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We study the dynamics of optically-induced nuclear spin polarization in a fluorine-doped ZnSe epilayer via time-resolved Kerr rotation. The nuclear polarization in the vicinity of a fluorine donor is induced by interaction with coherently…

Mesoscale and Nanoscale Physics · Physics 2016-02-24 F. Heisterkamp , E. Kirstein , A. Greilich , E. A. Zhukov , T. Kazimierczuk , D. R. Yakovlev , A. Pawlis , M. Bayer

Hyperfine interactions between electron and nuclear spins in the quantum Hall regime provide powerful means for manipulation and detection of nuclear spins. In this work we demonstrate that significant changes in nuclear spin polarization…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Y. Q. Li , V. Umansky , K. von Klitzing , J. H. Smet

We analyze electron spin relaxation in electronic transport through coherently coupled double quantum dots in the spin blockade regime. In particular, we focus on hyperfine interaction as the spin relaxation mechanism. We pay special…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 Carlos López-Monís , Jesús Iñarrea , Gloria Platero

Sizable nuclear spin polarization is pumped in individual InP/GaInP dots in a wide range of external magnetic fields B_ext=0-5T by circularly polarized optical excitation. We observe nuclear polarization of up to ~40% at Bext=1.5T and…

Dynamic nuclear polarization (DNP) has revolutionized the field of NMR spectroscopy, expanding its reach and capabilities to investigate diverse materials, biomolecules, and complex dynamic processes. Bringing high-efficiency DNP to the…

Mesoscale and Nanoscale Physics · Physics 2024-02-27 Sahand Tabatabaei , Pritam Priyadarsi , Namanish Singh , Pardis Sahafi , Daniel Tay , Andrew Jordan , Raffi Budakian

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

The effect of nuclear spins in Fe/GaAs all-electrical spin-injection devices is investigated. At temperatures below 50 K, strong modifications of the non-local spin signal are found that are characteristic for hyperfine coupling between…

Mesoscale and Nanoscale Physics · Physics 2010-04-08 G. Salis , A. Fuhrer , S. F. Alvarado

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

We theoretically study the interplay of spin-orbit and hyperfine interactions in dynamical nuclear polarization in two-electron semiconductor double quantum dots near the singlet $(S)$ - triplet $(T_+)$ anticrossing. The goal of the scheme…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 Marko J. Rančić , Guido Burkard

Resistively detected NMR (RDNMR) based on dynamic nuclear polarization (DNP) in a quantum Hall ferromagnet (QHF) is a highly-sensitive method for the discovery of fascinating quantum Hall phases; however, the mechanism of this DNP and in…

Mesoscale and Nanoscale Physics · Physics 2017-04-25 K. F. Yang , K. Nagase , Y. Hirayama , T. D. Mishima , M. B. Santos , H. W. Liu

Dynamic nuclear polarization experiments use microwave irradiation to transfer the larger electron polarization to nuclear spins of interest, and thus enhance the NMR transitions above thermal equilibrium. How the polarization transfer from…

Chemical Physics · Physics 2026-01-12 Gian-Marco Camenisch , Nino Wili , Gunnar Jeschke , Matthias Ernst

We present a technique for manipulating the nuclear spins and the emission polarization from a single optically active quantum dot. When the quantum dot is tunnel coupled to a Fermi sea, we have discovered a natural cycle in which an…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 C. Kloeffel , P. A. Dalgarno , B. Urbaszek , B. D. Gerardot , D. Brunner , P. M. Petroff , D. Loss , R. J. Warburton

A stimulated wave of polarization, which implements a simple mechanism of quantum amplification, is experimentally demonstrated in a chain of four J-coupled nuclear spins, irradiated by a weak radio-frequency transverse field. The "quantum…

Quantum Physics · Physics 2007-05-23 Jae-Seung Lee , Travis Adams , A. K. Khitrin

The spin interaction between an electron and nuclei was investigated optically in a single self-assembled InAlAs quantum dot (QD). In spin dynamics, the correlation time of the coupled electron-nuclear spin system and the electron spin…

Materials Science · Physics 2011-08-29 R. Kaji , H. Sasakura , S. Adachi , S. Muto

We have observed millisecond-long coherent evolution of nuclear spins in a quantum wire at 1.2 K. Local, all-electrical manipulation of nuclear spins is achieved by dynamic nuclear polarization in the breakdown regime of the Integer Quantum…

Mesoscale and Nanoscale Physics · Physics 2009-10-01 A. Corcoles , C. J. B. Ford , M. Pepper , G. A. C. Jones , H. E. Beere , D. A. Ritchie

We model the electron and hole spin dynamics in an undoped double quantum dot structure, considering the carrier tunneling between quantum dots. Taking into account also the presence of an in-plane or tilted magnetic field, we provide the…

Mesoscale and Nanoscale Physics · Physics 2018-01-15 Michał Gawełczyk , Paweł Machnikowski

Dynamic nuclear polarisation, which transfers the spin polarisation of electrons to nuclei, is routinely applied to enhance the sensitivity of nuclear magnetic resonance; it is also critical in spintronics, particularly when spin…

Linearly polarized light tuned slightly below the optical transition of the negatively charged exciton (trion) in a single quantum dot causes the spontaneous nuclear spin polarization (self-polarization) at a level close to 100%. The…

Mesoscale and Nanoscale Physics · Physics 2008-04-02 V. L. Korenev

Resonant laser scattering along with photon correlation measurements have established the atom-like character of quantum dots. Here, we present measurements which challenge this identification for a wide range of experimental parameters:…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 C. Latta , A. Högele , Y. Zhao , A. N. Vamivakas , P. Maletinsky , M. Kroner , J. Dreiser , I. Carusotto , A. Badolato , D. Schuh , W. Wegscheider , M. Atature , A. Imamoglu

Irradiating a semiconductor with circularly polarized light creates spin-polarized charge carriers. If the material contains atoms with non-zero nuclear spin, they interact with the electron spins via the hyperfine coupling. Here, we…

Mesoscale and Nanoscale Physics · Physics 2016-09-09 Raphael W. Mocek , Danil O. Tolmachev , Giovanni Cascio , Dieter Suter
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