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We report on a precision measurement of the $(5\mathrm{p})^{5}6\mathrm{p} \, [1/2]_{0}\leftarrow (5\mathrm{p})^{6} \, ^{1}\mathrm{S}_{0}$ transition wavenumber of Xe by Doppler-free two-photon spectroscopy using…

Atomic Physics · Physics 2025-09-11 M. H. Rayment , R. Stech , F. Merkt

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

We provide a basis for the laser intensity dependence of the momentum distributions of electrons and ions arising from strong-field non-sequential double ionization (NSDI) at intensities in the range $I=1-6.5 \times 10^{14} W/cm^2$. To do…

Atomic Physics · Physics 2007-05-23 Phay J. Ho

Nonradiative energy dissipation in electronically excited polyatomic molecules proceeds through conical intersections, loci of degeneracy between electronic states. We observe a marked enhancement of laser-induced double ionization in the…

With a classical ensemble model that including electron correlations during the whole ionization process, we investigated strong-field sequential double ionization of Ar by elliptically polarized pulses at the quantitative level. The…

Atomic Physics · Physics 2015-06-04 Yueming Zhou , Cheng Huang , Qing Liao , Peixiang Lu

We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…

Atomic Physics · Physics 2015-05-14 Michael Spanner , Serguei Patchkovskii

We report on tunnel ionization of Xe by 2-cycle, intense, infrared laser pulses and its dependence on carrier-envelope-phase (CEP). At low values of optical field ($E$), the ionization yield is maximum for cos-like pulses with the…

We study double ionization in a one-dimensional model of a three-electron atom exposed to strong short laser fields. The corresponding ab initio simulations reveal a characteristic ``knee'' in the ionization yield at lower field intensities…

Atomic Physics · Physics 2025-06-30 Dmitry Efimov

We examine the nature and statistical properties of electron-electron collisions in the recollision process in a strong laser field. The separation of the double ionization yield into sequential and nonsequential components leads to a…

Atomic Physics · Physics 2015-05-14 Francois Mauger , Cristel Chandre , Turgay Uzer

The pump-probe experiments enabled by X-ray free-electron lasers (XFEL) will allow us to directly observe correlated electronic motion with attosecond time resolution by detecting photoelectron pairs in coincidence. In helium, the…

Optical frequency metrology in atoms and ions can probe hypothetical fifth-forces between electrons and neutrons by sensing minute perturbations of the electronic wave function induced by them. A generalized King plot has been proposed to…

We consider the final stage of triple ionization of atoms in a strong linearly polarized laser field. We propose that for intensities below the saturation value for triple ionization the process is dominated by the simultaneous escape of…

Quantum Physics · Physics 2009-11-07 Krzysztof Sacha , Bruno Eckhardt

We present new experimental and theoretical cross sections for electron-impact single ionization of Xe$^{12+}$ and Xe$^{13+}$ ions, and double ionization of Xe$^{12+}$, Xe$^{13+}$ and Xe$^{14+}$ ions for collision energies from the…

Here, we identify a new mechanism where the early stage of electron ionization in the field of strong femtosecond laser pulse determines the final yield of non-sequential double ionization. By using simple trajectory methods we prove that…

Quantum Physics · Physics 2025-02-07 Ivan P. Christov

Ionization of an atom or molecule presents surprising richness beyond our current understanding: strong-field ionization with low-frequency fields recently revealed unexpected kinetic energy structures (1, 2). A solid grasp on electron…

The present work explores quantitative limits to the Single-Active Electron (SAE) approximation, often used to deal with strong-field ionization and subsequent attosecond dynamics. Using a time-dependent multi\-configuration approach,…

Atomic Physics · Physics 2025-11-04 Jean-Nicolas Vigneau , Tung Nguyen-Dang , Eric Charron , Osman Atabek

As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

Atomic Physics · Physics 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

Femtosecond high-order harmonic transient absorption spectroscopy is used to resolve the complete |j,m> quantum state distribution of Xe+ produced by optical strong-field ionization of Xe atoms at 800nm. Probing at the Xe N_4/5 edge yields…

In Xe+Sn central collisions from 12 to 20 MeV/A measured with the INDRA 4$\pi$ multidetector, the three-fragment exit channel occurs with a significant cross section. In this contribution, we show that these fragments arise from two…

Nuclear Experiment · Physics 2013-12-17 Diego Gruyer , J. D. Frankland , E. Bonnet , M. Boisjoli , A. Chbihi , L. Manduci , P. Marini , K. Mazurek , P. N. Nadtochy

The uncorrelated (``sequential'') and correlated (``nonsequential'') double ionization of the H2 molecule in strong laser pulses is investigated using the tools of nonlinear dynamics. We focus on the phase-space dynamics of this system,…

Chaotic Dynamics · Physics 2009-11-30 François Mauger , Cristel Chandre , T. Uzer