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The ferroelectric property of BaTiO$_3$ crystal arises from the strong Pseudo Jahn-Teller (PJT) interactions between the non-degenerate ground electronic state, $^1A_{1g}$ and the degenerate $^1T_{1u}$ symmetry states through the nuclear…

Materials Science · Physics 2025-05-06 Mantu Kumar Sah , Soumya Mukherjee , Satyam Ravi , Satrajit Adhikari

We demonstrate that small but finite ferroelectric polarization ($\sim$0.01 $\mu$C/cm$^2$) emerges in orthorhombic LuFeO$_3$ ($Pnma$) at $T_N$ ($\sim$600 K) because of commensurate (k = 0) and collinear magnetic structure. The synchrotron…

We present a first principles study of the series of multiferroic barium fluorides with the composition BaMF4, where M is Mn, Fe, Co, or Ni. We discuss trends in the structural, electronic, and magnetic properties, and we show that the…

Materials Science · Physics 2009-11-11 Claude Ederer , Nicola A. Spaldin

We use first principles density functional theory calculations to investigate the effect of biaxial strain in the low-temperature structural and ferroelectric properties of [111]-oriented SrTiO$_3$. We find that [111] biaxial strain,…

Materials Science · Physics 2019-03-27 Sebastian E. Reyes-Lillo , Karin M. Rabe , Jeffrey B. Neaton

We present results of local spin density approximation pseudopotential calculations for the ferroelectromagnet, yttrium manganite (YMnO3). The origin of the differences between ferroelectric and non-ferroelectric perovskite manganites is…

Materials Science · Physics 2015-06-25 Alessio Filippetti , Nicola A. Hill

The work carried out first-principles calculations within the framework of density functional theory to study the structural stability of the CsSnI3 compound and the influence of phase transitions on their electronic and optical properties.…

The $\beta$ and $\gamma$ phases of methylammonium chloride CH$_3$NH$_3$Cl and methylammonium bromide CH$_3$NH$_3$Br are identified to be ferroelectric $via$ pyroelectric current and dielectric constant measurements. The magnetic…

Materials Science · Physics 2024-05-17 Chu Xin Peng , Lei Meng , Yi Yang Xu , Tian Tian Xing , Miao Miao Zhao , Peng Ren , Fei Yen

The full potential linearized augmented plane wave (FLAPW) method was used to study the crystal structure and electronic structure properties of PbFe0.5Nb0.5O3 (PFN). The optimized crystal structure, density of states, band structure and…

Materials Science · Physics 2009-11-10 Yuan Xu Wang , C L Wang , M L Zhao , J L Zhang

The antiferrodistortive (AFD) structural transitions of calcium titanate (CaTiO3) at ambient pressure have been extensively studied during the last few years. It is found none of the AFD polymorphs is polar or ferroelectric. However, it was…

Materials Science · Physics 2013-05-30 Yijia Gu , Karin Rabe , Eric Bousquet , Venkatraman Gopalan , Long-Qing Chen

Extensive inelastic neutron scattering measurements of phonons on a single crystal of CaFe2As2 allowed us to establish a fairly complete picture of phonon dispersions in the main symmetry directions. The phonon spectra were also calculated…

We provide a comprehensive theory of magnetic phases in two-dimensional triangulene crystals, using both Hubbard model and density functional theory (DFT) calculations. We consider centrosymmetric and non-centrosymmetric triangulene…

Mesoscale and Nanoscale Physics · Physics 2024-11-01 G. Catarina , J. C. G. Henriques , A. Molina-Sánchez , A. T. Costa , J. Fernández-Rossier

First-principles density-functional calculations reveal a large spin-phonon coupling in cubic SrMnO$_{3}$, with ferromagnetic ordering producing a polar instability. Through combination of this coupling with the strain-polarization coupling…

Materials Science · Physics 2012-09-10 Jun Hee Lee , Karin M. Rabe

We have used a shell model to study the phonon dynamics of multiferroic manganites RMnO3 (R= Tb, Dy, Ho). The calculated phonon dynamical properties, crystal structure, Raman frequencies and specific heat are found to be in good agreement…

Materials Science · Physics 2010-04-06 Renu Choithrani , Mala N. Rao , S. L. Chaplot , N. K. Gaur , R. K. Singh

A second-principles effective interatomic potential is introduced for the prototypical perovskite CaTiO$_3$ (CTO), relying on a Taylor polynomial expansion of the Born-Oppenheimer energy surface around the cubic reference structure, in…

Materials Science · Physics 2025-12-04 Huazhang Zhang , Michael Marcus Schmitt , Louis Bastogne , Xu He , Philippe Ghosez

The temperature-dependent polarization of SrTiO_3 thin films is investigated using confocal scanning optical microscopy. A homogeneous out-of-plane and inhomogeneous in-plane ferroelectric phase are identified from images of the linear…

Materials Science · Physics 2009-11-07 Oleg Tikhomirov , Hua Jiang , Jeremy Levy

Amongst the X(Sn,Pb)Y$_3$ perovskites currently under scrutiny for their photovoltaic applications, the cubic B-$\alpha$ phase of CsSnI$_3$ is arguably the best characterized experimentally. Yet, according to the standard harmonic theory of…

Materials Science · Physics 2015-11-25 Christopher E. Patrick , Karsten W. Jacobsen , Kristian S. Thygesen

We report on a systematic optical investigation of w\"ustite. In addition, the sample under consideration, Fe0.93O, has been characterized in detail by electrical transport, dielectric, magnetic and thermodynamic measurements. From infrared…

Strongly Correlated Electrons · Physics 2015-06-04 F. Schrettle , Ch. Kant , P. Lunkenheimer , F. Mayr , J. Deisenhofer , A. Loidl

Phonon frequencies at {\Gamma},X,M,R-points of Brilloin zone in cubic phase of Ba(Ti,Zr,Hf)O3 were first time calculated by frozen phonon method using density functional theory (DFT) with hybrid exchange correlation functional PBE0. The…

Materials Science · Physics 2010-10-07 Robert A Evaestov

We report a systematic first-principles study based on density functional theory (DFT) of the structural and ferroelectric properties of the $R_2$Ti$_2$O$_{7}$ perovskite-related oxides with $R=$ La, Ce, Pr, and Nd. We show that, in all…

Materials Science · Physics 2021-03-09 Maribel Núñez Valdez , Nicola A. Spaldin

The antipolar $Pbcn$ phase of HfO$_2$ has been suggested to play an important role in the phase transition and polarization switching mechanisms in ferroelectric hafnia. In this study, we perform a comprehensive benchmark of density…

Materials Science · Physics 2025-03-06 Di Fan , Tianyuan Zhu , Shi Liu
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