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We study the dynamics of the phase behavior of a polymer blend in the presence of shear flow. By adopting a two fluid picture and using a generalization of the concept of material derivative, we construct kinetic equations that describe the…

Soft Condensed Matter · Physics 2009-10-30 Tao Sun , Anna C. Balazs , David Jasnow

Recent experiments performed on a variety of soft glassy materials have demonstrated that any imposed shear flow serves to simultaneously fluidize these systems in all spatial directions [Ovarlez \textit{et al.} (2010)]. When probed with a…

Soft Condensed Matter · Physics 2012-02-27 T. F. F. Farage , J. M. Brader

The process of crystal nucleation can be accelerated or retarded by ultrasonic vibration, which is particularly attractive for the addictive manufacture and thermoplastic forming of metallic glasses, however, the effect and mechanism of…

Materials Science · Physics 2022-12-06 Baoshuang Shang , Noel Jakse , Pengfei Guan , Weihua Wang , Jean-louis Barrat

The nucleation of crystals in liquids is one of nature's most ubiquitous phenomena, playing an important role in areas such as climate change and the production of drugs. As the early stages of nucleation involve exceedingly small time and…

Classical theory of nucleation based on Becker-Doering equations and coarsening for a binary alloy.

Materials Science · Physics 2007-05-23 J. C. Neu , L. L. Bonilla

Shear flow is known to induce huge density fluctuations in otherwise clear and uniform polymer solutions. This effect is rooted in the elasticity of the entangled polymer network, and can span distances over a thousand chains wide. It has…

Computational Physics · Physics 2018-08-21 Airidas Korolkovas

Nucleation and growth is the dominant relaxation mechanism driving first order phase transitions. In two-dimensional at systems nucleation has been applied to a wide range of problems in physics, chemistry and biology. Here we study…

Soft Condensed Matter · Physics 2016-03-09 Leopoldo R. Gomez , Nicolas A. Garcia , Vincenzo Vitelli , Jose Lorenzana , Daniel A. Vega

Heterogeneous nucleation of a new bulk phase on a flat substrate can be associated with the surface phase transition called wetting transition. When this bulk heterogeneous nucleation occurs on a completely-wettable flat substrate with a…

Soft Condensed Matter · Physics 2015-05-28 Masao Iwamatsu

A kinetic theory of homogeneous crystal nucleation in unary droplets is presented taking into account that a crystal nucleus can form not only in the volume-based mode (with all its facets within the droplet) but also in the…

Materials Science · Physics 2016-09-28 Yuri S. Djikaev

Heterogeneous nucleation on catalytic surfaces plunged into a fluid is described through a stochastic model. To generate this non-equilibrium process we assume that the turn on of a electrostatic potential triggers a complex dynamics that…

Chemical Physics · Physics 2007-05-23 P. C. T. Dajello , I. Mozolevski , Z. G. S. Kipervaser

Non-aligning self-propelled particles with purely repulsive excluded volume interactions undergo athermal motility-induced phase separation into a dilute gas and a dense cluster phase. Here, we use enhanced sampling computational methods…

Soft Condensed Matter · Physics 2016-10-05 Gabriel S. Redner , Caleb G. Wagner , Aparna Baskaran , Michael F. Hagan

The shear viscosity in the dilute regime of a model for confined granular matter is studied by simulations and kinetic theory. The model consists on projecting into two dimensions the motion of vibrofluidized granular matter in shallow…

Statistical Mechanics · Physics 2015-06-22 Rodrigo Soto , Dino Risso , Ricardo Brito

The motion of a deformable active particle in linear shear flow is explored theoretically. Based on symmetry considerations, in two spatial dimensions, we propose coupled nonlinear dynamical equations for the particle position, velocity,…

Soft Condensed Matter · Physics 2014-01-28 Mitsusuke Tarama , Andreas M. Menzel , Borge ten Hagen , Raphael Wittkowski , Takao Ohta , Hartmut Löwen

Understanding the mechanism of nucleation of the stable phase inside the metastable parent phase during a first order phase transition has been a subject of outstanding interest in natural science. The problem becomes even more challenging…

Soft Condensed Matter · Physics 2007-05-23 Prabhakar Bhimalapuram , Suman Chakrabarty , Biman Bagchi

We theoretically investigate homogeneous crystal nucleation in a solution containing a solute and a volatile solvent. The solvent evaporates from the solution, thereby continuously increasing the concentration of the solute. We view it as…

Soft Condensed Matter · Physics 2023-11-16 R. de Bruijn , J. J. Michels , P. van der Schoot

Motivated by the reported peculiar dynamics of a red blood cell in shear flow, we develop an analytical theory for the motion of a nearly--spherical fluid particle enclosed by a visco--elastic incompressible interface in linear flows. The…

Fluid Dynamics · Physics 2010-07-06 Petia M. Vlahovska , Yuan-nan Young , Gerrit Danker , Chaouqi Misbah

Recently, it was shown that a theoretical description of nucleation based on fluctuating hydrodynamics and classical density functional theory can be used to determine non-classical nucleation pathways for crystallization (Lutsko, Sci. Adv.…

Chemical Physics · Physics 2024-06-26 James F. Lutsko , Cédric Schoonen

The past few years have seen many advances in our understanding of the dynamics of polymeric fluids. These include improvements on the successful reptation theory; an emerging molecular theory of semiflexible chain dynamics; and an…

Soft Condensed Matter · Physics 2007-05-23 Peter D. Olmsted

We review our recent modeling of crystal nucleation and polycrystalline growth using a phase field theory. First, we consider the applicability of phase field theory for describing crystal nucleation in a model hard sphere fluid. It is…

Soft Condensed Matter · Physics 2007-05-23 L. Granasy , T. Pusztai , T. Borzsonyi

We analyze the behavior of supercooled fluids under shear both theoretically and numerically. Theoretically, we generalize the mode-coupling theory of supercooled fluids to systems under stationary shear flow. Our starting point is the set…

Soft Condensed Matter · Physics 2009-11-10 Kunimasa Miyazaki , David R. Reichman , Ryoichi Yamamoto