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We investigate the nonequilibrium dynamics of the transverse field Ising chain (TFIC) using time-resolved resonant inelastic X-ray scattering (tr-RIXS) in a pump-probe setup within a condensed matter setting. The tr-RIXS spectra reveal…

Strongly Correlated Electrons · Physics 2025-09-26 Menglian Shi , Zhengzhong Du , Yi Lu

The presence of multiple bipartite entangled modes in squeezed states generated by four wave mixing in atomic vapors enables ultra-trace sensing, imaging, and metrology applications that are impossible to achieve with single-spatial-mode…

Quantum Physics · Physics 2015-12-31 B. J. Lawrie , R. C. Pooser , N. Otterstrom

The tunability and spatial precision of paramagnetic molecules makes them attractive for quantum sensing. However, usual microwave-based detection methods have poor temporal and spatial resolution, and optical methods compatible with…

Quantum Physics · Physics 2024-07-30 Erica Sutcliffe , Nathanael P. Kazmierczak , Ryan G. Hadt

The photoionization of chiral molecules prepared in a coherent superposition of excited states can give access to the underlying chiral coherent dynamics in a procedure known as photoexcitation induced photoelectron circular dichroism…

Atomic and Molecular Clusters · Physics 2018-08-29 Alex G Harvey , Zdeněk Mašín , Olga Smirnova

A novel technique to sensitively and selectively isolate multiple-quantum coherences in a femtosecond pump-probe setup is presented. Detecting incoherent observables and imparting lock-in amplification, even weak signals of highly dilute…

Atomic Physics · Physics 2017-02-28 Lukas Bruder , Marcel Binz , Frank Stienkemeier

Time Resolved Correlation (TRC) is a recently introduced light scattering technique that allows to detect and quantify dynamic heterogeneities. The technique is based on the analysis of the temporal evolution of the speckle pattern…

Soft Condensed Matter · Physics 2007-05-23 Agnes Duri , Hugo Bissig , Veronique Trappe , Luca Cipelletti

We discuss the potential creation and measurement of coherences in both dispersive solids and qubit-like single levels using current generation time- and angle-resolved photoemission technology. We show that in both cases, when both the…

Mesoscale and Nanoscale Physics · Physics 2020-05-22 Alexander F. Kemper , Avinash Rustagi

Two-dimensional electronic spectroscopy (2DES) can be implemented with different geometries, e.g., BOXCARS, collinear and pump-probe geometries. The pump-probe geometry has its advantage of overlapping only two beams and reducing phase…

Quantum Physics · Physics 2024-03-04 Mao-Rui Cai , Xue Zhang , Zi-Qian Cheng , Teng-Fei Yan , Hui Dong

In time-resolved pump-probe vibrational spectroscopy the internal stretch mode of polar molecules is utilized as a key observable to characterize the ultrafast dynamics of adsorbates on surfaces. The adsorbates non-adiabatic intermode…

Materials Science · Physics 2023-03-13 Raúl Bombín , Alberto S. Muzas , Dino Novko , J. Iñaki Juaristi , Maite Alducin

Coherent excitation of materials via ultrafast laser pulses can have interesting, observable dynamics in time-resolved photoemission measurements. The broad spectral width of ultrafast pump pulses can coherently excite multiple exciton…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Avinash Rustagi , Alexander F. Kemper

We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron and electron-phonon interactions, and captures exciton formation as well as the transition…

Materials Science · Physics 2025-02-13 Zhenlin Zhang , Wei Hu , Enrico Perfetto , Gianluca Stefanucci

We investigate photon tunneling in a pair of coupled inverted circular split-ring microwave resonators with four discrete chiral orientations. By varying the spacing between the resonators, we observe strong modulation of the transmission…

Developing from the transient absorption (TA) spectroscopy, the two dimensional (2D) spectroscopy with pump-probe geometry has emerged as a versatile approach for alleviating the difficulty on implementing the 2D spectroscopy with other…

Optics · Physics 2023-08-04 Mao-Rui Cai , Xue Zhang , Zi-Qian Cheng , Teng-Fei Yan , Hui Dong

Time-resolved x-ray scattering (TRXS) measures internuclear separations in a molecule following laser-induced photoexcitation. The molecular dynamics induced by the excitation laser may lie on one or several bound or dissociative electronic…

Atomic Physics · Physics 2019-09-25 MR Ware , JM Glownia , N Al-Sayyad , JT O'Neal , PH Bucksbaum

Understanding optical responses of topological matter is a central problem for enabling optoelectronic applications based on topological physics, which is of fundamental concern for photocurrents control and spectroscopy. Currently, schemes…

Other Condensed Matter · Physics 2026-04-24 Osamah Sufyan , Ofer Neufeld

Thermodynamic uncertainty relation (TUR) bounds coherence in stochastic oscillatory systems. In this paper, we show that both dynamical and thermodynamic bounds play important roles for the excitable oscillators, e.g. neurons. Firstly, we…

Statistical Mechanics · Physics 2024-12-24 Chunming Zheng

Optical pump-probe signals can be viewed as work done by the matter while transferring the energy between two coherent baths (from pump to probe). In thermodynamics a heat engine, such as laser, is a device which performs similar work but…

Quantum Physics · Physics 2021-04-14 Md Qutubuddin , Konstantin E. Dorfman

Time-resolved measurements of materials provide a wealth of information on quasiparticle dynamics, and have been the focus of optical studies for decades. In this paper, we develop a theory for explicitly evaluating time-resolved resonant…

Strongly Correlated Electrons · Physics 2019-03-27 Yuan Chen , Yao Wang , Chunjing Jia , Brian Moritz , Andrij M. Shvaika , James K. Freericks , Thomas P. Devereaux

Nonstationary molecular states which contain electronic coherences can be impulsively created and manipulated by using recently-developed ultrashort optical and X-ray pulses via photoexcitation, photoionization and Auger processes. We…

Chemical Physics · Physics 2015-09-02 Konstantin E. Dorfman , Kochise Bennett , Shaul Mukamel

In classical superconductors an energy gap and phase coherence appear simultaneously with pairing at the transition to the superconducting state. In high-temperature superconductors, the possibility that pairing and phase coherence are…

Superconductivity · Physics 2014-09-05 Ivan Madan , Toru Kurosawa , Yasunori Toda , Migaku Oda , Tomaz Mertelj , Primoz Kusar , Dragan Mihailovic