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Solid-solutions of the "soft" quantum spin ice pyrochlore magnets Tb2B2O7 with B=Ti and Sn display a novel magnetic ground state in the presence of strong B-site disorder, characterized by a low susceptibility and strong spin fluctuations…

We have investigated the magnetic ground-state of the multiferroic relaxor ferroelectric \pfn with $\mu$SR spectroscopy and neutron scattering. We find that a transition to a partially disordered phase occurs below T=20 K that coexists with…

Materials Science · Physics 2009-09-13 G. -M. Rotaru , B. Roessli , A. Amato , S. N. Gvasaliya , C. Mudry , S. G. Lushnikov , T. A. Shaplygina

Motivated by recent experimental and theoretical progress on the Er2Ti2O7 pyrochlore XY antiferromagnet, we study the problem of quantum order-by-disorder in pyrochlore XY systems. We consider the most general nearest-neighbor pseudo…

Strongly Correlated Electrons · Physics 2013-11-15 Anson W. C. Wong , Zhihao Hao , Michel J. P. Gingras

The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based…

Strongly Correlated Electrons · Physics 2025-09-10 A. Brassington , Q. Ma , G. Duan , S. Calder , A. I. Kolesnikov , K. M. Taddei , G. Sala , E. S. Choi , H. Wang , W. Xie , B. A. Frandsen , N. Li , X. F. Sun , C. Liu , R. Yu , H. D. Zhou , A. A. Aczel

Over the past two decades, the magnetic ground states of all rare earth titanate pyrochlores have been extensively studied, with the exception of Sm$_2$Ti$_2$O$_7$. This is, in large part, due to the very high absorption cross-section of…

Some frustrated pyrochlore antiferromagnets, such as Y2Mo2O7, show a spin-freezing transition and magnetic irreversibilities below a temperature Tf similar to what is observed nonlinear magnetization measurements on Y2Mo2O7 that provide…

Disordered Systems and Neural Networks · Physics 2009-10-28 M. J. P. Gingras , C. V. Stager , N. P. Raju , B. D. Gaulin , J. E. Greedan

A comprehensive set of muon spin spectroscopy and neutron scattering measurements supported by ab-initio and model Hamiltonian simulations have been used to investigate the magnetic ground state of Na$_2$PrO$_3$. $\mu$SR reveals N\'eel…

Neutron diffraction and nuclear quadrupole resonance (NQR) measurements were employed to investigate magnetic order in the non-ferroelectric phase preceding the low-temperature multiferroic state in FeTe2O5Br. Refnement of the neutron…

Strongly Correlated Electrons · Physics 2013-04-10 M. Pregelj , P. Jeglič , A. Zorko , O. Zaharko , T. Apih , A. Gradišek , M. Komelj , H. Berger , D. Arčon

We report an analysis of neutron diffraction from single crystals of the spin-liquid pyrochlore Tb2Ti2O7 under the application of magnetic fields along the crystallographic $[110]$ direction. Such a perturbation has been shown to destroy…

Strongly Correlated Electrons · Physics 2009-11-17 J. P. C. Ruff , B. D. Gaulin , K. C. Rule , J. S. Gardner

The pyrochlore insulator Yb2Ti2O7 has attracted the attention of experimentalists and theoreticians alike for about 15 years. Conflicting neutron diffraction data on the possible existence of magnetic Bragg reflections at low temperature…

Strongly Correlated Electrons · Physics 2016-08-26 A. Yaouanc , P. Dalmas de Reotier , L. Keller , B. Roessli , A. Forget

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

Elastic and inelastic neutron scattering measurements have been carried out to investigate the magnetic properties of superconducting (Tc~8K) HoNi2B2C. The inelastic measurements reveal that the lowest two crystal field transitions out of…

supr-con · Physics 2012-08-27 T. E. Grigereit , J. W. Lynn , R. J. Cava , J. J. Krajewski , W. F. Peck,

We report extensive measurements on a new compound (Yb0.24Sn0.76)Ru that crystallizes in the cubic CsCl structure. Valence band photoemission and L3 x-ray absorption show no divalent component in the 4f configuration of Yb. Inelastic…

The XY pyrochlore Yb$_2$Ti$_2$O$_7$, with pseudo spin 1/2 at the Yb$^{3+}$ site, has been celebrated as potential host for the quantum spin ice state. The substitution of non-magnetic Ti with Pt gives Yb$_2$Pt$_2$O$_7$, a system with…

Strongly Correlated Electrons · Physics 2018-10-03 S. K. Takahashi , A. Arsenault , C. Mauws , A. M. Hallas , C. Sarkis , K. A. Ross , C. R. Wiebe , M. Tachibana , G. M. Luke , T. Imai

We report on the crystal field level splitting and magnetic ground state of the Jeff = 1/2 square lattice antiferromagnets YbBi2ClO4 and YbBi2IO4 using powder inelastic neutron scattering (INS) and neutron diffraction measurements. Both…

Strongly Correlated Electrons · Physics 2025-03-25 Pyeongjae Park , Qianli Ma , G. Sala , S. Calder , Douglas L. Abernathy , Matthew B. Stone , Andrew F. May , Andrew D. Christianson

We present an experimental and theoretical study of the anisotropic pyrochlore phase diagram. Inelastic field-dependent neutron scattering on Yb$_2$Ti$_2$O$_7$ shows intrinsic broadening and a flat low-energy magnon mode which is partially…

Strongly Correlated Electrons · Physics 2025-11-20 Shang-Shun Zhang , Anish Bhardwaj , S. M. Koohpayeh , D. M. Pajerowski , Jeffrey G. Rau , Hitesh J. Changlani , Allen Scheie

The magnetic ground state of two isostructural coordination polymers (i) the quasi two-dimensional S = 1/2 square-lattice antiferromagnet [Cu(HF$_{2}$)(pyrazine)$_{2}$]SbF$_{6}$; and (ii) a new compound…

We investigated the nature of the spin glass-like phase transition in the geometrically frustrated pyrochlore lattices Y$_{2}$Mo$_{2}$O$_{7}$ using the local probes nuclear and muon magnetic resonances, and the field-dependent long range…

Strongly Correlated Electrons · Physics 2010-09-24 Oren Ofer , Amit Keren , Jason S. Gardner , Yang Ren , W. A. MacFarlane

We report muon spin relaxation and inelastic neutron measurements on the Heusler system YbPd$_2$Sn. Localised anisotropic and quasi-elastic Yb magnetic fluctuations are observed below $T = 150$K. Both $\mu$SR and neutron data indicate a…

Strongly Correlated Electrons · Physics 2009-11-07 A. Amato , B. Roessli , P. Fischer , N. Bernhoeft , A. Stunault , C. Baines , A. Dönni , H. Sugawara