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We propose and analyze a mechanism for inducing spin Hall currents in ordinary (1H phase) monolayer transition metal dichalcogenides (TMDs) due to the nonlinear process of optical rectification. The photo-induced spin current is…

Mesoscale and Nanoscale Physics · Physics 2018-12-07 Alireza Taghizadeh , T. G. Pedersen

We present time-resolved Kerr rotation measurements, showing spin lifetimes of over 100 ns at room temperature in monolayer MoSe$_2$. These long lifetimes are accompanied by an intriguing temperature dependence of the Kerr amplitude, which…

The presence of two spin-split valleys in monolayer (1L) transition metal dichalcogenide (TMD) semiconductors supports versatile exciton species classified by their spin and valley quantum numbers. While the spin-0 intravalley exciton,…

Mesoscale and Nanoscale Physics · Physics 2020-07-22 Yueh-Chun Wu , Sarath Samudrala , Andrew McClung , Takashi Taniguchi , Kenji Watanabe , Amir Arbabi , Jun Yan

Transition metal dichalcogenide (TMD) monolayers are interesting materials in part because of their strong spin-orbit coupling. This leads to intrinsic spin-splitting of opposite signs in opposite valleys, so the valleys are intrinsically…

Mesoscale and Nanoscale Physics · Physics 2018-11-21 Dibya Kanti Mukherjee , Arijit Kundu , H. A. Fertig

We investigated the valley depolarization and carrier relaxation process of monolayer and bilayer WS2 at 10 K by using time-resolved Kerr rotation (TRKR) and differential reflectance measurement simultaneously. Two decay processes extracted…

Mesoscale and Nanoscale Physics · Physics 2018-03-28 Huimin Su , Aiying Deng , Zhiheng Zhen , Jun-Feng Dai

Chiral light-matter interactions can enable polarization to control the direction of light emission in a photonic device. Most realizations of chiral light-matter interactions require external magnetic fields to break time-reversal symmetry…

Optics · Physics 2019-07-19 Zhili Yang , Shahriar Aghaeimeibodi , Edo Waks

Achieving robust and electrically controlled valley polarization in monolayer transition metal dichalcogenides (ML-TMDs) is a frontier challenge for realistic valleytronic applications. Theoretical investigations show that integration of 2D…

Monolayer transition metal dichalcogenide (TMDC) crystals, as direct-gap materials with unusually strong light-matter interaction, have attracted much recent attention. In contrast to the initial understanding, the minima of the conduction…

Monolayer transition metal dichalcogenides are promising materials for valleytronic operations. They exhibit two inequivalent valleys in the Brillouin zone, and the valley populations can be directly controlled and determined using…

Mesoscale and Nanoscale Physics · Physics 2017-09-29 Kathleen M. McCreary , Marc Currie , Aubrey T. Hanbicki , Hsun-Jen Chuang , Berend T. Jonker

Monolayer transition metal dichalcogenides (TMDs) have been in focus of current research, among others due to their remarkable exciton landscape consisting of bright and dark excitonic states. Although dark excitons are not directly visible…

Materials Science · Physics 2020-12-21 Maja Feierabend , Samuel Brem , August Ekman , Ermin Malic

Monolayer transition metal dichalcogenides (TMDs) offer a novel two-dimensional platform for semiconductor devices. One such application, whereby the added low dimensional crystal physics (i.e. optical spin selection rules) may prove TMDs a…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Matthew Brooks , Guido Burkard

Monolayer transition metal dichalcogenides, known for exhibiting strong excitonic resonances, constitute a very interesting and versatile platform for investigation of light-matter interactions. In this work we report on a strong coupling…

Mesoscale and Nanoscale Physics · Physics 2019-05-20 M. Król , K. Lekenta , R. Mirek , K. Łempicka , D. Stephan , K. Nogajewski , M. R. Molas , A. Babiński , M. Potemski , J. Szczytko , B. Piętka

Strong coupling between the electronic states of monolayer transition metal dichalcogenides (TMDC) such as MoS$_2$, MoSe$_2$, WS$_2$, or WSe$_2$, and a two-dimensional (2D) photonic cavity gives rise to several exotic effects. The Dirac…

Mesoscale and Nanoscale Physics · Physics 2017-08-02 Amrit De , Roger Lake

Spin-forbidden intravalley dark exciton in tungsten-based transition metal dichalcogenides (TMDCs), owing to its unique spin texture and long lifetime, has attracted intense research interest. Here, we show that we can control the dark…

We study van der Waals heterostructures consisting of monolayer MoSe$_2$ and few-layer Cr$_2$Ge$_2$Te$_6$ fully encapsulated in hexagonal Boron Nitride using low-temperature photoluminescence and polar magneto-optic Kerr effect…

Embedding a WS$_2$ monolayer in flakes of hexagonal boron nitride allowed us to resolve and study the photoluminescence response due to both singlet and triplet states of negatively charged excitons (trions) in this atomically thin…

Mesoscale and Nanoscale Physics · Physics 2018-06-08 D. Vaclavkova , J. Wyzula , K. Nogajewski , M. Bartos , A. O. Slobodeniuk , C. Faugeras , M. Potemski , M. R. Molas

Valley-selective optical selection rules and a spin-valley locking in transition-metal dichalcogenide (TMDC) monolayers are at the heart of "valleytronic physics", which exploits the valley degree of freedom and has been a major research…

Photo-induced charge separation in transition metal dichalcogenide heterobilayers is being explored for moir\'e excitons, spin-valley polarization, and quantum phases of excitons/electrons. While different momentum spaces may be critically…

Mesoscale and Nanoscale Physics · Physics 2020-05-27 Fang Liu , Qiuyang Li , Xiaoyang Zhu

Single-layer semiconducting transition-metal dichalcogenides, lacking point inversion symmetry, provide an efficient platform for valleytronics, where the electronic, magnetic, valley and lattice degrees of freedom can be selectively…

Mesoscale and Nanoscale Physics · Physics 2024-11-19 Emmanuele Cappelluti , Habib Rostami , Federico Cilento

We measured the lifetime of optically created valley polarization in single layer WS2 using transient absorption spectroscopy. The electron valley relaxation is very short (< 1ps). However the hole valley lifetime is at least two orders of…

Materials Science · Physics 2014-08-06 Cong Mai , Yuriy G. Semenov , Andrew Barrette , Yifei Yu , Zhenghe Jin , Linyou Cao , Ki Wook Kim , Kenan Gundogdu