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We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

The ground state of the quantum spin ice candidate magnet Yb2Ti2O7 is known to be sensitive to weak disorder at the 1 percent level which occurs in single crystals grown from the melt. Powders produced by solid state synthesis tend to be…

Strongly Correlated Electrons · Physics 2016-03-09 J. Gaudet , K. A. Ross , E. Kermarrec , N. P. Butch , G. Ehlers , H. A. Dabkowska , B. D. Gaulin

Low-temperature powder neutron diffraction measurements are performed in the ordered magnetic state of the pyrochlore antiferromagnet Gd2Sn2O7. Symmetry analysis of the diffraction data indicates that this compound has the ground state…

We present an interpretation of zero field diffuse neutron scattering and of high field magnetisation data at very low temperature in the frustrated pyrochlore system Tb2Ti2O7. This material has antiferromagnetic exchange interactions and…

Strongly Correlated Electrons · Physics 2013-12-16 P. Bonville , A. Gukasov , I. Mirebeau , S. Petit

We report neutron diffraction measurements of the magnetic structures in two pyrochlore iridates, Yb2Ir2O7 and Lu2Ir2O7. Both samples exhibit the all-in-all-out magnetic structure on the Ir4+ sites below TN~ 150,K, with a low temperature…

In the pyrochlore compounds, Tb$_2$Ti$_2$O$_7$ and Tb$_2$Sn$_2$O$_7$, only the Tb$^{3+}$ ions are magnetic. They exhibit quite abnormal -- and, in view of their chemical similarity, strikingly different -- magnetic behaviour, as probed by…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apetrei , I. N. Goncharenko , R. Moessner

We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

The ytterbium pyrochlore magnets, Yb2B2O7 (B = Sn, Ti, Ge) are well described by S_eff = 1/2 quantum spins decorating a network of corner-sharing tetrahedra and interacting via anisotropic exchange. Structurally, only the non-magnetic…

Strongly Correlated Electrons · Physics 2016-03-30 A. M. Hallas , J. Gaudet , N. P. Butch , M. Tachibana , R. S. Freitas , G. M. Luke , C. R. Wiebe , B. D. Gaulin

The thermodynamic properties of the pyrochlore Yb2Ti2O7 material are calculated using the numericallinked-cluster (NLC) calculation method for an effective anisotropic-exchange spin-1/2 Hamiltonian with parameters recently determined by…

Strongly Correlated Electrons · Physics 2014-04-11 N. R. Hayre , K. A. Ross , R. Applegate , T. Lin , R. R. P. Singh B. D. Gaulin , M. J. P. Gingras

The rare earth pyrochlore material Gd2Ti2O7 is considered to be an ideal model frustrated Heisenberg antiferromagnet with additional dipolar interactions. For this system there are several untested theoretical predictions of the ground…

Condensed Matter · Physics 2009-11-07 J. D. M. Champion , A. S. Wills , T. Fennell , S. T. Bramwell , J. S. Gardner , M. A. Green

Recent neutron scattering and specific heat studies on the pyrochlore Yb2Ti2O7 have revealed variations in its magnetic behavior below 265mK. In the best samples, a sharp anomaly in the specific heat is observed at T=265mK. Other samples,…

Strongly Correlated Electrons · Physics 2013-02-01 K. A. Ross , Th. Proffen , H. A. Dabkowska , J. A. Quilliam , L. R. Yaraskavitch , J. B. Kycia , B. D. Gaulin

Paramagnetic correlations in the magnetic material Yb2Ti2O7 have been investigated via neutron scattering, revealing a [111] rod of scattering intensity. Assuming interactions between the Yb^{3+} ions composed of all symmetry-allowed…

Strongly Correlated Electrons · Physics 2011-06-28 Jordan D. Thompson , Paul A. McClarty , Henrik M. Ronnow , Louis P. Regnault , Andreas Sorge , Michel J. P. Gingras

Neutron powder diffraction and inelastic measurements were performed examining the 5d pyrochlore Y$_2$Ir$_2$O$_7$. Temperature dependent measurements were performed between 3.4 K and 290 K, spanning the magnetic transition at 155 K. No sign…

Strongly Correlated Electrons · Physics 2014-05-30 M. C. Shapiro , S. C. Riggs , M. B. Stone , C. R. de la Cruz , S. Chi , A. A. Podlesnyak , I. R. Fisher

Dy2Ti2O7 is a geometrically frustrated magnetic material with a strongly correlated spin ice regime that extends from 1 K down to as low as 60 mK. The diffuse elastic neutron scattering intensities in the spin ice regime can be remarkably…

Statistical Mechanics · Physics 2008-08-02 Taras Yavors'kii , Tom Fennell , Michel J. P. Gingras , Steven T. Bramwell

Recent elastic and inelastic neutron scattering studies of the highly frustrated pyrochlore antiferromagnet Tb2Ti2O7 have shown some very intriguing features that cannot be modeled by the local <111> classical Ising model, naively expected…

Disordered Systems and Neural Networks · Physics 2007-05-23 Ying-Jer Kao , Matthew Enjalran , Adrian Del Maestro , Hamid R. Molavian , Michel J. P. Gingras

We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

Neutron scattering measurements show the ferromagnetic XY pyrochlore Yb2Ti2O7 to display strong quasi-two dimensional (2D) spin correlations at low temperature, which give way to long range order (LRO) under the application of modest…

Strongly Correlated Electrons · Physics 2010-02-08 K. A. Ross , J. P. C. Ruff , C. P. Adams , J. S. Gardner , H. A. Dabkowska , Y. Qiu , J. R. D. Copley , B. D. Gaulin

We report neutron scattering and muon spin relaxation measurements (muSR) on the pyrochlore antiferromagnet Yb2Ge2O7. Inelastic neutron scattering was used to probe the transitions between crystal electric field levels, allowing us to…

We document the coexistence of ferro- and anti-ferromagnetism in pyrochlore $\rm Yb_2Ti_2O_7$ using three neutron scattering techniques on stoichiometric crystals: elastic neutron scattering shows a canted ferromagnetic ground state,…

Strongly Correlated Electrons · Physics 2020-10-27 A. Scheie , J. Kindervater , S. Zhang , H. J. Changlani , G. Sala , G. Ehlers , A. Heinemann , G. S. Tucker , S. M. Koohpayeh , C. Broholm

We report neutron diffraction studies of TbCo$_2$Zn$_{20}$ and TbFe$_2$Zn$_{20}$, two isostructural compounds which exhibit dramatically different magnetic behavior. In the case of TbCo$_2$Zn$_{20}$, magnetic Bragg peaks corresponding to…

Strongly Correlated Electrons · Physics 2015-05-18 W. Tian , A. D. Christianson , J. L. Zarestky , S. Jia , S. L. Bud'ko , P. C. Canfield , P. M. B. Piccoli , A. J. Schultz
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