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Methods which aim at universal applicability must be able to describe both weak and strong electronic correlation with equal facility. Such methods are in short supply. The combination of symmetry projection for strong correlation and…

Chemical Physics · Physics 2020-05-14 Yiheng Qiu , Thomas M. Henderson , Jinmo Zhao , Gustavo E. Scuseria

While coupled cluster theory accurately models weakly correlated quantum systems, it often fails in the presence of strong correlations where the standard mean-field picture is qualitatively incorrect. In many cases, these failures can be…

Nuclear Theory · Physics 2020-05-14 Y. Qiu , T. M. Henderson , T. Duguet , G. E. Scuseria

Spin-projected Hartree-Fock is introduced as a particle-hole excitation ansatz over a symmetry-adapted reference determinant. Remarkably, this expansion has an analytic expression that we were able to decipher. While the form of the…

Strongly Correlated Electrons · Physics 2016-11-08 Yiheng Qiu , Thomas M. Henderson , Gustavo E. Scuseria

Coupled cluster and symmetry projected Hartree-Fock are two central paradigms in electronic structure theory. However, they are very different. Single reference coupled cluster is highly successful for treating weakly correlated systems,…

We study the structure of the number projected BCS (PBCS) wave function in the particle-hole basis, displaying its similarities with coupled clusters theory (CCT). The analysis of PBCS together with several modifications suggested by the…

Nuclear Theory · Physics 2016-06-15 J. Dukelsky , S. Pittel , C. Esebbag

We present an extension of the pair coupled cluster doubles (p-CCD) method to quasiparticles and apply it to the attractive pairing Hamiltonian. Near the transition point where number symmetry gets spontaneously broken, the proposed…

The past several years have seen renewed interest in the use of symmetry-projected Hartree-Fock for the description of strong correlations. Unfortunately, these symmetry-projected mean-field methods do not adequately account for dynamic…

Chemical Physics · Physics 2017-08-22 Thomas M. Henderson , Gustavo E. Scuseria

Coupled cluster theory is the method of choice for weakly correlated systems. But in the strongly correlated regime, it faces a symmetry dilemma, where it either completely fails to describe the system, or has to artificially break certain…

Chemical Physics · Physics 2020-05-14 Yiheng Qiu , Thomas M. Henderson , Jinmo Zhao , Gustavo E. Scuseria

We extend previous studies of the BCS canonical approach for the attractive Hubbard model. A derivation of the BCS formulation is presented for both the Hubbard and a simpler reduced Hamiltonian. Using direct diagonalization, exact one and…

Superconductivity · Physics 2009-11-10 Nathan Salwen , Steven A. Sheets , Stephen R. Cotanch

We present an implementation of a perturbative triples correction for the coupled cluster ansatz including single and double excitations based on the transcorrelated Hamiltonian. Transcorrelation introduces explicit electron correlation in…

Chemical Physics · Physics 2025-02-19 Maximilian Mörchen , Alberto Baiardi , Michał Lesiuk , Markus Reiher

The BCS and/or HFB theories are extended by treating the effect of four quasi-particle states perturbatively. The approach is tested on the pairing hamiltonian, showing that it combines the advantage of standard perturbation theory valid at…

Nuclear Theory · Physics 2015-06-05 Denis Lacroix , Danilo Gambacurta

Alpha($^{4}$He)-cluster models have often been used to describe light nuclei. Towards the application to multi-cluster systems involving heavy clusters, we study the relative wave functions of the $\alpha+^{16}$O and $\alpha+^{40}$Ca…

Nuclear Theory · Physics 2018-08-01 T. Arai , W. Horiuchi , D. Baye

Transcorrelated coupled cluster and distinguishable cluster methods are presented. The Hamiltonian is similarity transformed with a Jastrow factor in the first quantisation, which results in up to three-body integrals. The coupled cluster…

Chemical Physics · Physics 2021-12-22 Thomas Schraivogel , Aron J. Cohen , Ali Alavi , Daniel Kats

In this work we present a coupled-cluster theory for the propagation of multireference electronic systems initiating at general quantum mechanical states. Our formalism is based on the infinitesimal analysis of modified cluster operators,…

Chemical Physics · Physics 2025-05-09 Martín A. Mosquera

The ground state pairing correlations in finite fermionic systems are described with a high degree of accuracy within a variational approach based on a combined coupled-cluster and particle-number-projected BCS ansatz. The flexibility of…

Nuclear Theory · Physics 2021-06-02 V. V. Baran , J. Dukelsky

An effective bosonic Hamiltonian of $1s$ excitons with ``spin'' degrees of freedom in two dimension is obtained through a projection procedure, starting from a conventional electron-hole Hamiltonian ${\cal H}_{eh}$. We first demonstrate…

Materials Science · Physics 2009-10-31 Jun-ichi Inoue , Tobias Brandes , Akira Shimizu

We consider a new formulation of the stochastic coupled cluster method in terms of the similarity transformed Hamiltonian. We show that improvement in the granularity with which the wavefunction is represented results in a reduction in the…

Chemical Physics · Physics 2016-02-02 Ruth S. T. Franklin , James S. Spencer , Alberto Zoccante , Alex J. W. Thom

We develop a coupled-cluster theory for bosonic mixtures of binary species in external traps, providing a promising theoretical approach to demonstrate highly accurately the many-body physics of mixtures of Bose-Einstein condensates. The…

Quantum Gases · Physics 2024-02-01 Anal Bhowmik , Ofir E. Alon

It is well-known that polynomial reproduction is not possible when approximating with Gaussian kernels. Quasi-interpolation schemes have been developed which use a finite number of Gaussians at different scales, which then reproduce…

Numerical Analysis · Mathematics 2020-01-24 Simon Hubbert , Jeremy Levesley

A BCS model characterized by a phenomenological pair potential with on-site ($V_0$), nearest ($V_1$), and next nearest ($V_2$) neighbour coupling constants, and an empirical quasiparticle dispersion taken from angle-resolved photoemission…

Condensed Matter · Physics 2009-10-22 R. Fehrenbacher , M. R. Norman
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