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We present a new kind of basis function for discretizing the Schr\"odinger equation in electronic structure calculations, called a gausslet, which has wavelet-like features but is composed of a sum of Gaussians. Gausslets are placed on a…

Chemical Physics · Physics 2018-01-17 Steven R. White

Free-particle Green's function plays a central role in the theoretical description of electron scattering and autoionization processes in quantum physics and chemistry. Recently, Gaussian basis set approaches have become increasingly…

Chemical Physics · Physics 2026-05-19 Dibyendu Mahato , Wojciech Skomorowski

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

With the aim of describing bound and continuum states for diatomic molecules, we develop and implement a spectral method that makes use of Generalized Sturmian Functions (GSF) in prolate spheroidal coordinates. In order to master all…

Atomic and Molecular Clusters · Physics 2021-06-02 D. M. Mitnik , F. A. Lopez , L. U. Ancarani

The search for gamma-ray counterparts to gravitational-wave events with the CALET Gamma-ray Burst Monitor (CGBM) requires accurate and robust background modeling. Previous CALET observing runs (O3 and O4) relied on averaged pre/post-event…

High Energy Astrophysical Phenomena · Physics 2025-11-20 Bisweswar Sen

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

Optical coherence encodes information about the correlations of the electromagnetic field. In combination with quantum optical approaches, it allows for the study of the correlations between photons. Since the pioneering papers of Glauber,…

Quantum Physics · Physics 2025-04-21 Philipp Stammer , Javier Rivera-Dean , Maciej Lewenstein

We investigate the high harmonic generation (HHG) from solids by simulating the dynamics of a single active electron in periodic potentials. The corresponding time-dependent Schr\"odinger equations (TDSE) are solved numerically by using…

Atomic Physics · Physics 2016-03-31 Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

In this work we construct Gaussian beam approximations to solutions of the high frequency Helmholtz equation with a localized source. Under the assumption of non-trapping rays we show error estimates between the exact outgoing solution and…

Numerical Analysis · Mathematics 2013-04-05 Hailiang Liu , James Ralston , Olof Runborg , Nicolay M. Tanushev

Closed-form expressions for all matrix elements required for variational calculation of the electronic structure of periodic solids have been derived using a basis of explicitly correlated Gaussians (ECGs). Periodic basis functions are…

Quantum Physics · Physics 2026-05-14 Kalman Varga

We analyze Gaussian analytic functions (GAFs) defined as power series with coefficients modeled by discrete stationary Gaussian processes, utilizing their spectral measures. We revisit some limit theorems for random analytic functions and…

Probability · Mathematics 2025-01-08 Tomoyuki Shirai

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…

Atomic Physics · Physics 2010-04-21 C. B. Madsen , M. Abu-samha , L. B. Madsen

Gaussian processes are popular and flexible models for spatial, temporal, and functional data, but they are computationally infeasible for large datasets. We discuss Gaussian-process approximations that use basis functions at multiple…

Methodology · Statistics 2020-12-22 Matthias Katzfuss , Wenlong Gong

We consider three distinct methods to compute the mass spectrum of gauge theories in the Hamiltonian formalism: (1) correlation-function scheme, (2) one-point-function scheme, and (3) dispersion-relation scheme. The first one examines…

High Energy Physics - Lattice · Physics 2023-11-02 Etsuko Itou , Akira Matsumoto , Yuya Tanizaki

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Xiao Zhang , Tao Zhu , Hongchuan Du , Hong-Gang Luo , Jeroen van den Brink , Rajyavardhan Ray

Credible forecasting and representation learning of dynamical systems are of ever-increasing importance for reliable decision-making. To that end, we propose a family of Gaussian processes (GP) for dynamical systems with linear…

Machine Learning · Computer Science 2025-02-11 Petar Bevanda , Max Beier , Armin Lederer , Alexandre Capone , Stefan Sosnowski , Sandra Hirche

We present a new adaptive method for electronic structure calculations based on novel fast algorithms for reduction of multivariate mixtures. In our calculations, spatial orbitals are maintained as Gaussian mixtures whose terms are selected…

Numerical Analysis · Mathematics 2019-06-19 Gregory Beylkin , Lucas Monzon , Xinshuo Yang

High-order harmonic generation (HHG) enables the up-conversion of intense infrared or visible femtosecond laser pulses into extreme-ultraviolet attosecond pulses. However, the highly nonlinear nature of the process results in low conversion…

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