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Monolayers of transition metal dichalcogenides (TMDs) have recently emerged as a promising optoelectronic platform. To leverage their full potential, however, it is important to understand and engineer the properties of the different…

Single layers of transition metal dichalcogenides are two-dimensional direct bandgap semiconductors with degenerate, but inequivalent, `valleys' in the electronic structure that can be selectively excited by polarized light. Coherent…

Materials Science · Physics 2017-07-21 Yen-Jung Chen , Jeffrey D. Cain , Teodor K. Stanev , Vinayak P. Dravid , Nathaniel P. Stern

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

Moire lattices attract significant attention in double-layer graphene and TMD layer heterostructures as well as in photonic crystals due to the interesting exotic physics that emerges within these structures. However, direct measurement of…

Integrating two-dimensional van der Waals materials with optical cavities has revealed a fascinating platform to study exciton-polariton physics. Manipulating exciton polaritons often requires external control over the electrical and…

Optics · Physics 2023-11-08 Zhi Wang , Li He , Bumho Kim , Bo Zhen

Transition metal dichalcogenide (TMD) monolayers are direct bandgap semiconductors that feature tightly bound excitons, strong spin-orbit coupling, and spin-valley degrees of freedom. Depending on the spin configuration of the electron-hole…

Localized excitons play a vital role in the optical response of monolayers of transition metal dichalcogenides and can be exploited as single photon sources for quantum information technology. While the optical properties of such localized…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 F. Lengers , T. Kuhn , D. E. Reiter

Atomically thin two-dimensional crystals have revolutionized materials science. In particular, monolayer transition metal dichalcogenides promise novel optoelectronic applications, due to their direct energy gaps in the optical range. Their…

The two-dimensional transition-metal dichalcogenides (2D TMDCs) are an intriguing platform for studying light-matter interactions because they combine the electronic properties of conventional semiconductors with the optical resonances…

Mesoscale and Nanoscale Physics · Physics 2022-05-02 Aaron H. Rose , Taylor J. Aubry , Hanyu Zhang , Jao van de Lagemaat

In transition metal dichalcogenides layers of atomic scale thickness, the electron-hole Coulomb interaction potential is strongly influenced by the sharp discontinuity of the dielectric function across the layer plane. This feature results…

Despite 2D materials holding great promise for a broad range of applications, the proliferation of devices and their fulfillment of real-life demands are still far from being realized. Experimentally obtainable samples commonly experience a…

Mesoscale and Nanoscale Physics · Physics 2021-01-07 Pavel V. Kolesnichenko , Qianhui Zhang , Changxi Zheng , Michael S. Fuhrer , Jeffrey A. Davis

Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical…

Controlling excitons at the nanoscale in semiconductor materials represents a formidable challenge in the fields of quantum photonics and optoelectronics. Achieving this control holds great potential for unlocking strong exciton-exciton…

We report a new dark exciton in monolayer MoS$_2$ using second harmonic generation spectroscopy. Hereby, the spectrally dependent second harmonic generation intensity splits into two branches, and an anticrossing is observed at $\sim$ 25…

Mesoscale and Nanoscale Physics · Physics 2024-08-22 Chenjiang Qian , Viviana Villafañe , Pedro Soubelet , Peirui Ji , Andreas V. Stier , Jonathan J. Finley

Excitons in monolayer transition metal dichalcogenide (TMD) provide a paradigm of composite Boson in 2D system. This letter reports a photoluminescence and reflectance study of excitons in monolayer molybdenum diselenide (MoSe2) with…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Ke Xiao , Tengfei Yan , Qiye Liu , Siyuan Yang , Chiming Kan , Ruihuan Duan , Zheng Liu , Xiaodong Cui

Exciton-polaritons, elementary excitations arising from the strong coupling regime between photons and excitons in insulators or semiconductors, represent a promising platform for studying quantum fluids of light and realizing prospective…

Excitons play a key role for the optoelectronic properties of hybrid systems. We apply near-field scanning optical microscopy (NSOM) with a $100\,\text{-nm}$ spatial resolution to study the photoluminescence of surface excitons (SX) in a…

Mesoscale and Nanoscale Physics · Physics 2015-03-31 Sebastian Friede , Sergei Kuehn , Sergey Sadofev , Sylke Blumstengel , Fritz Henneberger , Thomas Elsaesser

Two-dimensional transition metal dichalcogenide (TMD) semiconductors provide a unique possibility to access the electronic valley degree of freedom using polarized light, opening the way to valley information transfer between distant…

Transport of elementary excitations is a fundamental property of 2D semiconductors, important for wide-ranging emergent phenomena and device applications. While exciton transport reported in 2D materials barely exceeds 1-2 $\mu$m, coherent…

Optics · Physics 2025-06-03 Xin Xie , Qiuyang Li , Chenxi Liu , Yuze Liu , Chulwon Lee , Kai Sun , Hui Deng

Low-dimensional materials differ from their bulk counterpart in many respects. In particular, the screening of the Coulomb interaction is strongly reduced, which can have important consequences such as the significant increase of exciton…