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Rydberg excited states of molecules pose a challenge for electronic structure calculations because of their highly diffuse electron distribution. Even large and elaborate atomic basis sets tend to underrepresent the long-range tail, overly…

We propose a novel type of Rydberg dimer, consisting of a Rydberg-state atom bound to a distant positive ion. The molecule is formed through long-range electric-multipole interaction between the Rydberg atom and the point-like ion. We…

Atomic Physics · Physics 2021-05-14 A. Duspayev , X. Han , M. A. Viray , L. Ma , J. Zhao , G. Raithel

Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…

Rydberg atoms represent a platform underpinning many recent developments in quantum computation, simulation, sensing, and metrology. They further facilitate optical nonlinearity at the single-photon level when coupled to photons propagating…

The interaction between atoms and a quantized radiation field is fundamentally important in quantum optics and quantum information science. Due to their unusual properties, Rydberg atoms are promising building blocks for two-qubit gates and…

Quantum Physics · Physics 2026-01-06 Francisco D. Santillan , Andreas Hanke

Ion-atom interactions are a comparatively recent field of research that has drawn considerable attention due to its applications in areas including quantum chemistry and quantum simulations. In first experiments, atomic ions and neutral…

Atomic Physics · Physics 2021-07-12 Leon Karpa

Theory of long-range interactions between an atom in its ground S state and a linear molecule in a degenerate state with a non-zero projection of the electronic orbital angular momentum is presented. It is shown how the long-range…

Chemical Physics · Physics 2015-05-20 Wojciech Skomorowski , Robert Moszynski

Great advances in precision quantum measurement have been achieved with trapped ions and atomic gases at the lowest possible temperatures. These successes have inspired ideas to merge the two systems. In this way one can study the unique…

Quantum Physics · Physics 2023-03-21 T. Feldker , H. Fürst , H. Hirzler , N. V. Ewald , M. Mazzanti , D. Wiater , M. Tomza , R. Gerritsma

A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A…

Atomic Physics · Physics 2008-07-15 Ivan C. H. Liu , Jovica Stanojevic , Jan M. Rost

Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from…

We introduce a novel method to engineer sharply peaked, distance-selective interactions between neutral atoms by exploiting interaction-induced resonances within a resonantly driven Rydberg ladder system. By tuning laser parameters, a…

Atomic Physics · Physics 2025-07-24 Mohammadsadegh Khazali

Quantum entanglement is crucial for simulating and understanding exotic physics of strongly correlated many-body systems, such as high--temperature superconductors, or fractional quantum Hall states. The entanglement of non-identical…

Quantum Physics · Physics 2017-10-25 Y. Zeng , P. Xu , X. D. He , Y. Y. Liu , M. Liu , J. Wang , D. J. Papoular , G. V. Shlyapnikov , M. S. Zhan

Realizing systems that support robust, controlled interactions between individual photons is an exciting frontier of nonlinear optics. To this end, one approach that has emerged recently is to leverage atomic interactions to create strong…

Quantum Physics · Physics 2016-08-11 James S. Douglas , Tommaso Caneva , Darrick E. Chang

Quantum simulation - the use of one quantum system to simulate a less controllable one - may provide an understanding of the many quantum systems which cannot be modeled using classical computers. Impressive progress on control and…

We show that the interaction between Rydberg atomic states can provide continuous spin squeezing of atoms with two ground states. The interaction prevents the simultaneous excitation of more than a single atom in the sample to the Rydberg…

Quantum Physics · Physics 2007-05-23 Isabelle Bouchoule , Klaus Moelmer

Trapped ions driven by electromagnetic radiation constitute one of the most developed quantum technologies to date. The scenarios range from proof-of-principle experiments to on-chip integration for quantum information units. In most cases,…

Quantum Physics · Physics 2023-09-26 T. Tassis , F. L. Semião

Interfacing light and matter at the quantum level is at the heart of modern atomic and optical physics and enables new quantum technologies involving the manipulation of single photons and atoms. A prototypical atom-light interface is…

Neutral atoms excited to Rydberg states can interact with each other via dipole-dipole interaction, which results in a physical phenomenon named Rydberg blockade mechanism. The effect attracts much attention due to its potential…

Quantum Physics · Physics 2015-06-12 Huaizhi Wu , Zhen-Biao Yang , Li-Tuo Shen , Shi-Biao Zheng

In a recent experiment, Barreiro et al. demonstrated the fundamental building blocks of an open-system quantum simulator with trapped ions [Nature 470, 486 (2011)]. Using up to five ions, single- and multi-qubit entangling gate operations…

Quantum Physics · Physics 2015-05-27 M. Mueller , K. Hammerer , Y. L. Zhou , C. F. Roos , P. Zoller

An atom chip has been fabricated for the study of interactions between $^{87}$Rb Rydberg atoms and a Au surface. The chip tightly confines cold atoms by generating high magnetic field gradients using microfabricated current-carrying wires.…

Atomic Physics · Physics 2025-10-15 O. Cherry , J. D. Carter , J. D. D. Martin