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We report first-principles calculations of the effects of quasiparticle self-energy and electron-hole interaction on the optical properties of single-walled BN nanotubes. Excitonic effects are shown to be even more important in BN nanotubes…

Materials Science · Physics 2007-08-23 Cheol-Hwan Park , Catalin D. Spataru , Steven G. Louie

The ground state of two-dimensional (2D) electron systems with equal low densities of electrons and holes in nearby layers is an exciton fluid. We show that a reservoir for excitons can be established by contacting the two layers separately…

Mesoscale and Nanoscale Physics · Physics 2018-08-10 Ming Xie , Allan H. MacDonald

Topological band theory has expanded into various domains in applied physics, offering significant potential for future technologies. Recent developments indicate that unique bulk band topology perceived for electrons can be realized in a…

Two-dimensional halide perovskites are among intensely studied materials platforms profiting from solution based growth and chemical flexibility. They feature exceptionally strong interactions among electronic, optical as well as…

Excitons - the particle-hole bound states - composed of localized electron-hole states in semiconducting systems are crucial to explaining the optical spectrum. Spectroscopic measurements can contain signatures of these two particle bound…

Mesoscale and Nanoscale Physics · Physics 2018-06-19 Avinash Rustagi , Alexander F. Kemper

This paper presents a theoretical model intended to address the question of energy transfer in two-dimensional molecular assemblies such as Scheibe aggregates. A new phonon-exciton interaction is introduced to explain the exciton width in J…

Condensed Matter · Physics 2009-09-25 E. A. Bartnik , M. Bednarz

Atomically thin materials such as graphene and monolayer transition metal dichalcogenides (TMDs) exhibit remarkable physical properties resulting from their reduced dimensionality and crystal symmetry. The family of semiconducting…

Time-dependent density functional theory (TDDFT) has been applied to the calculation of absorption spectra for two-dimensional atomic layer materials. We reveal that the character of the first bright exciton state of bi-layer hexagonal…

Materials Science · Physics 2020-01-08 Yasumitsu Suzuki , Kazuyuki Watanabe

Excitons, quasi particles composed of an electron and a hole, play an important role in optical responses in low-dimensional nanostructures. In this work, we have investigated exciton diffusion in a monolayer MoSe2 encapsulated between…

Mesoscale and Nanoscale Physics · Physics 2020-09-30 T. Hotta , S. Higuchi , A. Ueda , K. Shinokita , Y. Miyauchi , K. Matsuda , K. Ueno , T. Taniguchi , K. Watanabe , R. Kitaura

We have carried out electron energy-loss investigations of the lowest singlet excitons in pentacene at 20 K. Our studies allow to determine the full exciton band structure in the a*,b* reciprocal lattice plane. The lowest singlet exciton…

Materials Science · Physics 2012-06-01 Friedrich Roth , Roman Schuster , Andreas König , Martin Knupfer , Helmuth Berger

We develop a microscopic theory of the Coulomb drag effect in a hybrid system consisting of spatially separated two-dimensional quantum gases of degenerate electrons and dipolar excitons. We consider both the normal-phase and condensate…

Mesoscale and Nanoscale Physics · Physics 2019-04-17 M. V. Boev , V. M. Kovalev , I. G. Savenko

Semiconductor excitons are commonly seen as hydrogen atom. This analogy requires a unique hole mass. In reality, this is not so due to the complexity of the semiconductor band structure. The precise consequences on the exciton physics of…

Strongly Correlated Electrons · Physics 2023-02-14 Shiue-Yuan Shiau , Benoit Eble , Monique Combescot

How atoms acquire three-dimensional bulk character is one of the fundamental questions in materials science. Before addressing this question, how atomic layers become a bulk crystal might give a hint to the answer. While atomically thin…

Mesoscale and Nanoscale Physics · Physics 2018-09-28 Ryuta Yagi , Taiki Hirahara , Ryoya Ebisuoka , Tomoaki Nakasuga , Shingo Tajima , Kenji Watanabe , Takashi Taniguchi

Using first-principles GW plus Bethe-Salpeter equation calculations, we identify anomalously strong excitonic effects in several vacancy-ordered double perovskites Cs2MX6 (M = Ti, Zr; X = I, Br). Giant exciton binding energies about 1 eV…

Computational Physics · Physics 2023-06-21 Fan Zhang , Weiwei Gao , Greis J. Cruz , Yi-yang Sun , Peihong Zhang , Jijun Zhao

Monolayer C$_3$N is an emerging two-dimensional indirect band gap semiconductor with interesting mechanical, thermal, and electronic properties. In this work we present a description of C$_3$N electronic and dielectric properties, focusing…

Mesoscale and Nanoscale Physics · Physics 2022-04-26 Miki Bonacci , Matteo Zanfrognini , Elisa Molinari , Alice Ruini , Marilia J. Caldas , Andrea Ferretti , Daniele Varsano

Monolayer phosphorene provides a unique two-dimensional (2D) platform to investigate the fundamental many-body interactions. However, owing to its high instability, unambiguous identification of monolayer phosphorene has been elusive.…

Materials Science · Physics 2014-12-23 Jiong Yang , Renjing Xu , Jiajie Pei , Ye Win Myint , Fan Wang , Zhu Wang , Shuang Zhang , Zongfu Yu , Yuerui Lu

Exciton condensation, the Bose-Einstein-like condensation of quasibosonic particle-hole pairs, has been the subject of much theoretical and experimental interest and holds promise for ultra-energy-efficient technologies. Recent advances in…

Linear carbon-based materials such as polyyne and cumulene oligomers provide a versatile platform for nano-physics and engineering. Direct gap quasi-1D polyyne structures are promising for the observation of strong and unusual excitonic…

Mesoscale and Nanoscale Physics · Physics 2021-01-05 Stella Kutrovskaya , Sevak Demirchyan , Anton Osipov , Stepan Baryshev , Anton Zasedatelev , Pavlos Lagoudakis , Alexey Kavokin

The system under consideration is a multi-component gas of interacting para- and orthoexcitons confined in a three dimensional potential trap. We calculate the spatially resolved optical emission spectrum due to interband transitions…

Quantum Gases · Physics 2010-08-11 S. Sobkowiak , D. Semkat , H. Stolz , Th. Koch , H. Fehske

We consider a neutral exciton localized on a model p-i-n junction defined in a two-dimensional crystal: MoSe$_2$ and phosphorene, using a variational approach to the effective mass Hamiltonian. The non-homogeneous electric field at the…

Mesoscale and Nanoscale Physics · Physics 2022-08-30 B. Szafran