combines the already known time scaled coordinate method with a new high…