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A unified viewpoint on the van Vleck and Herman-Kluk propagators in Hilbert space and their recently developed counterparts in Wigner representation is presented. It is shown that the numerical protocol for the Herman-Kluk propagator, which…

Chemical Physics · Physics 2018-03-14 Fabian Gottwald , Sergei D. Ivanov

We propose a conjugate application of the Bargmann representation of quantum mechanics. Applying the Maslov method to the semiclassical connection formula between the two representations, we derive a uniform semiclassical approximation for…

Quantum Physics · Physics 2009-11-11 A. D. Ribeiro , M. Novaes , M. A. M. de Aguiar

We modify the pre-factor of the semiclassical propagator to improve its efficiency in practical implementations. The new pre-factor represents the smooth portion of an orbit's contribution, and leads to fast convergence in numerical…

Other Condensed Matter · Physics 2015-06-25 Quanlin Jie , Bambi Hu , Baowen Li

In this paper we consider the problem of computing the stationary distribution of nearly completely decomposable Markov processes, a well-established area in the classical theory of Markov processes with broad applications in the design,…

Numerical Analysis · Mathematics 2025-06-19 Vasileios Kalantzis , Mark S. Squillante , Chai Wah Wu

When the semiclassical Herman-Kluk propagator is used for evaluating quantum-mechanical observables or time-correlation functions, the initial conditions for the guiding trajectories are typically sampled from the Husimi density. Here, we…

Quantum Physics · Physics 2024-04-10 Fabian Kröninger , Caroline Lasser , Jiří Vaníček

In this paper, the use of partitioned linear multistep methods (PLMM) as time integrators for the numerical approximation of some partial differential equations (pdes) is studied. We consider the periodic initial-value problem of two…

Numerical Analysis · Mathematics 2025-11-06 Begoña Cano , Angel Durán , Melquíades Rodríguez

To alleviate the computational cost associated with on-the-fly ab initio semiclassical calculations of molecular spectra, we propose the single-Hessian thawed Gaussian approximation, in which the Hessian of the potential energy at all…

Chemical Physics · Physics 2024-09-26 Tomislav Begušić , Manuel Cordova , Jiří Vaníček

Calculating intermolecular charge transfer integrals in organic semiconductors requires substantial computer resource for each individual calculation. We might alternatively construct a machine learning model for transfer integrals, which…

Disordered Systems and Neural Networks · Physics 2025-11-11 Keerati Keeratikarn , Christoph Ortner , Jarvist Moore Frost

The quantum partition function at finite temperature requires computing the trace of the imaginary time propagator. For numerical and Monte Carlo calculations, the propagator is usually split into its kinetic and potential parts. A higher…

Statistical Mechanics · Physics 2009-11-10 Siu A. Chin

We use a semiclassical approximation to derive the partition function for an arbitrary potential in one-dimensional Quantum Statistical Mechanics, which we view as an example of finite temperature scalar Field Theory at a point. We rely on…

Quantum Physics · Physics 2009-10-31 C. A. A. de Carvalho , R. M. Cavalcanti

In this paper we study recent developments in the approximation of the spread option pricing. As the Kirk\'s Approximation is extremely flawed in the cases when the correlation is very high, we explore a recent development that allows…

Pricing of Securities · Quantitative Finance 2018-12-13 Suren Harutyunyan , AdriÀ Masip BorrÀs

Based on the work done by an electromagnetic field on an atomic or molecular electronic system, a general gauge invariant formulation of transient absorption spectroscopy is presented within the semi-classical approximation. Avoiding…

A continuous approximation for the results of [1] is obtained. In this approximation the energy distribution is represented in the form of the product of the Gibbs factor and superstatistics factor. The mutual weights of the factors are…

Chemical Physics · Physics 2007-05-23 V. V. Ryazanov

We deal with an initial-boundary value problem for the multidimensional acoustic wave equation, with the variable speed of sound. For a three-level semi-explicit in time higher-order vector compact scheme, we prove stability and derive 4th…

Numerical Analysis · Mathematics 2026-01-01 Alexander Zlotnik , Timofey Lomonosov

We study smooth, caustic-free, chaotic semiclassical dynamics on two-dimensional phase space and find that the dynamics can be approached by an iterative procedure which constructs an approximation to the exact long-time semiclassical…

chao-dyn · Physics 2009-08-14 L. Kaplan

Time-spectral solution of ordinary and partial differential equations is often regarded as an inefficient approach. The associated extension of the time domain, as compared to finite difference methods, is believed to result in…

Computational Physics · Physics 2017-04-14 Jan Scheffel , Kristoffer Lindvall

For a subquadratic symbol $H$ on $\R^d\times\R^d = T^*(\R^d)$, the quantum propagator of the time dependent Schr\"odinger equation $i\hbar\frac{\partial\psi}{\partial t} = \hat H\psi$ is a Semiclassical Fourier-Integral Operator when $\hat…

Mathematical Physics · Physics 2015-05-13 Didier Robert

Two semimetrics on probability distributions are proposed, given as the sum of differences of expectations of analytic functions evaluated at spatial or frequency locations (i.e, features). The features are chosen so as to maximize the…

Machine Learning · Statistics 2016-10-31 Wittawat Jitkrittum , Zoltan Szabo , Kacper Chwialkowski , Arthur Gretton

Continuous-time Bayesian networks is a natural structured representation language for multicomponent stochastic processes that evolve continuously over time. Despite the compact representation, inference in such models is intractable even…

Artificial Intelligence · Computer Science 2012-05-14 Ido Cohn , Tal El-Hay , Nir Friedman , Raz Kupferman

We propose and analyze a quasi-Monte Carlo (QMC) algorithm for efficient simulation of wave propagation modeled by the Helmholtz equation in a bounded region in which the refractive index is random and spatially heterogenous. Our focus is…

Numerical Analysis · Mathematics 2021-01-27 M. Ganesh , Frances Y. Kuo , Ian H. Sloan