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We demonstrate a method of magnetic resonance imaging with single nuclear-spin sensitivity under ambient conditions. It employs a network of isolated electronic-spin quantum bits (qubits) that act as quantum reporters on the surface of high…

Magnetic resonance imaging, based on the manipulation and detection of nuclear spins, is a powerful imaging technique that typically operates on the scale of millimeters to microns. Using magnetic resonance force microscopy, we have…

Other Condensed Matter · Physics 2007-06-27 H. J. Mamin , M. Poggio , C. L. Degen , D. Rugar

Solid state defects such as nitrogen vacancy (NV) centers in diamond have been utilized for NMR sensing at ambient temperatures for samples at the nano-scale and up to the micro-scale. Similar to standard NMR, NV-sensitivities can be…

Quantum Physics · Physics 2026-01-28 Oliver T. Whaites , Jaime García Oliván , Jorge Casanova

Hybrid photoelectric detection of NV magnetic resonances (PDMR) is anticipated to lead to scalable quantum chip technology. To achieve this goal, it is crucial to prove that PDMR readout is compatible with the coherent spin control. Here we…

Sensing single nuclear spins is a central challenge in magnetic resonance based imaging techniques. Although different methods and especially diamond defect based sensing and imaging techniques in principle have shown sufficient…

Nuclear magnetic resonance (NMR) technique benefits from high magnetic field not only due to the field-enhanced measurement sensitivity and resolution, but also because it is a powerful tool to investigate field-induced physics in modern…

Instrumentation and Detectors · Physics 2023-05-05 Wenqi Wei , Qinying Liu , Le Yuan , Jian Zhang , Shiyu Liu , Rui Zhou , Yongkang Luo , Xiaotao Han

Over the last decade, frequency-domain in-situ high-pressure nuclear magnetic resonance (NMR) spectroscopy in diamond anvil cells (DACs) has been employed as a structural and electronic probe of condensed matter systems at pressures well…

Instrumentation and Detectors · Physics 2026-01-08 Thomas Meier , Meng Yang , Yishan Zhou , Yunhua Fu , Rui Zhang , Ziliang Wang , Tianyao Zheng , Rajesh Jana , Takeshi Nakagawa

Spin-labeling of molecules with paramagnetic ions is an important approach for determining molecular structure, however current ensemble techniques lack the sensitivity to detect few isolated spins. In this Letter, we demonstrate…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Matthew Pelliccione , Bryan A. Myers , Laetitia Pascal , Ananda Das , Ania C. Bleszynski Jayich

We review instrumentation for nuclear magnetic resonance (NMR) in zero and ultra-low magnetic field (ZULF, below 0.1 $\mu$T) where detection is based on a low-cost, non-cryogenic, spin-exchange relaxation free (SERF) $^{87}$Rb atomic…

In nanoscale metrology applications, measurements are commonly limited by the performance of the sensor. Here we show that in nuclear magnetic resonance (NMR) spectroscopy measurements using single nitrogen-vacancy (NV) centers in diamond,…

Solid state spins in diamond, in particular negatively charged nitrogen-vacancy centers (NV), are leading contenders in the field of quantum sensing. While addressing of single NVs offers nanoscale spatial resolution, many implementations…

Quantum Physics · Physics 2023-01-11 Yuchun Zhu , Elena Losero , Christophe Galland , Valentin Goblot

We present a novel approach to the detection of weak magnetic fields that takes advantage of recently developed techniques for the coherent control of solid-state electron spin quantum bits. Specifically, we investigate a magnetic sensor…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. M. Taylor , P. Cappellaro , L. Childress , L. Jiang , D. Budker , P. R. Hemmer , A. Yacoby , R. Walsworth , M. D. Lukin

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

Quantum Physics · Physics 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

Nitrogen-vacancy (NV) centers in diamond are a versatile quantum sensing platform for high sensitivity measurements of magnetic fields, temperature and strain with nanoscale spatial resolution. A common bottleneck is the analysis of…

Nitrogen-vacancy (NV) centers in diamond have emerged as valuable tools for sensing and polarizing spins. Motivated by potential applications in chemistry, biology, and medicine, we show that NV-based sensors are capable of detecting single…

Quantum Physics · Physics 2016-03-10 M. Bruderer , P. Fernández-Acebal , R. Aurich , M. B. Plenio

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

Mesoscale and Nanoscale Physics · Physics 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg

The nitrogen-vacancy (NV) color center in diamond is an atom-like system in the solid-state which specific spin properties can be efficiently used as a sensitive magnetic sensor. An external magnetic field induces Zeeman shifts of the NV…

Mesoscale and Nanoscale Physics · Physics 2015-07-17 M. Chipaux , A. Tallaire , J. Achard , S. Pezzagna , J. Meijer , V. Jacques , J. -F. Roch , T. Debuisschert

The nuclear spin is a prime candidate for quantum information applications due to its weak coupling to the environment and inherently long coherence times. However, this weak coupling also challenges the addressability of the nuclear spin.…

Quantum Physics · Physics 2025-12-15 Hester G. Vennema , Cristina Mier , Evert W. Stolte , Leonard Edens , Jinwon Lee , Sander Otte

Different approaches have improved the sensitivity of either electron or nuclear magnetic resonance to the single spin level. For optical detection it has essentially become routine to observe a single electron spin or nuclear spin.…

Mesoscale and Nanoscale Physics · Physics 2016-06-29 Jörg Wrachtrup , Amit Finkler

Mechanical resonators operating in the high-frequency regime have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also very…

Mesoscale and Nanoscale Physics · Physics 2023-11-29 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino
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