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Recent advances in techniques for generating quantum light have stimulated research on novel spectroscopic measurements using quantum entangled photons. One such spectroscopy technique utilizes non-classical correlations among entangled…

Chemical Physics · Physics 2021-07-28 Yuta Fujihashi , Akihito Ishizaki

The increasing complexity of the recent photonic experiments challenges developing efficient multi-channel coincidence counting systems with high-level functionality. Here, we report a coincidence unit able to count detection events ranging…

Optics · Physics 2024-02-29 Josef Hloušek , Jan Grygar , Michal Dudka , Miroslav Ježek

Conventional nonlinear spectroscopy uses classical light to detect matter properties through the variation of its response with frequencies or time delays. Quantum light opens up new avenues for spectroscopy by utilizing parameters of the…

Quantum Physics · Physics 2017-02-01 Konstantin E. Dorfman , Frank Schlawin , Shaul Mukamel

Encoding information in the time-frequency domain is demonstrating its potential for quantum information processing. It offers a novel scheme for communications with large alphabets, computing with large quantum systems, and new approaches…

Quantum Physics · Physics 2019-12-02 Ilaria Gianani , Marco Sbroscia , Marco Barbieri

Photon coincidence spectroscopy is a promising technique for probing the nonlinear regime of cavity quantum electrodynamics in the optical domain, however its accuracy is mitigated by two factors: higher-order photon correlations, which…

Quantum Physics · Physics 2009-09-25 L. Horvath , B. C. Sanders

Recent theoretical studies in quantum spectroscopy have emphasized the potential of non-classical correlations in entangled photon pairs for selectively targeting specific nonlinear optical processes in nonlinear optical responses. However,…

Chemical Physics · Physics 2026-04-21 Yuta Fujihashi , Ozora Iso , Ryosuke Shimizu , Akihito Ishizaki

In the evaluation of novel scintillators, it is important to ensure that the spectrum of the light emitted by the scintillator is well matched to the response of the photomultiplier. In attempting to measure this spectrum using radioactive…

Instrumentation and Detectors · Physics 2008-11-26 J E McMillan , C J Martoff

We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of…

Quantum Physics · Physics 2018-09-12 Alex O. C. Davis , Valerian Thiel , Brian J. Smith

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

The development of single-photon counting detectors and arrays has made tremendous steps in recent years, not the least because of various new applications in, e.g., LIDAR devices. In this work, a 3D imaging device based on real thermal…

Time-frequency duality, which enables control of optical waveforms by manipulating amplitudes and phases of electromagnetic fields, plays a pivotal role in a wide range of modern optics. The conventional one-dimensional (1D) time-frequency…

Quantum Physics · Physics 2018-09-17 Rui-Bo Jin , Takuma Saito , Ryosuke Shimizu

The authors demonstrate a form of two-photon-counting interferometry by measuring the coincidence counts between single-photon-counting detectors at an output port of a Mach-Zehnder Interferometer (MZI) following injection of broad-band…

We demonstrate quantum interference of three photons that are distinguishable in time, by resolving them in the conjugate parameter, frequency. We show that the multiphoton interference pattern in our setup can be manipulated by tuning the…

Ultrafast imaging of photon statistics in two dimensions is a powerful tool for probing non-equilibrium and transient optical phenomena, yet it remains experimentally challenging due to the simultaneous need for high temporal resolution and…

Quantum Physics · Physics 2026-03-20 C. Hainaut , K. Ouahrouche , A. Rancon , G. Patera , C. Ouarkoub , M. Le Parquier , P. Suret , A. Amo

The paper presents a system for measuring photon statistics and photon timing in the few-photon regime down to the single-photon level. The measurement system is based on superconducting nanowire single photon detectors and a…

Instrumentation and Detectors · Physics 2018-04-04 N. Lusardi , J. W. N. Los , R. B. M. Gourgues , G. Bulgarini , A. Geraci

Quantum spectroscopy was performed using the frequency-entangled broadband photon pairs generated by spontaneous parametric down-conversion. An absorptive sample was placed in front of the idler photon detector, and the frequency of signal…

Quantum Physics · Physics 2009-11-10 Atsushi Yabushita , Takayoshi Kobayashi

In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…

Quantum Physics · Physics 2026-04-24 Arunangshu Debnath , Shaul Mukamel

The second-order temporal interference between two independent single-mode continuous-wave lasers is discussed by employing two-photon interference in Feynman's path integral theory. It is concluded that whether the second-order temporal…

Optics · Physics 2016-03-18 Jianbin Liu , Dong Wei , Hui Chen , Yu Zhou , Huaibin Zheng , Hong Gao , Fu-li Li , Zhuo Xu

A unified description of multitime correlation functions, nonlinear response functions, and quantum measurements is developed using a common generating function which allows a direct comparison of their information content. A general formal…

Statistical Mechanics · Physics 2009-11-10 Shaul Mukamel

Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…

Optics · Physics 2024-03-08 Bingxin Xu , Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué
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