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We present a study of the possibility to significantly enhance the efficiency of high-order harmonic generation (HHG) using few-cycle optical waveforms obtained by superposing two laser pulses of different color delayed optimally relative…

Optics · Physics 2024-12-11 O. V. Meshkov , M. Yu. Emelin , M. Yu. Ryabikin

The combination of high-order harmonic generation (HHG) with resonant XUV excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process is investigated theoretically. In this setup, the…

Atomic Physics · Physics 2023-01-10 Christian Buth , Markus C. Kohler , Joachim Ullrich , Christoph H. Keitel

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

High-order harmonic generation (HHG) is combined with resonant x-ray excitation of a core electron into the transient valence vacancy that is created in the course of the HHG process. To describe this setting, I develop a…

Atomic Physics · Physics 2015-10-15 Christian Buth

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2007-05-23 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel

High harmonic generation (HHG) is a manifestation of the strongly nonlinear response of matter to intense laser fields and has, as the basis for coherent XUV sources a variety of applications. Recently, HHG from atoms in a phase and…

Optics · Physics 2020-05-20 Jonas Wätzel , Jamal Berakdar

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

The generation of high harmonics (HHG) in atomic systems by the highly non-linear response to an intense laser field is a prominent pathway to the synthesis of ever shorter laser pulses at increasingly higher photon energies. Extensions of…

Atomic Physics · Physics 2022-11-23 Mohammad Monfared , Elnaz Irani , Christoph Lemell , Joachim Burgdörfer

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

Theoretical approaches to strong field phenomena driven by plasmonic fields are based on the length gauge formulation of the laser-matter coupling. From the theoretical viewpoint it is known there exists no preferable gauge and consequently…

Atomic Physics · Physics 2015-12-30 A. Chacón , M. Lewenstein , M. F. Ciappina

High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…

We theoretically investigate correlated electron dynamics in high-harmonic generation (HHG), using all-electron \emph{ab initio} simulations for three-dimensional real alkali-metal atoms. The resulting harmonic spectra exhibit a plateau…

Atomic Physics · Physics 2019-04-10 Yang Li , Takeshi Sato , Kenichi L. Ishikawa

A theoretical model is developed describing high-order harmonic generation (HHG) from a gas of multiply-charged ions driven by a laser field of relativistic intensity. Macroscopic propagation of harmonics is investigated in a relativistic…

Atomic Physics · Physics 2012-02-21 Markus C. Kohler , Karen Z. Hatsagortsyan

We report measurements and theoretical simulations of high-order harmonic generation (HHG) in aligned N$_2$ molecules using a 1200-nm intense laser field when the generating pulse is perpendicular to the aligning one. With increasing laser…

When a high power laser beam irradiates a small aperture on a solid foil target, the strong laser field drives surface plasma oscillation at the periphery of this aperture, which acts as a "relativistic oscillating window". The diffracted…

Plasma Physics · Physics 2021-04-07 Longqing Yi

High-order harmonic generation is investigated for H$_2^+$ and D$_2^+$ with and without Born-Oppenheimer approximation by numerical solution of full dimensional electronic time-dependent Schr\"{o}dinger equation under 4-cycle intense laser…

Atomic Physics · Physics 2014-10-22 Hamed Ahmadi , Ali Maghari , Hassan Sabzyan , Ali Reza Niknam , Mohsen Vafaee

High harmonic generation (HHG) in solids could enable attosecond and ultraviolet light sources with high compactness, great controllability and rich functions. However, the HHG process is accompanied by a quite large wavevector mismatch…

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…