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We investigate high-order harmonic generation in ZnO driven by linearly polarized multi-color pulses. It is shown that the intensities of the harmonics in the plateau region can be enhanced by two to three orders of magnitude when driven by…

Computational Physics · Physics 2020-03-25 Xiaohong Song , Shidong Yang , Ruixin Zuo , Torsten Meier , Weifeng Yang

We extend the semi-classical trajectory description for the high-order harmonic generation~(HHG) from solids by integrating the effect of electron-scattering. Comparing the extended semi-classical trajectory model with a one-dimensional…

For decades, most research on high harmonic generation (HHG) considered matter as quantum but light as classical, leaving the quantum-optical nature of the harmonics an open question. Here we explore the quantum properties of high…

Quantum Physics · Physics 2023-11-21 Matan Even Tzur , Michael Birk , Alexey Gorlach , Ido Kaminer , Michael Krueger , Oren Cohen

We consider optical high harmonic generation in a hydrogen atom confined in a breathing spherical box by considering atomic nucleus as fixed at the center of sphere. In such spherically symmetric, dynamical trap, the high harmonic…

Quantum Physics · Physics 2019-02-19 S. Rakhmanov , D. Matrasulov , B. Eshchanov , V. I. Matveev

A calculation of the high-harmonic generation (HHG) in $\alpha$-quartz using the time-dependent density functional theory is reported. The inter-band process is attributed to the dominant in HHG above the band gap. The photon energy is set…

Optics · Physics 2017-01-04 T. Otobe

The irradiation of atoms by a strong IR laser field of frequency $\omega$ results in the emission of odd-harmonics of $\omega$ ("IR harmonics") up to some maximal cut-off frequency. The addition of an XUV field of frequency…

Atomic Physics · Physics 2008-02-04 Avner Fleischer , Nimrod Moiseyev

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

High-order harmonic generation (HHG) provides a broad spectral bandwidth for synthesizing attosecond pulses. However, in the current HHG schemes, only part of the harmonics can be phase-locked, which limits the ability to achieve shorter…

Optics · Physics 2024-06-18 ShiJun Wang , XuanYang Lai , XiaoJun Liu

We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

We study nonlinear optical response of Landau quantized graphene to an intense electromagnetic wave. In particular, we consider high harmonic generation process. It is shown that one can achieve efficient generation of high harmonics with…

Mesoscale and Nanoscale Physics · Physics 2017-05-24 H. K. Avetissian , A. G. Ghazaryan , G. F. Mkrtchian , Kh. V. Sedrakian

We present a model for quasi-phase matching (QPM) in high-order harmonic generation (HHG). Using a one-dimensional description, we analyze the time-dependent, ultrafast wave-vector balance to calculate the on-axis harmonic output versus…

High-order harmonic generation (HHG), a robust tabletop source for producing attosecond pulses, has been extensively utilized in attosecond metrology. Traditionally, HHG driven by classical laser fields involves two typical quantum paths…

High-harmonic generation (HHG) of a two-level-system driven by an intense monochromatic phase-locked laser is studied in terms of complex spectral analysis with the Floquet method. In contrast to the phenomenological approaches, this…

Quantum Physics · Physics 2021-02-03 Hidemasa Yamane , Ken-ichi Noba , Tomio Petrosky , Satoshi Tanaka

We consider the process of high-order harmonics generation (HHG) in the xenon atom enhanced by the inter-shell correlation between the valence 5p and inner 4d shells. We derive the HHG spectrum from a numerical solution of the one-electron…

Atomic Physics · Physics 2019-07-17 Alexander W. Bray , David Freeman , Sebastian Eckart , Anatoli S. Kheifets

We show that high-order harmonics generated from molecules by intense laser pulses can be expressed as the product of a returning electron wave packet and the photo-recombination cross section (PRCS) where the electron wave packet can be…

Atomic Physics · Physics 2008-04-04 Anh-Thu Le , R. Della Picca , P. D. Fainstein , D. A. Telnov , M. Lein , C. D. Lin

The sub-cycle dynamics of electrons driven by strong laser fields is central to the emerging field of attosecond science. We demonstrate how the dynamics can be probed through high-order harmonic generation, where different trajectories…

We study the phase matching of resonant high-harmonic generation (HHG) and high-order frequency mixing (HFM) in plasma. We solve numerically the propagation equations coupled with the time-dependent Schr\"odinger equation for the nonlinear…

Optics · Physics 2024-04-30 Vasily V. Strelkov , Margarita A. Khokhlova

Various interference effects are known to exist in the process of high harmonic generation (HHG) both at the single atom and macroscopic levels. In particular, the quantum path difference between the long and short trajectories of electron…

An accurate analytic model describing high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results…

Time- and angle-resolved photoemission spectroscopy has played an important role in revealing the non-equilibrium electronic structures of solid-state materials. The implementation of high harmonic generation to obtain a higher photon…

Strongly Correlated Electrons · Physics 2022-06-29 Takeshi Suzuki , Shik Shin , Kozo Okazaki