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Diamond properties down to the quantum-size region are still poorly understood. High-pressure high-temperature (HPHT) synthesis from chloroadamantane molecules allows precise control of nanodiamond size. Thermal stability and optical…

Materials Science · Physics 2022-02-23 E. A. Ekimov , A. A. Shiryaev , Yu. Grigoriev , A. Averin , E. Shagieva , S. Stehlik , M. V. Kondrin

The combination of nanodiamonds with plasmonic metal particles is being explored for synergic effects that can enhance biosensing and antibacterial treatments, energy harvesting, photocatalysis, and quantum centres. Here we systematically…

Understanding the dynamics of molecules adsorbed to surfaces or confined to small volumes is a matter of increasing scientific and technological importance. Here, we demonstrate a pulse protocol using individual paramagnetic nitrogen…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 T. Staudacher , N. Raatz , S. Pezzagna , J. Meijer , F. Reinhard , C. A. Meriles , J. Wrachtrup

The sensitivity of magnetic and electric field sensors based on nitrogen-vacancy (NV) center in diamond strongly depends on the available concentration of NV and their coherence properties. Achieving high coherence times simultaneously with…

The integration of NMR and high pressure technique brings unique opportunities to study electronic, structural and dynamical properties under extreme conditions. Despite a great degree of success has been achieved using coil-based schemes,…

Quantum Physics · Physics 2022-03-22 Yan-Xing Shang , Fang Hong , Jian-Hong Dai , Ya-Nan Lu , Hui Yu , Yong-Hong Yu , Xiao-Hui Yu , Xin-Yu Pan , Gang-Qin Liu

Nanodiamonds have emerged as promising materials for quantum computing, biolabeling, and sensing due to their ability to host color centers with remarkable photostability and long spin-coherence times at room temperature. Recently, a…

The evolution of the polycrystalline pattern of electron paramagnetic resonance (EPR) spectra of intrinsic and induced paramagnetic centers in an ensemble of submicrometer diamond particles on diminishing average particle size is…

Mesoscale and Nanoscale Physics · Physics 2019-12-24 G. G. Zegrya , D. M. Samosvat , V. Yu. Osipov , A. Ya. Vul' , A. I. Shames

Nanodiamonds containing negatively charged nitrogen vacancy centres (${\text{NV}}^{-}$) have applications as localized sensors in biological material and have been proposed as a platform to probe the macroscopic limits of spatial…

The negatively charged nitrogen-vacancy centre (NV$^-$) in diamond has been utilized in a wide variety of sensing applications. The centre's long spin coherence and relaxation times ($T_2^*$, $T_2$ and $T_1$) at room temperature are crucial…

The widespread use of nanodiamond as a biomedical platform for drug-delivery, imaging, and sub-cellular tracking applications stems from their non-toxicity and unique quantum mechanical properties. Here, we extend this functionality to the…

Mesoscale and Nanoscale Physics · Physics 2016-06-23 Ewa Rej , Torsten Gaebel , David E. J. Waddington , David J. Reilly

Single NV centers in HPHT IIa diamond are fabricated by helium implantation through lithographic masks. The concentrations of created NV centers in different growth sectors of HPHT are compared quantitatively. It is shown that the purest…

Substitutional nitrogen atoms in a diamond crystal (P1 centers) are, on one hand, a resource for creation of nitrogen-vacancy (NV) centers, that have been widely employed as nanoscale quantum sensors. On the other hand, P1's electron spin…

Coherence times of spin qubits in solid-state platforms are often limited by the presence of a spin bath. While some properties of these typically dark bath spins can be indirectly characterized via the central qubit, it is important to…

Quantum Physics · Physics 2025-02-12 Ethan Q. Williams , Chandrasekhar Ramanathan

Nanodiamonds (NDs) hosting optically active defects are an important technical material for applications in quantum sensing, biological imaging, and quantum optics. The negatively charged silicon vacancy (SiV) defect is known to fluoresce…

In diamond, nitrogen defects like the substitutional nitrogen defect (Ns) or the nitrogen-vacancy-hydrogen complex (NVH) outnumber the nitrogen vacancy (NV) defect by at least one order of magnitude creating a dense spin bath. While neutral…

Hydrothermal synthesis offers an economical and scalable way to produce nanodiamonds under relatively mild, low-pressure and low-temperature conditions. However,its sustainability and the detailed mechanisms behind diamond formation in such…

By efficient nanoscale plasma etching, the nitrogen-vacancy (NV) centers in diamond were brought to the sample surface step by step successfully. At each depth, we used the relative ratios of spin coherence times before and after applying…

Mesoscale and Nanoscale Physics · Physics 2018-01-03 Wenlong Zhang , Jian Zhang , Junfeng Wang , Fupan Feng , Shengran Lin , Liren Lou , Wei Zhu , Guanzhong Wang

Optically-detected paramagnetic centers in wide-bandgap semiconductors are emerging as a promising platform for nanoscale metrology at room temperature. Of particular interest are applications where the center is used as a probe to…

Mesoscale and Nanoscale Physics · Physics 2015-12-09 Abdelghani Laraoui , Daniela Pagliero , Carlos A. Meriles

Diamond has been extensively investigated recently due to a wide range of potential applications of nitrogen-vacancy (NV) defect centers existing in a diamond lattice. The applications include magnetometry and quantum information…

Mesoscale and Nanoscale Physics · Physics 2016-03-25 Viktor Stepanov , Susumu Takahashi

Understanding the profile of a qubit's wavefunction is key to its quantum applications. Unlike conducting systems, where a scanning tunneling microscope can be used to probe the electron distribution, there is no direct method for…

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