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We investigated the high-order harmonic generation (HHG) process of diatomic molecular ion $\mathrm{H}_2^+$ in non-Born-Oppenheimer approximations. The corresponding three-dimensional time-dependent Schr\"odinger equation is solved with…

Atomic Physics · Physics 2017-02-28 Mu-Zi Li , Guang-Rui Jia , Xue-Bin Bian

We establish time-resolved high harmonic generation (tr-HHG) as a powerful spectroscopy for photoinduced dynamics in strongly correlated materials through a detailed investigation of the insulator-to-metal transitions in vanadium dioxide.…

Acting as a highly nonlinear response to the strong laser field, high harmonic generation (HHG) naturally contains the fingerprints of atomic and electronic properties of materials. Electronic properties of a solid such as band structure…

Materials Science · Physics 2023-04-20 Shi-Qi Hu , Hui Zhao , Xin-Bao Liu , Da-Qiang Chen , Sheng Meng

We demonstrate a simple method to improve the Lewenstein model for the description of high-order harmonic generation (HHG). It is shown that HHG spectra can be expressed as the product of a returning electron wave packet and the…

Atomic Physics · Physics 2007-07-31 Anh-Thu Le , Toru Morishita , C. D. Lin

Using a fully real-space perspective on high harmonic generation (HHG) in solids, we examine the relationship between microscopic response, macroscopic propagation of this response to the far field, and the extremely short dephasing times…

When a laser pulse impinges on a molecule which is invariant under certain symmetry operations selection rules for harmonic generation (HG) arise. In other words: symmetry controls which channels are open for the deposition and emission of…

Atomic Physics · Physics 2009-11-07 D. Bauer , F. Ceccherini

In this paper, we investigate the effects of full electronic correlation on the high harmonic generation in the helium atom subjected to laser pulses of extremely high intensity. To do this, we perform real-time propagations of the helium…

Chemical Physics · Physics 2022-05-18 Aleksander P. Woźniak , Michał Przybytek , Maciej Lewenstein , Robert Moszyński

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV)…

We investigate a two-level atom in the field of a strong laser pulse. The resulting time-dependent polarization is the source of a radiation the frequency components of which are essentially harmonics of the driving field's carrier…

Quantum Physics · Physics 2016-09-13 Ákos Gombkötő , Attila Czirják , Sándor Varró , Péter Földi

Strong field driven electric currents in condensed matter systems open new frontiers in petahertz electronics. In this regime new challenges arise as the role of the band structure and the quantum nature of electron-hole dynamics have yet…

High harmonic generation (HHG) is a widely explored process in solids, where intense lasers drive attosecond-to-femtosecond electron dynamics within bands, causing high-energy emission. While electrons and photons are considered the main…

Optics · Physics 2026-04-28 Adam Herling , Ofer Neufeld

We theoretically investigate electron-hole recollisions in high-harmonic generation (HHG) in band-gap solids irradiated by linearly and elliptically polarized drivers. We find that in many cases the emitted harmonics do not originate in…

Atomic Physics · Physics 2021-06-15 Lun Yue , Mette B. Gaarde

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

High-order harmonic generation (HHG) by hydrogenlike atoms/ions in the uniform periodic electric field, formed by the two linearly polarized counterpropagating laser beams of relativistic intensities, is studied. The relativistic quantum…

Atomic Physics · Physics 2011-06-14 H. K. Avetissian , A. G. Markossian , G. F. Mkrtchian

The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

High-harmonic generation (HHG) from solid state offers promising potential for attosecond optics with enhanced efficiency and compact configurations. However, Current implementations face critical limitations imposed by material damage…

Optics · Physics 2025-08-19 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Lin-Wang Wang , Jun-Wei Luo , Zhi Wang

We present theoretical studies of high-order harmonic generation (HHG) driven by plasmonic fields in two-electron atomic systems. Comparing the two-active electron and single-active electron approximation models of the negative hydrogen ion…

Atomic Physics · Physics 2016-11-03 A. Chacón , M. F. Ciappina , M. Lewenstein

A theoretical study on the high-harmonic generation (HHG) in solids by a synthesized driver field is carried out. The vector potential of the driver field is instrumental in determining the Bloch oscillations of the electrons in a periodic…

Atomic and Molecular Clusters · Physics 2023-05-02 Nivash R. , Amol R Holkundkar , Jayendra N. Bandyopadhyay