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Employing density functional theory calculations we explore initial stage of competitive alloying of co-deposited silver and indium atoms into a silicon surface. Particularly, we identify respective adsorption positions and activation…

Materials Science · Physics 2023-02-17 D. V. Prodan , G. V. Paradezhenko , D. Yudin , A. A. Pervishko

Theoretical and experimental investigation of the electronic and magnetic structure of transition metal atoms on an insulating interface with a metallic substrate at low temperatures is quite challenging. In this paper, we show a density…

The radiative torque (RAT) alignment of interstellar grains with ordinary paramagnetic susceptibilities has been supported by earlier studies. The alignment of such grains depends on the so-called RAT parameter $q^{\max}$ that is determined…

Astrophysics of Galaxies · Physics 2016-11-15 Thiem Hoang , A. Lazarian

The nuclear time-dependent density functional theory (TDDFT) is a tool of choice for describing various dynamical phenomena in atomic nuclei. In a recent study, we reported an extension of the framework - the multiconfigurational TDDFT…

Nuclear Theory · Physics 2024-01-24 Petar Marević , David Regnier , Denis Lacroix

We employ dispersion-corrected density-functional theory to study the adsorption of tetrapyrrole 2H-porphine (2H-P) at Cu(111) and Ag(111). Various contributions to adsorbate-substrate and adsorbate-adsorbate interactions are systematically…

Chemical Physics · Physics 2016-09-05 Moritz Müller , Katharina Diller , Reinhard J. Maurer , Karsten Reuter

We calculate the efficiency of iron K line emission and iron K absorption in photoionized models using a new set of atomic data. These data are more comprehensive than those previously applied to the modeling of iron K lines from…

Astrophysics · Physics 2009-11-10 T. R. Kallman , P. Palmeri , M. A. Bautista , C. Mendoza , J. H. Krolik

A stochastic approach to time-dependent density functional theory (TDDFT) is developed for computing the absorption cross section and the random phase approximation (RPA) correlation energy. The core idea of the approach involves…

Chemical Physics · Physics 2016-11-04 Yi Gao , Daniel Neuhauser , Roi Baer , Eran Rabani

While first-principles calculations of electrode-molecule binding play an indispensable role in obtaining atomic-level understanding in surface science and electrochemistry, a significant challenge remains because the adsorption energy is…

Materials Science · Physics 2024-03-29 Juho Lee , Hyeonwoo Yeo , Ryong-Gyu Lee , Yong-Hoon Kim

Line defects and scattering amplitudes have proven to be fruitful objects of study in the context of holographic dualities. They serve as valuable theoretical laboratories for the development of non-perturbative methods and have provided…

High Energy Physics - Theory · Physics 2025-09-18 Martín Lagares

We demonstrate that ground state energies approaching chemical accuracy can be obtained by combining the adiabatic connection fluctuation-dissipation theorem (ACFDT) with time-dependent density functional theory (TDDFT). The key ingredient…

Materials Science · Physics 2014-05-29 Thomas Olsen , Kristian S. Thygesen

In this paper, we evaluate of the adsorption/ desorption of ammonia molecules on a graphene surface by studying the Fermi level shift. Based on a physically plausible model, the adsorption and desorption rates of ammonia molecules on…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Shanshan Chen , Weiwei Cai , David Chen , Yujie Ren , Xuesong Li , Yanwu Zhu , Rodney S. Ruoff

We have combined scanning tunneling microscopy with inelastic electron tunneling spectroscopy (IETS) and density functional theory (DFT) to study a tetracyanoethylene monolayer on Ag(100). Images show that the molecules arrange in locally…

Materials Science · Physics 2013-07-01 Daniel Wegner , Ryan Yamachika , Xiaowei Zhang , Yayu Wang , Michael F. Crommie , Nicolás Lorente

We study a $d=2$ discrete solid--on--solid model of complete wetting of a rough substrate with random self--affine boundary, having roughness exponent $\zeta_s$. A suitable transfer matrix approach allows to discuss adsorption isotherms, as…

Condensed Matter · Physics 2009-10-22 G. Giugliarelli , A. L. Stella

Theory of adsorption on a surface with nanolocal defects is proposed. Two efficacy parameters of surface modification for nanotechnological purposes are introduced, where the modification is a creation of nanolocal artificial defects. The…

Chemical Physics · Physics 2009-10-31 Yu. E. Lozovik , A. M. Popov

Fermi edge adsorption singularities (FES) are studied using a combination of conformal field theory (CFT), an exact sum rule and numerical work on a tight binding model which is shown to exhibit remarkable simplifying features. The…

Condensed Matter · Physics 2009-10-30 Alexandre M. Zagoskin , Ian Affleck

Grain boundaries play a critical role in applications of superconducting Nb$_3$Sn: in dc applications, grain boundaries preserve the material's inherently high critical current density by pinning flux, while in ac applications grain…

Materials Science · Physics 2020-11-12 Michelle M. Kelley , Nathan S. Sitaraman , Tomás A. Arias

We analyze, with Density Functional Theory (DFT) calculations, the adsorption energies of Li$_2$O$_2$, Na$_2$O$_2$ and NaO$_2$ on clean and oxygen passivated TiC (111) surfaces. We show, that after deposition of two molecular layers of…

Chemical Physics · Physics 2018-09-10 Keren Raz , Polina Tereshchuk , Diana Golodnitsky , Amir Natan

We report a first-principles calculation that models the effect of iron (Fe) atoms on the adsorption of a tungsten (W) atom on W(100) surfaces. The adsorption of a W atom on a clean W(100) surface is compared with that of a W atom on a…

Materials Science · Physics 2009-11-13 J. Houze , Sungho Kim , Seong-Jin Park , Randall M. German , M. F. Horstemeyer , Seong-Gon Kim

Machine learning thermodynamic perturbation theory (MLPT) is a promising approach to compute finite temperature properties when the goal is to compare several different levels of ab initio theory and/or to apply highly expensive…

We investigate the atomic hydrogen adsorption on Mg(0001) by using density-functional theory within the generalized gradient approximation and a supercell approach. The coverage dependence of the adsorption structures and energetics is…

Materials Science · Physics 2009-04-29 Yanfang Li , Ping Zhang , Bo Sun , Yu Yang , Yinghui Wei