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Triplet excitons have been the focus of considerable attention with regards to the functioning of polymer solar cells, because these species are long-lived and quench subsequently generated singlet excitons in their vicinity. The role of…

Chemical Physics · Physics 2018-02-14 Florian Steiner , John M. Lupton , Jan Vogelsang

The emergence of oxygenic photosynthesis created a new niche with dramatic potential to transform energy flow through Earth's biosphere. However, more primitive forms of photosynthesis that fix CO2 into biomass using electrons from reduced…

Earth and Planetary Astrophysics · Physics 2019-07-31 Kazumi Ozaki , Katharine J. Thompson , Rachel L. Simister , Sean A. Crowe , Christopher T. Reinhard

We present the results of kinetic modelling of quantum effects in laser-beam interaction. In the developed numerical model, electron-positron pair production by hard photons, hard photon emission and the electromagnetic fields generated by…

Plasma Physics · Physics 2015-05-27 Evgeny Nerush , Igor Kostyukov

Two-electron charged self-assembled quantum dot molecules exhibit a decoherence-avoiding singlet-triplet qubit subspace and an efficient spin-photon interface. Here, we demonstrate that the cycling transitions originating from auxiliary…

Mesoscale and Nanoscale Physics · Physics 2015-09-15 Y. L. Delley , M. Kroner , S. Faelt , W. Wegscheider , A. İmamoğlu

We show influence of electric field and magnetic flux on spin entanglement in an artificial triangular molecule build of coherently coupled quantum dots. In a subspace of doublet states an explicit relation of concurrence with spin…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Jukub Luczak , Bogdan R. Bulka

We have investigated the low temperature specific heat properties as a function of magnetic field in the strongly correlated layered cobalt oxide [BiBa$_{0.66}$K$_{0.36}$O$_2$]CoO$_2$. These measurements reveal two kinds of magnetic field…

Strongly Correlated Electrons · Physics 2010-08-24 P. Limelette , H. Muguerra , S. Hebert

A new dual plasma coating process to produce platinum-free catalysts for the oxygen reduction reaction in a fuel cell is introduced. The catalysts thus produced were analysed with various methods. Electrochemical characterisation was…

Full control of molecular interactions, including reactive losses, would open new frontiers in quantum science. Here, we demonstrate extreme tunability of chemical reaction rates by using an external electric field to shift excited…

Singlet fission, an exciton multiplication process in organic semiconductors which converts one singlet exciton into two triplet excitons is a promising way to reduce thermalization losses in conventional solar cells. One way to harvest…

Applied Physics · Physics 2018-10-09 Moritz H. Futscher , Akshay Rao , Bruno Ehrler

Fe(II)-porphyrins (FeP) play an important role in many reactions relevant to material science and biological processes, due to their closely lying spin states. However, this small energetic separation also makes it challenging to establish…

Photodissociation of a molecule produces a spatial distribution of photofragments determined by the molecular structure and the characteristics of the dissociating light. Performing this basic chemical reaction at ultracold temperatures…

Atomic Physics · Physics 2018-01-24 M. McDonald , I. Majewska , C. -H. Lee , S. S. Kondov , B. H. McGuyer , R. Moszynski , T. Zelevinsky

We probe the dynamics of dissociating CS$_2$ molecules across the entire reaction pathway upon excitation. Photoelectron spectroscopy measurements using laboratory-generated femtosecond extreme ultraviolet pulses monitor the competing…

A quantum kinetic theory for correlated charged-particle systems in strong time-dependent electromagnetic fields is developed. Our approach is based on a systematic gauge-invariant nonequilibrium Green's functions formulation. We…

Strongly Correlated Electrons · Physics 2017-08-23 M. Bonitz , Th Bornath , D. Kremp , H. Haberland , M. Schlanges , P. Hilse

We report on the spin properties of individual Mn atoms in II-VI semiconductor strain free quantum dots. Strain free Mn-doped CdTe quantum dots are formed by width fluctuations in thin quantum wells lattice matched on a CdTe substrate.…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 L. Besombes , H. Boukari

We show that spin-orbit coupling in a quantum dot molecule allows for coherent manipulation of two electron spin states using Raman transitions. Such two-electron spin states defined by the singlet and triplet states of two exchange coupled…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Hakan E. Türeci , J. M. Taylor , A. Imamoglu

A combination of electron spin interactions in a magnetic field allows us to control the resonance frequencies of a high-Q Whispering Gallery (WG) cavity mode doublet, resulting in precise measurements of an avoided crossing between the two…

Quantum Physics · Physics 2014-10-17 Maxim Goryachev , Warrick G. Farr , Daniel L. Creedon , Michael E. Tobar

Energy spectrum fine structure of triplet two-electron states is investigated theoretically. Spin-orbit interaction induced terms in the effective Hamiltonian of electron-electron interaction are derived for zinc-blende lattice…

Mesoscale and Nanoscale Physics · Physics 2009-12-10 M. M. Glazov

Ultra-intense laser pulses can create sufficiently strong fields to probe quantum electrodynamics effects in a novel regime. By colliding a 60 GeV electron bunch with a laser pulse focussed to the maximum achievable intensity of $10^{23}$…

Photons are ideal carriers for quantum information as they can have a long coherence time and can be transmitted over long distances. These properties are a consequence of their weak interactions within a nearly linear medium. To create and…

Quantum entanglement effects between the electronic spin and charge degrees of freedom are examined in an organic molecular solid, termed a dimer-Mott insulating system, in which molecular dimers are arranged in a crystal as fundamental…

Strongly Correlated Electrons · Physics 2016-05-18 Makoto Naka , Sumio Ishihara
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