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We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

The atomic response to an ultra-intense driving field produces a characteristic high-harmonic spectrum featuring a rapid drop in intensity for the lower harmonics, followed by a plateau and a sharp cutoff. This response vanishes for…

Quantum Physics · Physics 2026-01-06 Lidija Petrovic , Philipp Stammer , Maciej Lewenstein , Javier Rivera-Dean

We introduce two-color counterrotating circularly polarized laser fields as a new way to spectrally control high harmonic generation (HHG) from relativistic plasma mirrors. Through particle-in-cell simulations, we show that only a selected…

Plasma Physics · Physics 2018-04-13 Zi-Yu Chen

The first scheme for quasi-phase-matching high harmonic generation of circularly polarized radiation is proposed: optical rotation quasi-phase-matching (ORQPM). In ORQPM propagation of the driving radiation in a system exhibiting circular…

Optics · Physics 2013-03-19 Lewis Z. Liu , Kevin O'Keeffe , Simon M. Hooker

High-order harmonic generation with bicircular fields - the combination of counter-rotating circularly polarized pulses at different frequencies - results in a series of short-wavelength XUV harmonics with alternating circular…

Quantum Physics · Physics 2019-07-25 Emilio Pisanty , Álvaro Jiménez-Galán

We investigate high-order harmonic spectra from aligned diatomic molecules in intense driving fields whose components have orthogonal polarizations. We focus on how the driving-field ellipticity influences structural interference patterns…

Attosecond metrology sensitive to sub-optical-cycle electronic and structural dynamics is opening up new avenues for ultrafast spectroscopy of condensed matter. Using intense lightwaves to precisely control the extremely fast carrier…

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…

Using numerical simulations, we show that atomic high order harmonic generation, HHG, with a circularly polarized laser field offers an ideal framework for quantum-classical correspondence in strong field physics. With an appropriate…

Atomic Physics · Physics 2014-02-06 Francois Mauger , A. D. Bandrauk , Adam Kamor , Turgay Uzer , Cristel Chandre

Generation of circularly-polarized high-harmonics with the same helicity to all orders is indispensable for chiral-sensitive spectroscopy with attosecond temporal resolution. Solid-state samples have added a valuable asset in controlling…

Optics · Physics 2023-06-06 Navdeep Rana , M. S. Mrudul , Gopal Dixit

We observe the generation of high harmonics in the plane perpendicular to the driving laser polarization and show that these are driven by the spin-orbit interaction. Using R-Matrix with time-dependence theory, we demonstrate that for…

High-harmonic generation (HHG) is a nonlinear process in which a strong driving field interacts with a material, resulting in the frequency up-conversion of the driver into its high-order harmonics. This process is highly sensitive to the…

Quantum Physics · Physics 2025-07-04 J. Rivera-Dean , P. Stammer , M. F. Ciappina , M. Lewenstein

We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center interference condition for elliptically polarized fields,…

Atomic Physics · Physics 2015-06-16 T. Das , B. B. Augstein , C. Figueira de Morisson Faria

When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a "relativistic oscillating window". The diffracted…

Plasma Physics · Physics 2021-04-07 Longqing Yi

The bi-circular scheme for high harmonic generation, which combines two counter-rotating circular fields with frequency ratio 2:1, has recently permitted to generate high harmonics with essentially circular polarization, opening the way for…

We investigate the high harmonic generation (HHG) in solids driven by laser fields with different ellipticities. The HHG spectra show a two-plateau structure within the energy gap between the valence band and the first conduction band.…

Optics · Physics 2018-06-01 Liang Li , Pengfei Lan , Xiaosong Zhu , Tengfei Huang , Peixiang Lu

The use of bichromatic counter-rotating laser field is known to generate high-order harmonics with non-zero ellipticity. By combining such laser field with a plasmonic-enhanced spatially inhomogeneous field, we propose a way to influence…

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

We investigate the polarization properties of high harmonic generation from polar molecules with a linearly polarized field. It is found that elliptically polarized harmonics are observed in a wide spectral range from the plateau to the…

Optics · Physics 2011-12-06 Meiyan Qin , Xiaosong Zhu , Qingbin Zhang , Weiyi Hong , Peixiang Lu

We investigate the spatial characteristics of high-order harmonic radiation generated in argon, and observe cross-like patterns in the far field. An analytical model describing harmonics from an astigmatic driving beam reveals that these…

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