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Dy2Ti2O7 is a geometrically frustrated magnetic material with a strongly correlated spin ice regime that extends from 1 K down to as low as 60 mK. The diffuse elastic neutron scattering intensities in the spin ice regime can be remarkably…

Statistical Mechanics · Physics 2008-08-02 Taras Yavors'kii , Tom Fennell , Michel J. P. Gingras , Steven T. Bramwell

Recently it has been suggested that long range magnetic dipolar interactions are responsible for spin ice behavior in the Ising pyrochlore magnets ${\rm Dy_{2}Ti_{2}O_{7}}$ and ${\rm Ho_{2}Ti_{2}O_{7}}$. We report here numerical results on…

Disordered Systems and Neural Networks · Physics 2009-10-31 Roger G. Melko , Byron C. den Hertog , Michel J. P. Gingras

We report a study of the low temperature bulk magnetic properties of the spin ice compound Dy2Ti2O7 with particular attention to the (T < 4 K) spin freezing transition. While this transition is superficially similar to that in a spin glass,…

Materials Science · Physics 2007-05-23 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , P. Schiffer

We have probed the low temperature magnetic behavior of the ordered spin ice material Tb2Sn2O7 through ac magnetic susceptibility measurements of both the pure material and samples with small percentages of Ti substituted on the Sn…

Strongly Correlated Electrons · Physics 2012-11-27 M. L. Dahlberg , M. J. Matthews , P. Jiramongkolchai , R. J. Cava , P. Schiffer

Among the frustrated magnetic materials, spin-ice stands out as a particularly interesting system. Residual entropy, freezing and glassiness, Kasteleyn transitions and fractionalisation of excitations in three dimensions all stem from a…

The description and detection of unconventional magnetic states such as spin liquids is a recurring topic in condensed matter physics. While much of the efforts have traditionally been directed at geometrically frustrated antiferromagnets,…

Strongly Correlated Electrons · Physics 2018-05-25 L. Bovo , M. Twengström , O. A. Petrenko , T. Fennell , M. J. P. Gingras , S. T. Bramwell , P. Henelius

The thermal equilibrium properties of the spin-ice material DTO, including specific heat, magnetization, and spin correlations, could be successfully reproduced by a model featuring magnetic interactions up to the third nearest neighbor and…

Strongly Correlated Electrons · Physics 2025-04-14 Mariano Marziali Bermudez , R. A. Borzi , D. A. Tennant , S. A. Grigera

The spin ice system Dy$_{2}$Ti$_{2}$O$_{7}$ exhibits strong frequency-dependent spin-freezing at $\sim$ 16 K temperature. Although it has been a matter of discussion for years, the origin of this unusual spin freezing is still unknown. The…

Strongly Correlated Electrons · Physics 2022-04-06 Sheetal , C. S. Yadav

We report the a.c. susceptibility study of Dy_xTb_{2-x}Ti_2O_7 with x in [0, 2]. In addition to the single-ion effect at Ts (single-ion effect peak temperature) corresponding to the Dy3+ spins as that in spin ice Dy_2Ti_2O_7 and a possible…

Materials Science · Physics 2015-03-13 Hui Xing , Mi He , Chunmu Feng , Hanjie Guo , Hao Zeng , Zhu-An Xu

We have studied the field-dependent ac magnetic susceptibility of single crystals of Dy2Ti2O7 spin ice along the [111] direction in the temperature range 1.8 K - 7 K. Our data reflect the onset of local spin ice order in the appearance of…

Strongly Correlated Electrons · Physics 2015-06-12 M. J. Matthews , C. Castelnovo , R. Moessner , S. A. Grigera , D. Prabhakaran , P. Schiffer

If magnetic frustration is most commonly known for undermining long-range order, as famously illustrated by spin liquids, the ability of matter to develop new collective mechanisms in order to fight frustration is no less fascinating,…

Strongly Correlated Electrons · Physics 2015-12-31 L. D. C. Jaubert , Owen Benton , Jeffrey G. Rau , J. Oitmaa , R. R. P. Singh , Nic Shannon , Michel J. P. Gingras

The magnetically frustrated spin ice family of materials is host to numerous exotic phenomena such as magnetic monopole excitations and macroscopic residual entropy extending to low temperature. A finite-temperature ordering transition in…

We report on the low-energy dynamics in the kagome antiferromagnet CaCu$_3$(OD)$_6$Cl$_2\cdot0.6$D$_2$O (Ca-kapellasite) as studied by use of $^2$D-NMR measurements. Previous $^{35}$Cl-NMR measurements revealed that the nuclear spin-lattice…

A frustrated system is one whose symmetry precludes the possibility that every pairwise interaction (``bond'') in the system can be satisfied at the same time. Such systems are common in all areas of physical and biological science. In the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Steven T. Bramwell , Michel J. -P. Gingras

Out-of-equilibrium investigation of strongly correlated materials deciphers the hidden equilibrium properties. Herein, we have investigated the out-of-equilibrium magnetic properties of polycrystalline Dy2Ti2O7 and Ho2Ti2O7 spin ices. The…

Strongly Correlated Electrons · Physics 2023-01-20 Pramod K. Yadav , Rajnikant Upadhyay , Rahul Kumar , Pavan Nukala , Chandan Upadhyay

Specific heat measurements were carried out on the closely related spin-chain oxides Ca3Co2O6 and Ca3CoRhO6. Both compounds consist of Ising magnetic chains that are arranged on a triangular lattice. The spin coupling along and between the…

Strongly Correlated Electrons · Physics 2009-11-10 V. Hardy , M. R. Lees , A. Maignan , S. Hebert , D. Flahaut , C. Martin , D. McK. Paul

Magnetic frustration and low dimensionality can prevent long range magnetic order and lead to exotic correlated ground states. SrDy$_2$O$_4$ consists of magnetic Dy$^{3+}$ ions forming magnetically frustrated zig-zag chains along the c-axis…

The Tb$_2$Ti$_2$O$_7$ pyrochlore magnetic material is attracting much attention for its {\em spin liquid} state, failing to develop long range order down to 50 mK despite a Curie-Weiss temperature $\theta_{\rm CW} \sim -14$ K. In this paper…

Statistical Mechanics · Physics 2007-05-23 Hamid R. Molavian , Michel J. P. Gingras , Benjamin Canals

We investigate the non-equilibrium behavior of the spin-ice material Dy$_2$Ti$_2$O$_7$ by studying its magnetization as a function of the rate at which an external field is swept. At temperatures below the enigmatic "freezing" temperature…

Materials Science · Physics 2011-01-13 D. Slobinsky , C. Castelnovo , R. A. Borzi , A. S. Gibbs , A. P. Mackenzie , R. Moessner , S. A. Grigera

Analysis of neutron diffraction, dc magnetization, ac magnetic susceptibility, heat capacity, and electrical resistivity for DyRuAsO in an applied magnetic field are presented at temperatures near and below those at which the structural…

Strongly Correlated Electrons · Physics 2015-06-22 Michael A. McGuire , V. Ovidiu Garlea , Andrew F. May , Brian C. Sales
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