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The magnetic excitation spectrum of copper pyrimidine dinitrate, a material containing S=1/2 antiferromagnetic chains with alternating g-tensor and the Dzyaloshinskii-Moriya interaction, and exhibiting a field-induced spin gap, is probed…

Strongly Correlated Electrons · Physics 2009-11-10 S. A. Zvyagin , A. K. Kolezhuk , J. Krzystek , R. Feyerherm

The S=1/2 antiferromagnetic Heisenberg chain exhibits a magnetic field driven quantum critical point. We study the low frequency spin dynamics in copper pyrazine dinitrate (CuPzN), a realization of this model system of quantum magnetism, by…

Strongly Correlated Electrons · Physics 2010-03-25 H. Kuehne , M. Guenther , S. Grossjohann , W. Brenig , F. J. Litterst , A. P. Reyes , P. L. Kuhns , M. M. Turnbull , C. P. Landee , H. -H. Klauss

We report the low-temperature multi-frequency ESR studies of copper pyrimidine dinitrate, a spin-1/2 antiferromagnetic chain with alternating $g$-tensor and the Dzyaloshinskii-Moriya interaction, allowing us to test a new theoretical…

Strongly Correlated Electrons · Physics 2009-11-11 S. A. Zvyagin , A. K. Kolezhuk , J. Krzystek , R. Feyerherm

High field mangetization, field-dependent specific heat measurements, and zero field inelastic magnetic neutron scattering have been used to explore the magnetic properties of copper pyrazine dinitrate (Cu(C4H4N2)(NO3)2). The material is an…

Strongly Correlated Electrons · Physics 2009-10-31 P. R. Hammar , M. B. Stone , Daniel H. Reich , C. Broholm , P. J. Gibson , M. M. Turnbull , C. P. Landee , M. Oshikawa

The magnetic insulator copper pyrazine dinitrate comprises antiferromagnetic spin-1/2 chains that are well described by the exactly solvable one-dimensional Heisenberg model, providing a unique opportunity for a quantitative comparison…

Strongly Correlated Electrons · Physics 2018-01-04 Oliver Breunig , Markus Garst , Andreas Klümper , Jens Rohrkamp , Mark M. Turnbull , Thomas Lorenz

We present the results of muon-spin relaxation measurements of spin excitations in the one-dimensional quantum Heisenberg antiferromagnet Cu(pyz)(NO$_{3}$)$_{2}$. Using density-functional theory we propose muon sites and assess the degree…

Strongly Correlated Electrons · Physics 2015-05-20 F. Xiao , J. S. Möller , T. Lancaster , R. C. Williams , F. L. Pratt , S. J. Blundell , D. Ceresoli , A. M. Barton , J. L. Manson

We investigate the quantum evolution of spin states of a single molecular magnet in a local electric field. The decoherence of a $\texttt{\{}\emph{Cu}_3\texttt{\}}$ single molecular magnet weakly coupled to a thermal bosonic environment can…

Quantum Physics · Physics 2015-06-18 Xiang Hao , Xiaoqun Wang , Chen Liu , Shiqun Zhu

We investigate the magnetic properties of a range of low-dimensional ferromagnets using a combination of first-principles calculations and atomistic spin dynamics simulations. This approach allows us to evaluate the ground state and finite…

Materials Science · Physics 2016-11-26 Lars Bergqvist , Andrea Taroni , Anders Bergman , Corina Etz , Olle Eriksson

Thermodynamic properties and elementary excitations in $S=1/2$ one-dimensional Heisenberg antiferromagnet KCuGaF$_6$ were investigated by magnetic susceptibility, specific heat and ESR measurements. Due to the Dzyaloshinsky-Moriya…

Strongly Correlated Electrons · Physics 2009-11-13 Rieko Morisaki , Toshio Ono , Hidekazu Tanaka , Hiroyuki Nojiri

We present the first evidence of magnetic order in the quasi-one-dimensional spin 1/2 molecular chain compound, copper pyrazine dinitrate Cu(C4H4N2)(NO3)2}. Zero field muon-spin relaxation measurements made at dilution refrigerator…

