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Ab-initio relativistic dynamical mean-field theory is applied to resolve the long-standing controversy between theory and experiment in the "simple" face-centered cubic phase of plutonium called delta-Pu. In agreement with experiment,…

Strongly Correlated Electrons · Physics 2009-11-11 L. V. Pourovskii , M. I. Katsnelson , A. I. Lichtenstein , L. Havela , T. Gouder , F. Wastin , A. B. Shick , V. Drchal , G. H. Lander

The Hohenberg-Kohn theorem of density functional theory (DFT) for the case of electrons interacting with an external magnetic field (that couples to spin only) is examined in more detail than previously. A unexpected generalization is…

Strongly Correlated Electrons · Physics 2009-10-31 H. Eschrig , W. E. Pickett

For more than three decades, clear discrepancies have existed between spin densities in momentum space revealed by Magnetic Compton scattering experiments and theoretical calculations based on density functional theory (DFT). Here by making…

Strongly Correlated Electrons · Physics 2024-02-02 A. D. N. James , E. I. Harris-Lee , S. B. Dugdale

Many theories published in the last decade propose that either ordered or disordered local moments are present in elemental plutonium at low temperatures. We present new experimental data and review previous experimental results. None of…

Materials Science · Physics 2009-11-10 J. C. Lashley , A. C. Lawson , R. J. McQueeney , G. H. Lander

We measured phonon frequencies and linewidths in doped and undoped BaFe2As2 single crystals by inelastic x-ray scattering and compared our results with density functional theory (DFT) calculations. In agreement with previous work, the…

We briefly report on calculated addition spectra for electrons in a circular quantum dot with perpendicular magnetic field. We compare our current density functional theory calculations with recent experiments by Tarucha et al. [PRL 77,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Oliver Steffens , Ulrich Roessler , Michael Suhrke

In the framework of density functional theory (DFT), the structural and magnetic properties of FeN mono nitride have been investigated using the all electrons augmented spherical wave method (ASW) with a generalized gradient GGA functional…

Materials Science · Physics 2009-09-08 A. Houari , S. F. Matar , M. A. Belkhir , M. Nakhl

Recent discoveries of multi-\textbf{Q} magnetic structures in centrosymmetric compounds have stimulated growing interest in their microscopic origin and observable properties. Here, we calculate the dynamical magnetic structure factor for a…

Strongly Correlated Electrons · Physics 2025-12-09 Artem O. Nosenko , Dmitri V. Efremov

The possibility of magnetic-order induced phonon anisotropy in single crystals of MnO and NiO is investigated using inelastic neutron scattering. Below Tn both compounds exhibit a splitting in their transverse optical phonon spectra of…

Strongly Correlated Electrons · Physics 2009-11-10 E. M. L. Chung , D. McK. Paul , G. Balakrishnan , M. R. Lees , A. Ivanov , M. Yethiraj

In this work using the density functional theory (DFT), we have studied the structural, electronic and magnetic properties of uranium dioxide with antiferromagnetic 1k-, 2k-, and 3k-order structures. Ordinary approximations in DFT, such as…

Materials Science · Physics 2020-08-25 Samira Sheykhi , Mahmoud Payami

The structural, magnetic, and thermodynamic properties of a new plutonium based compound, Pu2Pt3Si5, are reported. Single crystals produced by a Sn-flux technique have been analyzed showing a ferromagnetic behavior at 58 K. Pu2Pt3Si5…

Materials Science · Physics 2013-12-06 J. -C. Griveau , E. Colineau , D. Bouëxiere , K. Gofryk , T. Klimczuk , J. Rebizant

In the previous papers (quant-ph/0204037), (quant-ph/0204134) on the basis of Dirac's equation we have considered the electromagnetic interpretation of the quantum theory of electron. Here we continue the electron structure study. Since the…

Quantum Physics · Physics 2007-05-23 Alexander G. Kyriakos

In this paper density functionals for Coulomb systems subjected to electric and magnetic fields are developed. The density functionals depend on the particle density, $\rho$, and paramagnetic current density, $j^p$. This approach is…

Mathematical Physics · Physics 2014-05-26 Andre Laestadius

The different crystal structures of ferromagnetic Ni$_2$MnGa have been calculated using density functional theory (DFT) with special emphasis on the modulated structures 10M and 14M. These are important for understanding the stability of…

Materials Science · Physics 2007-05-23 A. Zayak , W. A. Adeagbo , P. Entel , V. D. Buchelnikov

The body-centered cubic Coulomb crystal of ions in the presence of a uniform magnetic field is studied using the rigid electron background approximation. The phonon mode spectra are calculated for a wide range of magnetic field strengths…

High Energy Astrophysical Phenomena · Physics 2014-11-20 D. A. Baiko

Electronic correlations associated with incipient magnetism have long been recognized as an important factor in stabilizing the largest atomic volume $\delta$ phase of plutonium, yet their strength compared to those in the rare earths and…

Strongly Correlated Electrons · Physics 2022-01-10 M. Wartenbe , P. H. Tobash , J. Singleton , L. E. Winter , S. Richmond , N. Harrison

We use density functional theory to study the structural, magnetic and electronic structure of the organo-metallic quantum magnet $\mathrm{NiCl_2-4SC(NH_2)_2}$ (DTN). Recent work has demonstrated the quasi-1D nature of the molecular crystal…

Mesoscale and Nanoscale Physics · Physics 2021-03-03 Maher Yazback , Jie-Xiang Yu , Shuanglong Liu , Long Zhang , Neil S. Sullivan , Hai-Ping Cheng

Phonon polaritons (PhPs) in freestanding and supported multilayers (MuLs) of hexagonal boron nitride (hBN) are systematically studied using a macroscopic optical-phonon model. The PhP properties such as confinement, group velocity,…

Mesoscale and Nanoscale Physics · Physics 2022-03-14 Jian-zhong Zhang

We present a Density Functional Theory (DFT) based first-principles study on iron chalcogenides superconductor FeSe, systematically investigating pressure and doping induced modifications to its electronic, magnetic, and lattice dynamical…

Materials Science · Physics 2025-04-17 Abyay Ghosh , Piotr Chudzinski , Myrta Grüning

The spherically averaged structure function $\soq$ obtained from pulsed neutron powder diffraction contains both elastic and inelastic scattering via an integral over energy. The Fourier transformation of $\soq$ to real space, as is done in…

Materials Science · Physics 2016-08-31 D. A. Dimitrov , D. Louca , H. Röder