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The fragmentation of molecular cations following inner-shell decay processes in molecules containing heavy elements underpins the x-ray damage effects observed in x-ray scattering measurements of biological and chemical materials, as well…

Chemical Physics · Physics 2024-06-17 Adam E. A. Fouda , Stephen H. Southworth , Phay J. Ho

Our exact theory for continuous harmonic perturbation of a one dimensional model atom by parametric variations of its potential is generalized for the cases when a) the atom is exposed to short pulses of an external harmonic electric field…

Atomic and Molecular Clusters · Physics 2016-11-03 Alexander Rokhlenko

We simulate the dynamics of H2+ and HD+ by direct solution of the time-dependent Schroedinger equation for the electronic and nuclear motion for the interaction of intense femtosecond pulses. On these timescales the rotational motion, even…

Atomic Physics · Physics 2007-05-23 J F McCann , Liang-You Peng , I D Williams , K T Taylor , D Dundas

We present a time-dependent quantum algorithm for nuclear inelastic scattering in the time-dependent basis function on qubits approach. This algorithm aims to quantum simulate a subset of the nuclear inelastic scattering problems that are…

Nuclear Theory · Physics 2021-07-28 Weijie Du , James P. Vary , Xingbo Zhao , Wei Zuo

A one dimensional model of the magnetic multipole volume plasma source has been developed for use in intense ion/neutral atom beam injectors. The model uses plasma transport coefficients for particle and energy flow to create a detailed…

Plasma Physics · Physics 2015-10-29 E Surrey , A J T Holmes

Ionization is a fundamental process in intense laser-matter interactions, and is known to cause plasma defocusing and intensity clamping. Here, we investigate theoretically the propagation dynamics of an intense laser pulse in a helium gas…

Optics · Physics 2020-11-25 Xiaohui Gao , Bonggu Shim

A scheme which allows to compute the dynamics of strongly correlated classical ions embedded into a partiallzy ionized quantum plasma by first principles molecular dynamics is presented. The dynamically screened dust approach of Joyce and…

Plasma Physics · Physics 2008-10-10 M. Bonitz , P. Ludwig , J. W. Dufty

Molecular rotation, vibration, internal rotation, isomerization, tunneling, intermolecular dynamics of weakly and strongly interacting systems, intra-to-inter-molecular energy transfer, hindered rotation and hindered translation over…

Chemical Physics · Physics 2022-12-02 Edit Mátyus , Alberto Martín Santa Daría , Gustavo Avila

We present a mixed quantum-classical approach to strong-field ionization - a semiclassical two-step model with quantum input. In this model the initial conditions for classical trajectories that simulate electron wave packet after…

Atomic Physics · Physics 2019-11-27 N. I. Shvetsov-Shilovski , M. Lein

The exact factorization of the time-dependent electron-nuclear wavefunction has been employed successfully in the field of quantum molecular dynamics simulations for interpreting and simulating light-induced ultrafast processes. In this…

Chemical Physics · Physics 2021-09-29 Federica Agostini , E. K. U. Gross

We investigate the time-evolution of quantum entanglement between an electron, liberated by a strong few-cycle laser pulse, and its parent ion-core. Since the standard procedure is numerically prohibitive in this case, we propose a novel…

Quantum Physics · Physics 2017-10-18 Szilárd Majorosi , Mihály G. Benedict , Attila Czirják

We present a theoretical framework to describe state-resolved ionization dynamics of neon atoms driven by ultraintense x-ray free-electron-laser pulses. In general, x-ray multiphoton ionization dynamics of atoms have been described by…

Atomic Physics · Physics 2023-01-10 Laura Budewig , Sang-Kil Son , Robin Santra

In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…

Atomic and Molecular Clusters · Physics 2009-11-13 Di-Fa Ye , Jing Chen , Jie Liu

We investigate the effect of incoherent perturbations on atomic photoionization due to a femtosecond mid-infrared laser pulse by solving the time-dependent stochastic Schr\"odinger equation. For a weak laser pulse which causes almost no…

Quantum Physics · Physics 2009-11-13 Kamal P. Singh , Jan M. Rost

In the first part of this paper, the different distinguishable pathways and regions of the single and sequential double ionization are determined and discussed. It is shown that there are two distinguishable pathways for the single…

Atomic Physics · Physics 2011-07-26 Firoozeh Sami , Mohsen Vafaee , Babak Shokri

We present a simple quantum mechanical model to describe Coulomb explosion of H$_2^+$ by short, intense, infrared laser pulses. The model is based on the length gauge version of the molecular strong-field approximation and is valid for…

Atomic Physics · Physics 2009-11-23 H. A. Leth , L. M. Madsen , J. F. McCann

The process of ionization of a hydrogen atom by a short infrared laser pulse is studied in the regime of very large pulse intensity, in the dipole approximation. Let $A$ denote the integral of the electric field of the pulse over time at…

Mathematical Physics · Physics 2015-05-18 Juerg Froehlich , Alessandro Pizzo , Benjamin Schlein

We have shown that it is possible to model accurately optical phenomena in intense laser fields by taking into account the intensity distribution over the laser beam. We developed a theoretical model that divided an intense laser beam into…

Atomic Physics · Physics 2016-03-09 Marcis Auzinsh , Andris Berzins , Ruvin Ferber , Florian Gahbauer , Uldis Kalnins

We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…

Atomic Physics · Physics 2015-05-18 C. P. J. Martiny , M. Abu-samha , L. B. Madsen

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost
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