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We achieve a quantum-noise-limited absorption sensitivity of 1.7/times10$^{-12}$ cm$^{-1}$ per spectral element at 400 s of acquisition time with cavity-enhanced frequency comb spectroscopy, the highest demonstrated for a comb-based…

Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are…

Broadband precision spectroscopy is indispensable for providing high fidelity molecular parameters for spectroscopic databases. We have recently shown that mechanical Fourier transform spectrometers based on optical frequency combs can…

Instrumentation and Detectors · Physics 2018-05-09 Lucile Rutkowski , Piotr Maslowski , Alexandra C. Johansson , Amir Khodabakhsh , Aleksandra Foltynowicz

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…

Two techniques that employ equally spaced trains of optical pulses to map an optical high frequency into a low frequency modulation of the signal that can be detected in real time are compared. The development of phase-stable optical…

Quantum Physics · Physics 2017-08-22 Kochise Bennett , Jeremy Rouxel , Shaul Mukamel

Optical frequency combs are key to optical precision measurements. While most frequency combs operate in the near-infrared regime, many applications require combs at mid-infrared, visible or even ultra-violet wavelengths. Frequency combs…

Frequency comb absorption spectroscopy combined with low-noise, fast homodyne measurements provide a toolbox for ultra-sensitive absorption measurements. Integrating these schemes on photonic platforms to bring them closer to practical…

Optics · Physics 2023-03-20 Jake Biele , Sabine Wollmann , Euan Allen

Optical frequency-comb-based-high-resolution spectrometers offer enormous potential for spectroscopic applications. Although various implementations have been demonstrated, the lack of suitable mid-infrared comb sources has impeded…

Optical frequency combs have had a remarkable impact on precision spectroscopy. Enabling this technology in the x-ray domain is expected to result in wide-ranging applications, such as stringent tests of astrophysical models and quantum…

Astronomical spectrographs require frequency calibration through sources like hollow-cathode lamps or absorption-gas cells. Laser frequency combs (LFCs) provide highest accuracy but are facing operational challenges. We aim to provide a…

Instrumentation and Methods for Astrophysics · Physics 2024-09-05 Ansgar Reiners , Michael Debus , Sebastian Schäfer , Eberhard Tiemann , Mathias Zechmeister

The outstanding phase-noise performance of optical frequency combs has led to a revolution in optical synthesis and metrology, covering a myriad of applications, from molecular spectroscopy to laser ranging and optical communications.…

Optics · Physics 2014-03-13 Victor Torres-Company , Andrew M. Weiner

Frequency combs (FC) have radically changed the landscape of frequency metrology and high-resolution spectroscopy investigations extending tremendously the achievable resolution while increasing signal to noise ratio. Initially developed in…

Instrumentation and Detectors · Physics 2019-05-14 S. Tammaro , O. Pirali , P. Roy , J. -F. Lampin , G. Ducournau , A. Cuisset , F. Hindle , G. Mouret

A laser frequency combs is a broad spectrum composed of equidistant narrow lines. Initially invented for frequency metrology, such combs enable new approaches to spectroscopy over broad spectral bandwidths, of particular relevance to…

Optics · Physics 2019-03-01 Nathalie Picqué , Theodor W. Hänsch

We have demonstrated a new technique that provides massively parallel comb spectroscopy sensitive specifically to ions through the combination of cavity-enhanced direct frequency comb spectroscopy with velocity modulation spectroscopy.…

Atomic Physics · Physics 2015-05-28 Laura C. Sinclair , Kevin C. Cossel , Tyler Coffey , Jun Ye , Eric A. Cornell

We describe a possible new technique for precise wavelength calibration of high-resolution astronomical spectrographs using femtosecond-pulsed mode-locked lasers controlled by stable oscillators such as atomic clocks. Such `frequency combs'…

Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…

Optics · Physics 2020-06-04 A. V. Muraviev , D. Konnov , K. L. Vodopyanov

Fourier transform spectroscopy based on incoherent light sources is a well-established tool in research fields from molecular spectroscopy and atmospheric monitoring to material science and biophysics. It provides broadband molecular…

Cavity-enhanced direct frequency comb spectroscopy combines broad spectral bandwidth, high spectral resolution, precise frequency calibration, and ultrahigh detection sensitivity, all in one experimental platform based on an optical…

Optics · Physics 2009-11-13 Michael J. Thorpe , Jun Ye

A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

We demonstrate the advantages of THz frequency combs for high-resolution spectroscopy. This benefits from wide spectral coverage and the exact knowledge of the frequency position of each comb component. Heterodyne detection combined with a…

Instrumentation and Detectors · Physics 2024-12-03 Francis Hindle , Alexandra Khabbaz , Anthony Roucou , Jean-Francois Lampin , Gaël Mouret
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