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Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…

The ionization of a one-dimensional model Helium atom in short laser pulses using time-dependent density functional theory is investigated. We calculate ionization probabilities as a function of laser intensity by approximating the…

Atomic Physics · Physics 2009-11-13 F. Wilken , D. Bauer

Double electron ionisation process occurs when an intense laser pulse interacts with atoms or molecules. Exact {\it ab initio} numerical simulation of such a situation is extremely computer resources demanding, thus often one is forced to…

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

Atomic Physics · Physics 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

We report the highest compression reached in laboratory plasmas using eight laser beams, E$_{laser}$$\approx$12 kJ, $\tau_{laser}$=2 ns in third harmonic on a CD$_2$ target at the ShenGuang-II Upgrade (SGII-Up) facility in Shanghai, China.…

Nuclear fusion in ultra-dense deuterium D(-1) induced by 0.2 J pulses with 5 ns pulse length ejects ions with energies in the MeV range. The ns-resolved signal to a collector can be observed directly on an oscilloscope, showing ions…

Instrumentation and Detectors · Physics 2019-04-30 Leif Holmlid

We study the dynamics of initial nucleation processes of photoinduced structural change of molecular crystals. In order to describe the nonadiabatic transition in each molecule, we employ a model of localized electrons coupled with a fully…

Materials Science · Physics 2009-11-13 Kunio Ishida , Keiichiro Nasu

We investigate the role of nuclear motion and strong-field-induced electronic couplings during the double ionization of deuterated water using momentum-resolved coincidence spectroscopy. By examining the three-body dicationic dissociation…

The fixed-nuclei full dimensional time-dependent Schr \"odinger equation is directly solved for H$_2^+$ in the linearly polarized laser field of $I \sim 1.0 \times 10^{14}$W cm$^{-2}$ and $\lambda \sim 1064 $nm Instantaneous ionization rate…

Atomic Physics · Physics 2007-05-23 Mohsen Vafaee , Hassan Sabzyan , Zahra Vafaee , Ali Katanforoush

We present a theoretical study of the ionization dynamics of a hydrogen atom exposed to attosecond laser pulses in the extreme ultra violet region at very high intensities. The pulses are such that the electron is expected to reach…

Atomic Physics · Physics 2017-04-12 Tor Kjellsson , Sølve Selstø , Eva Lindroth

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

We demonstrate how the shape of femtosecond laser pulses can be tailored in order to obtain maximal ionization of atoms or molecules. For that purpose, we have overlayed a direct-optimization scheme on top of a fully unconstrained…

Computational Physics · Physics 2015-05-13 A. Castro , E. Rasanen , A. Rubio , E. K. U. Gross

We report the production of highly spin-polarized Deuterium atoms via photodissociation of deuterium iodide at 270 nm. The velocity distribution of both the deuterium and iodine photodissociation products is performed via velocity mapping…

Chemical Physics · Physics 2017-06-14 D. Sofikitis , P. Glodic , G. Koumarianou , H. Jiang , L. Bougas , P. C. Samartzis , A. Andreev , T. P. Rakitzis

We revisit the stabilization of ionization of atoms subjected to a superintense laser pulse using nonlinear dynamics. We provide an explanation for the lack of complete ionization at high intensity and for the decrease of the ionization…

Chaotic Dynamics · Physics 2015-06-23 Michael Norman , C. Chandre , T. Uzer , Peijie Wang

We investigate bulk ion heating in solid buried layer targets irradiated by ultra-short laser pulses of relativistic intensities using particle-in-cell simulations. Our study focuses on a CD2-Al-CD2 sandwich target geometry. We find…

Plasma Physics · Physics 2013-10-22 Lingen Huang , Michael Bussmann , Thomas Kluge , Anle Lei , Wei Yu , Thomas E. Cowan

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

The processes of ionization and energy transfer in a quantum system composed of two distant H atoms with an initial internuclear separation of 100 atomic units (5.29 nm) have been studied by the numerical solution of the time-dependent…

Quantum Physics · Physics 2017-09-13 Guennaddi K. Paramonov , Andre D. Bandrauk , Oliver Kühn

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

Atomic Physics · Physics 2015-02-25 Lun Yue , Lars Bojer Madsen

Using extreme-ultraviolet attosecond-pulse-trains, we investigate the photoionization dynamics of a Helium atom in the presence of moderately-strong (~10^12 W/cm^2) femtosecond laser pulses. The electronic structure of a laser-dressed atom…

Atomic Physics · Physics 2011-08-02 Niranjan Shivaram , Henry Timmers , Xiao-Min Tong , Arvinder S. Sandhu