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An experimental realization of high-precision direct frequency comb spectroscopy using counter-propagating femtosecond pulses on two-photon atomic transitions is presented. Doppler broadened background signal, hampering precision…

Atomic Physics · Physics 2013-07-11 Itan Barmes , Stefan Witte , Kjeld S. E. Eikema

We demonstrate numerically a method of focusing two-photon field inside one-dimensional random media. The approach is based on coherent control of backscattering achieved by adaptive spectral pulse shaping. The spectral phases of a…

Optics · Physics 2016-03-02 Alex C. Han , Valery Milner

We present a new method for generating a regular train of ultrashort optical pulses in a prepared two-level medium. The train develops from incident monochromatic probe radiation travelling in a medium of atoms, which are in a quantum…

Quantum Physics · Physics 2015-05-13 Gevorg Muradyan , A. Zh. Muradyan

While time-resolved pump-probe differential reflectivity and transmitivity measurements are routinely used to monitor the population relaxation dynamics on the subpicosecond time scale, it is also known that the signal in the negative delay…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Richarj Mondal , Basabendra Roy , Bipul Pal , Bhavtosh Bansal

A pulsed source of entangled photons is desirable for some applications. Yet, such a source has intrinsic problems arising from the simultaneous arrival of the signal and noise photons to the detectors. These problems are analyzed and…

Optics · Physics 2015-06-18 Mónica B. Agüero , Alejandro A. Hnilo , Marcelo G. Kovalsky

We demonstrate low-frequency interferometric impulsive stimulated Raman scattering (ISRS) imaging with high robustness to distortions by optical scattering. ISRS is a pump-probe coherent Raman spectroscopy that can capture Raman vibrational…

We present a novel and straightforward approach for the spatio-spectral characterization of ultrashort pulses. This minimally intrusive method relies on placing a mask with specially arranged pinholes in the beam path before the focusing…

Intense ultrashort pulse lasers are used for fs resolution pumpprobe experiments more and more at large scale facilities, such as free electron lasers (FEL). Measurement of the arrival time of the laser pulses and stabilization to the…

Instrumentation and Detectors · Physics 2023-07-19 Marta Csatari Divall , Patrick Mutter , Edwin J. Divall , Christoph P. Hauri

We present a robust approach to incorporating models for the time-variable broadening of the pulse profile due to scattering in the ionized interstellar medium into profile-domain pulsar timing analysis. We use this approach to…

Instrumentation and Methods for Astrophysics · Physics 2017-04-12 L. Lentati , M. Kerr , S. Dai , R. M. Shannon , G. Hobbs , S. Oslowski

We consider the theory of the non-linear spectroscopy for a single molecule undergoing stochastic dynamics and interacting with a sequence of two laser pulses. General expressions for photon counting statistics are obtained, and an exact…

Optics · Physics 2008-01-13 F. Shikerman , E. Barkai

We demonstrate a pump-probe strobe light spectroscopy for sensitive detection of magneto-optical dynamics in the context of hybrid magnonics. The technique uses a combinatorial microwave-optical pump-probe scheme, leveraging both the…

With their brilliance and temporal structure, X-ray free-electron laser can unveil atomic-scale details of ultrafast phenomena. Recent progress in split-and-delay optics (SDO), which produces two X-ray pulses with time-delays, offers bright…

The radio polarization characteristics of millisecond pulsars (MSPs) differ significantly from those of non-recycled pulsars. In particular, the position angle (PA) swings of many MSPs deviate from the S-shape predicted by the rotating…

Solar and Stellar Astrophysics · Physics 2015-05-27 C. T. Y. Chung , A. Melatos

We demonstrate an approach to two-dimensional electronic spectroscopy (2DES) that combines the benefits of shot-to-shot detection at high-repetition rates with the simplicity of a broadband white light continuum input and conventional…

Optics · Physics 2023-10-03 Asha S. Thomas , Vivek N. Bhat , Vivek Tiwari

Stimulated Raman scattering of a laser pump pulse seeded by a Stokes pulse generically leaves a two-level medium initially at rest in an excited state constituted of static solitons and radiation. The soliton birth manifests as sudden very…

solv-int · Physics 2016-09-08 J. Leon , A. V. Mikhailov

In a single shot, we measure the full propagation path, including the evolution to pulse collapse, of a high power femtosecond laser pulse propagating in air. This technique enables single-shot examination of the effect of parameters that…

Compton scattering of short and ultra short (sub-cycle) laser pulses off mildly relativistic electrons is considered within a QED framework. The temporal shape of the pulse is essential for the differential cross section as a function of…

High Energy Physics - Phenomenology · Physics 2015-06-22 Alexander I. Titov , Burkhard Kampfer , Takuya Shibata , Atsushi Hosaka , Hideaki Takabe

Nonlinear spectroscopy employs a series of laser pulses to interrogate dynamics in large interacting many-body systems, and has become a highly successful method for experiments in chemical physics. Current quantum optical experiments…

Quantum Physics · Physics 2016-10-19 Frank Schlawin , Manuel Gessner , Shaul Mukamel , Andreas Buchleitner

Coherent phonons (CP) generated by laser pulses on the femtosecond scale have been proposed as a means to achieve ultrafast, non-thermal switching in phase-change materials such as Ge$_{2}$Sb$_{2}$Te$_{5}$(GST). Here we use ultrafast…

Despite the multitude of available methods, the characterisation of ultrafast pulses remains a challenging endeavour, especially at the single-photon level. We introduce a pulse characterisation scheme that maps the magnitude of its…