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The influence of a chemically or electrically heterogeneous distribution of interaction sites at a planar substrate on the number density of an adjacent fluid is studied by means of classical density functional theory (DFT). In the case of…

Soft Condensed Matter · Physics 2018-05-25 Maximilian Mußotter , Markus Bier , S. Dietrich

We study the temporal response of the electric current in an electrolyte under a sudden switch on or switch off of an external electric field of arbitrary magnitude. We use Stochastic Density Functional Theory including hydrodynamic…

Statistical Mechanics · Physics 2023-08-02 Haggai Bonneau , Vincent Démery , Élie Raphaël

By using the generalized version of the Shell Theorem analytical equations are derived to calculate the electric energy of a charged sphere and the field energy of the electrolyte inside and around the sphere. These electric energies are…

Soft Condensed Matter · Physics 2021-01-21 Istvan P. Sugar

A variational theory is developed to study electrolyte solutions, composed of interacting point-like ions in a solvent, in the presence of dielectric discontinuities and charges at the boundaries. Three important and non-linear…

Soft Condensed Matter · Physics 2013-05-29 Sahin Buyukdagli , Manoel Manghi , John Palmeri

The interaction of an electron with a local static charge distribution (e.g., an atom or molecule) is dominated at large distances by the radial 1/r Coulomb potential. The second order effect comes from the non-central electric dipole…

Quantum Physics · Physics 2023-02-08 A. D. Alhaidari , H. Bahlouli

The present paper is devoted to the study of a simple model of interacting electrons in a random background. In a large interval $\Lambda$, we consider $n$ one dimensional particles whose evolution is driven by the Luttinger-Sy model, i.e.,…

Mathematical Physics · Physics 2014-08-26 Frédéric Klopp , Nikolaj Veniaminov

Influences of nonlinear screening on effective interactions between spherical macroions in charged colloids are described via response theory. Nonlinear screening, in addition to generating effective many-body interactions, is shown to…

Soft Condensed Matter · Physics 2007-05-23 A. R. Denton

Transfer-ionization in fast collisions between a bare ion and an atom, in which one of the atomic electrons is captured by the ion whereas another one is emitted, crucially depends on dynamic electron-electron correlations. We show that in…

Atomic Physics · Physics 2013-05-15 A. B. Voitkiv

The interaction force between likely charged particles/surfaces is usually repulsive due to the Coulomb interaction. However, the counterintuitive like-charge attraction in electrolytes has been frequently observed in experiments, which has…

Soft Condensed Matter · Physics 2016-11-08 Pei Liu , Manman Ma , Zhenli Xu

A new method to determine electron correlation energy is described. This method is based on a better representation of the potential due to interacting electrons that is obtained by specifying both the average and standard deviation. The…

Materials Science · Physics 2007-05-23 T. R. S. Prasanna

We study the semiclassical dynamics of interacting electrons in a biased crystal lattice. A complex dynamical scenario emerges from the interplay between the Coulomb and the external electric fields. When the electrons are far apart, the…

Strongly Correlated Electrons · Physics 2013-06-27 Christopher Gaul , Antonio Rodríguez , Rodrigo P. A. Lima , Francisco Domínguez-Adame

The starting point is the problem of finding the interaction energy of two coinciding homogeneous cubic charge distributions. The brute force method of subdividing the cube into $N^3$ sub-cubes and doing the sums results in slow convergence…

Atomic and Molecular Clusters · Physics 2007-05-23 Hanno Essen

Understanding the response of the surface of metallic solids to external electric field sources is crucial to characterize electrode-electrolyte interfaces. Continuum electrostatics offer a simple description of the induced charge density…

Chemical Physics · Physics 2021-12-14 Giovanni Pireddu , Laura Scalfi , Benjamin Rotenberg

A nonlinear response theory is developed and applied to electrostatic interactions between spherical macroions, screened by surrounding microions, in charge-stabilized colloidal suspensions. The theory describes leading-order nonlinear…

Soft Condensed Matter · Physics 2009-11-10 A. R. Denton

The effective electron-electron interaction in the electron gas depends on both the density and spin local field factors. Variational Diagrammatic Quantum Monte Carlo calculations of the spin local field factor are reported and used to…

Quantum Gases · Physics 2021-01-27 Carl A. Kukkonen , Kun Chen

Polymer electrolytes typically exhibit diminished ionic conductivity due to the presence of correlation effects between the cations and anions. Microscopically, transient ionic aggregates, e.g. {\it ion-pairs}, {\it ion-triplets} or higher…

Materials Science · Physics 2008-04-15 Arijit Maitra , Andreas Heuer

We derive formulae for the electrostatic interaction between two long, rigid macromolecules that may have arbitrary surface charge patterns and cross at an arbitrary interaxial angle. We calculate the dependence of the interaction energy on…

Soft Condensed Matter · Physics 2009-10-31 A. A. Kornyshev , S. Leikin

We study charge regulation of colloidal particles inside aqueous electrolyte solutions. To stabilize colloidal suspension against precipitation, colloidal particles are synthesized with either acidic or basic groups on their surface. In…

Soft Condensed Matter · Physics 2020-09-16 Amin Bakhshandeh , Derek Frydel , Yan Levin

Progress in electrochemical applications of ionic liquids builds on an understanding of electrical double-layer. This computational study focuses on structure-determined quantities -- maximum packing density, potentials and capacitances --…

Interfering electrons in a mesoscopic ring are irradiated with both classical and nonclassical microwaves. The average intensity of the charges is calculated as a function of time and it is found that it depends on the nature of the…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 D. I. Tsomokos , C. C. Chong , A. Vourdas
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