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The molecular photo cell, i.e., a single molecule donor-acceptor complex, beside being technologically important, is a paradigmatic example of a many-body system operating in strong non-equilibrium. The quantum transport and the…

Mesoscale and Nanoscale Physics · Physics 2020-07-06 Subhajit Sarkar , Yonatan Dubi

Imperfect photons' indistinguishability limits the performance of photonic quantum communication and computation . Distillation protocols, inspired by entanglement purification, enhance photons' indistinguishability by leveraging quantum…

Strong light-matter interactions facilitate not only emerging applications in quantum and non-linear optics but also modifications of materials properties. In particular the latter possibility has spurred the development of advanced…

Mesoscale and Nanoscale Physics · Physics 2021-08-17 Jakub Fojt , Tuomas P. Rossi , Tomasz J. Antosiewicz , Mikael Kuisma , Paul Erhart

To absorb the photons below the band-gap energy effectively, we proposed a quantum dot (QD) photocell modeled by multi-level system for the quantum yields and photo-to-charge efficiency limits. The theoretical results show the quantum…

Mesoscale and Nanoscale Physics · Physics 2024-02-26 Shun-Cai Zhao , Jing-Yi Chen

Tin-phthalocyanine molecules adsorbed on a NaCl ultrathin film on Au(111) exhibit electrofluorescence excited by a current across a scanning tunneling microscope junction. Exploring the dependence of the molecular monomer photon yield on…

Mesoscale and Nanoscale Physics · Physics 2026-03-03 Maximilian Kögler , Nicolas Néel , Jörg Kröger

It is thought that nature already exploits quantum mechanical properties to increase the efficiency of solar energy harvesting devices. So, the operation of these devices can be enhanced by clever design of a nanoscopic, quantum mechanical…

Mesoscale and Nanoscale Physics · Physics 2024-07-17 Baharak Mohamad Jafari Navadel , Esfandyar Faizi , Baharam Ahansaz , Jaber Jahanbin Sardroodi

This work discusses the problem of optimal excitation of a three-level atom of ladder-configuration by light in the two-photon state and coherent light carrying an average of two photons. The applied atom-light interaction model is based on…

Quantum Physics · Physics 2025-03-25 Masood Valipour , Gniewomir Sarbicki , Karolina Słowik , Anita Dąbrowska

The functional properties of photoactive proteins are governed by the interplay between bright and dark excited states. While the bright states are well-studied, the dark states, which are fundamental to photostability and light harvesting,…

Efficient devices for light harvesting and photon sensing are fundamental building blocks of basic energy science and many essential technologies. Recent efforts have turned to biomimicry to design the next generation of light-capturing…

To understand the photophysics of molecular aggregates, exciton model of J- and H-aggregate has been extensively utilized. However, it lacks consideration of crystal symmetry. Although discrete molecules may lack symmetry, their aggregates…

Mesoscale and Nanoscale Physics · Physics 2023-10-10 Qingyun Wan , Chi-Ming Che

Engineering the local density of states with nanophotonic structures is a powerful tool to control light-matter interactions via the Purcell effect. At optical frequencies, control over the electric field density of states is typically used…

We study excitation energy transfer in a simple model of photosynthetic complex. The model, described by Lindblad equation, consists of pigments interacting via dipole-dipole interaction. Overlapping of pigments induces an on-site energy…

Biological Physics · Physics 2012-09-19 Simon Jesenko , Marko Znidaric

Natural and artificial light harvesting systems often operate in a regime where the flux of photons is relatively low. Besides absorbing as many photons as possible it is therefore paramount to prevent excitons from annihilation via photon…

Quantum Physics · Physics 2017-10-24 K. D. B. Higgins , B. W. Lovett , E. M. Gauger

Single-photon and correlated two-photon sources are important elements for optical information systems. Nonlinear downconversion light sources are robust and stable emitters of single photons and entangled photon pairs. However, the rate of…

Optics · Physics 2017-09-22 Artur R. Davoyan , Harry A. Atwater

Photoinduced charge-transfer excitations are key to understand the primary processes of natural photosynthesis and for designing photovoltaic and photocatalytic devices. In this paper, we use Bacteriochlorophyll dimers extracted from the…

Chemical Physics · Physics 2023-04-11 Zohreh Hashemi , Matthias Knodt , Mario R. G. Marques , Linn Leppert

Efficient coupling of light to single atomic systems has gained considerable attention over the past decades. This development is driven by the continuous growth of quantum technologies. The efficient coupling of light and matter is an…

Quantum Physics · Physics 2015-07-24 Markus Sondermann , Gerd Leuchs

Elaborating reliable and versatile strategies for efficient light coupling between free space and thin films is of crucial importance for new technologies in energy efficiency. Nanostructured materials have opened unprecedented…

Optics · Physics 2013-04-10 Kevin Vynck , Matteo Burresi , Francesco Riboli , Diederik S. Wiersma

Nano-scaled metallic or dielectric structures may provide various ways to trap light into thin-film solar cells for improving the conversion efficiency. In most schemes, the textured active layers are involved into light trapping structures…

Optics · Physics 2014-12-01 DongLin Wang , Gang Su

Photosynthetic organisms use networks of chromophores to absorb sunlight and deliver the energy to reaction centres, where charge separation triggers a cascade of chemical steps to store the energy. We present a detailed model of the…

We present a theory for the diffraction of large molecules or nanoparticles at a standing light wave. Such particles can act as a genuine photon absorbers due to their numerous internal degrees of freedom effecting fast internal energy…

Quantum Physics · Physics 2016-10-26 Kai Walter , Stefan Nimmrichter , Klaus Hornberger