Strongly Correlated Electrons · Physics 2007-11-14 T. Lancaster , S. J. Blundell , M. L. Brooks , P. J. Baker , F. L. Pratt , J. L. Manson , C. P. Landee , C. Baines

A comprehensive comparison between the magnetic field- and temperature-dependent low frequency spin dynamics in the antiferromagnetic spin-1/2 Heisenberg chain (AFHC) system copper pyrazine dinitrate, probed via the 13C-nuclear magnetic…

Strongly Correlated Electrons · Physics 2015-05-19 H. Kuehne , A. A. Zvyagin , M. Guenther , A. P. Reyes , P. L. Kuhns , M. M. Turnbull , C. P. Landee , H. -H. Klauss

We present a 13C-NMR study of the magnetic field driven transition to complete polarization of the S=1/2 antiferromagnetic Heisenberg chain system copper pyrazine dinitrate Cu(C_4H_4N_2)(NO_3)_2 (CuPzN). The static local magnetization as…

Strongly Correlated Electrons · Physics 2009-08-13 H. Kuehne , H. -H. Klauss , S. Grossjohann , W. Brenig , F. J. Litterst , A. P. Reyes , P. L. Kuhns , M. M. Turnbull , C. P. Landee

The magnetic excitation spectrum in the two-dimensional (2D) S=1/2 Heisenberg antiferromagnet copper deuteroformate tetradeuterate (CFTD) has been measured for temperatures up to T\sim J/2, where J=6.31+-0.02 meV is the 2D exchange…

Magnetic excitations in copper pyrimidine dinitrate, a spin-1/2 antiferromagnetic chain with alternating $g$-tensor and Dzyaloshinskii-Moriya interactions that exhibits a field-induced spin gap, are probed by means of pulsed-field electron…

Materials Science · Physics 2011-02-25 S. A. Zvyagin , E. Čižmár , M. Ozerov , J. Wosnitza , R. Feyerherm , S. R. Manmana , F. Mila

We report magnetization, electron spin resonance (ESR), and muon spin relaxation ($\mu $SR) measurements on single crystals of the $S=1/2$ (Cu$% ^{+2}$) kagom\'{e} compound Cu(1,3-benzendicarboxylate). The $\mu $SR is carried to…

Strongly Correlated Electrons · Physics 2015-06-18 Oren Ofer , Lital Marcipar , V. Ravi Chandra , Snir Gazit , Daniel Podolsky , Daniel P. Arovas , Amit Keren

A new elementary-excitation, the so called "breather excitation", is observed directly by millimeter-submillimeter wave electron spin resonance (ESR) in the Heisenberg quantum spin-chain Cu benzoate, in which a field-induced gap is found…

Strongly Correlated Electrons · Physics 2009-10-31 T. Asano , H. Nojiri , Y. Inagaki , J. P. Boucher , T. Sakon , Y. Ajiro , M. Motokawa

We investigate the low-temperature magnetic properties of the molecule-based chiral spin chain [Cu(pym)(H$_2$O)$_4$]SiF$_6\cdot$H$_2$O (pym = pyrimidine). Electron-spin resonance, magnetometry and heat capacity measurements reveal the…

We compare theoretical results for electron spin resonance (ESR) properties of the Heisenberg-Ising Hamiltonian with ESR experiments on the quasi-one-dimensional magnet Cu(py)$_2$Br$_2$ (CPB). Our measurements were performed over a wide…

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

The magnetic state of the single-component molecular compound, [Cu(tmdt)$_{2}$], is investigated by means of $^{1}$H-NMR. An abrupt spectral broadening below 13 K and a sharp peak in nuclear spin-lattice relaxation rate, $T_{1}^{-1}$, at 13…

Strongly Correlated Electrons · Physics 2012-05-31 Rina Takagi , Kazuya Miyagawa , Kazushi Kanoda , Biao Zhou , Akiko Kobayashi , Hayao Kobayashi
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