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The present work reports on the generation of short-pulse coherent extreme ultraviolet radiation of controlled polarization. The proposed strategy is based on high-order harmonics generated in pre-aligned molecules. Field-free molecular…

An extreme ultraviolet (EUV) single attosecond pulse passing through a laser-dressed dense gas is studied theoretically. The weak EUV pulse pumps the helium gas from the ground state to the 2s2p(1P) autoionizing state, which is coupled to…

Atomic Physics · Physics 2013-01-18 Wei-Chun Chu , C. D. Lin

We investigate two-photon double ionization of helium by intense ($10^{15} W/cm^2$) ultrashort ($\approx 300$ as) soft X-ray pulses (E = 91.6 eV). The time-dependent two-electron Schr\"odinger equation is solved using a coupled channel…

Atomic Physics · Physics 2007-05-23 I. F. Barna , J. Wang , J. Burgdoerfer

We present theoretical studies on real-time probing the electron density evolution of an atom in a strong infrared (IR) laser field with few-cycle near-infrared (NIR) and attosecond extreme-ultraviolet (XUV) pulses. Our results indicate…

Atomic Physics · Physics 2015-06-04 Yunpei Deng , Xinhua Xie

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight

Non-equilibrium processes following the irradiation of atomic clusters with short pulses of vacuum ultraviolet radiation are modelled using kinetic Boltzmann equations. The dependence of the ionization dynamics on the cluster size is…

Plasma Physics · Physics 2009-11-13 B. Ziaja , H. Wabnitz , E. Weckert , T. Möller

Photoelectron angular distributions (PADs) obtained from ionization of potassium atoms using moderately intense femtosecond IR fields ($\sim$10$^{12}$Wcm$^{-2}$) of various polarization states are shown to provide a route to "complete"…

Atomic Physics · Physics 2015-01-15 Paul Hockett , Matthias Wollenhaupt , Christian Lux , Thomas Baumert

Ionization of an atom or molecule by a strong laser field produces sub-optical cycle wave packets whose control has given rise to attosecond science. The final states of the wave packets depend on ionization and deflection by the laser…

We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…

Atomic Physics · Physics 2009-11-10 C. Figueira de Morisson Faria , X. Liu , A. Sanpera , M. Lewenstein

The model is constructed of the propagation of gamma-ray burst radiation through a dense molecular cloud. The main processes of the interaction of the radiation with the interstellar gas are taken into account in the simulations: the…

High Energy Astrophysical Phenomena · Physics 2024-05-20 Aleksandr Nesterenok

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

An ab initio simulation of strong-field photodissociation of diatomic molecules was developed, inspired by recent dissociation experiments of F2-. The transition between electronic states was modeled, including the laser pulse and…

Atomic Physics · Physics 2020-06-26 Bar Ezra , Shimshon Kallush , Ronnie Kosloff

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

The development of ultra-short intense laser sources in the visible and extreme ultraviolet (XUV) spectral range led to fascinating studies in laser-matter interactions and attosecond science. In the majority of these studies the system…

We investigate the absorption line shapes of laser-dressed atoms beyond the single-atom response, by using extreme ultraviolet (XUV) attosecond pulse trains to probe an optically thick helium target under the influence of a strong infrared…

Atomic Physics · Physics 2015-06-24 Chen-Ting Liao , Arvinder Sandhu , Seth Camp , Kenneth J. Schafer , Mette B. Gaarde

We investigate laser-induced nonsequential double ionization from aligned diatomic molecules, using the strong-field approximation in its length and velocity gauge formulations. Throughout, we consider that the first electron dislodges the…

Atomic Physics · Physics 2008-12-10 C. Figueira de Morisson Faria

We study the temporal aspects of laser-assisted extreme ultraviolet (XUV) photoionization using attosecond pulses of harmonic radiation. The aim of this paper is to establish the general form of the phase of the relevant transition…

We present experimental results for the ionization of aniline and benzene molecules subjected to intense ultrashort laser pulses. Measured parent molecular ions yields were obtained using a recently developed technique capable of…

The interaction of short laser pulses with small rare gas clusters is investigated by using a microscopic, semi-classical model with an explicit treatment of the inner-atomic dynamics. Field and collisional ionisation as well as…

Atomic and Molecular Clusters · Physics 2007-05-23 D. Bauer