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Related papers: Time Delay in Molecular Photoionization

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We theoretically study time-resolved photoemission in atoms as probed by attosecond streaking. We review recent advances in the study of the photoelectric effect in the time domain and show that the experimentally accessible time shifts can…

Atomic Physics · Physics 2015-03-06 Stefan Nagele , Renate Pazourek , Michael Wais , Georg Wachter , Joachim Burgdörfer

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

Due to the absorption of high energetic ultraviolet (UV) photons by the surface layers of the cold molecular clouds, only low energetic photons are able to penetrate into the inner regions of these clouds. This leads to lower…

We suggest an explanation of the recently observed discrepancy between the experimental and theoretical results on ionization of atoms, encapsulated into the fullerenes by photons with the energies of about 80-190eV. On the ground of…

Atomic Physics · Physics 2015-06-19 M. Ya. Amusia , L. V. Chernysheva , E. G. Drukarev

The Wigner time delay is a measure of the time spent by a particle inside the scattering region of an open system. For chaotic systems, the statistics of the individual delay times (whose average is the Wigner time delay) are thought to be…

Chaotic Dynamics · Physics 2013-03-06 Gregory Berkolaiko , Jack Kuipers

Photoionization of matter is one of the fastest electronic processes in nature. Experimental measurements of photoionization dynamics have become possible through attosecond metrology. However, all experiments reported to date contain a…

Quantum Physics · Physics 2025-02-11 Meng Han , Jia-Bao Ji , Leung Chung Sum , Kiyoshi Ueda , Hans Jakob Wörner

We study the elastic scattering of slow electrons by two-atomic molecule in the frame of non-overlapping atomic potentials model. The molecular continuum wave function is represented as a combination of a plane wave and two spherical…

Chemical Physics · Physics 2021-02-03 M. Ya. Amusia , A. S. Baltenkov

In the semiclassical picture of photoionization process in intense laser fields, the ionization rate solely depends on the amplitude of the electric field and the final photoelectron momentum corresponds to the instant of ionization of the…

Atomic Physics · Physics 2019-05-09 Li Guo , Shilin Hu , Mingqing Liu , Zheng Shu , Xiwang Liu , Jie Li , Weifeng Yang , Ronghua Lu , Shensheng Han , Jing Chen

The interaction of strong laser fields with matter intrinsically provides powerful tools to image transient dynamics with an extremely high spatiotemporal resolution. Here, we study strong-field ionisation of laser-aligned molecules and…

We determine and analyze the quantum phases and time delays in photoionization and photorecombination of valence 3p and 3s electrons of argon using the Kohn-Sham local density functional approach. The time-dependent local density…

Recent attoclock experiments using the attsecond angular streaking technique enabled the measurement of the tunneling time delay during laser induced strong field ionization. Theoretically the tunneling time delay is commonly modelled by…

Quantum Physics · Physics 2015-05-19 Enderalp Yakaboylu , Michael Klaiber , Karen Z. Hatsagortsyan

In this Letter, we investigate the non-dipole effects in time delay of photoelectrons emitted by multi-electron atoms, negative ions, and respective endohedrals. We present the necessary general formulas in the frame of the random phase…

Atomic Physics · Physics 2020-12-02 M. Ya. Amusia , L. V. Chernysheva

Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets , I. A. Ivanov , Igor. Bray

The photon-ion merged-beams technique for the photoionization of mass/charge selected ionized atoms, molecules and clusters by x-rays from synchrotron radiation sources is introduced. Examples for photoionization of atomic ions are…

Atomic Physics · Physics 2017-02-22 S. Schippers , A. L. D. Kilcoyne , R. A. Phaneuf , A. Müller

We study time-delays in atomic multiphoton ionization (MPI) using the phase-sensitive detection of photoelectron vortices. Photoelectron vortices are created by MPI with counter-rotating circularly polarized (CRCP) ultrashort double pulse…

Atomic Physics · Physics 2025-01-13 D. Köhnke , T. Bayer , M. Wollenhaupt

We present temporal intensity correlation measurements of light scattered by a hot atomic vapor. Clear evidence of photon bunching is shown at very short time-scales (nanoseconds) imposed by the Doppler broadening of the hot vapor.…

Atomic Physics · Physics 2016-06-01 A. Dussaux , T. Passerat de Silans , W. Guerin , O. Alibart , S. Tanzilli , F. Vakili , R. Kaiser

Photoionization is a key step in many attosecond processes. Accurately determining the photoionization time delay is critical to understanding electron dynamics during and after ionization and can guide future efforts to manipulate electron…

Atomic Physics · Physics 2026-02-26 J. Aygun , D. Yaacoub , A. L. Harris

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker

We have observed the signatures of valence electron rearrangement in photoexcited ammonia using ultrafast hard X-ray scattering. Time-resolved X-ray scattering is a powerful tool for imaging structural dynamics in molecules because of the…

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