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Sr2IrO4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr2Ir1-xFexO4 (0<x<0.32) and Sr2Ir1-xCoxO4 (0<x<0.22). Fe doping retains the…

Strongly Correlated Electrons · Physics 2020-12-21 Bing Hu , Hengdi Zhao , Yu Zhang , Pedro Schlottmann , Feng Ye , Gang Cao

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

Sr$_2$IrO$_4$ is an extensively studied spin-orbit coupling induced insulator with antiferromagnetic ground state. The delicate balance between competing energy scales plays crucial role for its low temperature phase, and the route of…

Strongly Correlated Electrons · Physics 2017-10-31 Imtiaz Noor Bhatti , R. S. Dhaka , A. K. Pramanik

We report a systematical structural, transport and magnetic study of Ca or Ba doped Sr2IrO4single crystals. Isoelectronically substituting Ca2+ (up to 15%) or Ba2+ (up to 4%) ion for the Sr2+ ion provides no additional charge carriers but…

Strongly Correlated Electrons · Physics 2018-05-04 H. D. Zhao , J. Terzic , H. Zheng , Y. F. Ni , Y. Zhang , Feng Ye , P. Schlottmann , G. Cao

Sr2IrO4 is a magnetic insulator assisted by strong spin-orbit coupling (SOC) whereas the Sr2RuO4 is a p-wave superconductor. The contrasting ground states have been shown to result from the critical role of the strong SOC in the iridate.…

Strongly Correlated Electrons · Physics 2016-04-26 S. J. Yuan , S. Aswartham , J. Terzic , H. Zheng , H. D. Zhao , P. Schlottmann , G. Cao

Sr2IrO4 exhibits a novel insulating state assisted by spin-orbit interactions. A series of polycrystalline samples of Sr2-xIrO4 have been synthesized. It is found that deep Sr-vacancies of Sr2-xIrO4 greatly reduce the rotation of IrO6…

Strongly Correlated Electrons · Physics 2016-11-01 Xuanyong Sun , S. L. Liu , Haiyun Wang , Bin Li , Jie Cheng , Z. H. Wang

Stoichiometric Sr2IrO4 is a ferromagnetic Jeff = 1/2 Mott insulator driven by strong spin-orbit coupling. Introduction of very dilute oxygen vacancies into single-crystal Sr2IrO4-delta with delta < 0.04 leads to significant changes in…

Strongly Correlated Electrons · Physics 2010-08-30 O. B. Korneta , Tongfei Qi , S. Chikara , S. Parkin L. E. De Long , P. Schlottmann , G. Cao

Antiferromagnetic (AFM) spintronics, where magneto-transport is governed by an antiferromagnet instead of a ferromagnet, opens fascinating new perspectives for both fundamental research and device technology, owing to their intrinsic…

Materials Science · Physics 2021-10-26 Haowen Wang , Wei Wang , Ni Hu , Tianci Duan , Songliu Yuan , Shuai Dong , Chengliang Lu , Jun-Ming Liu

It is commonly anticipated that an insulating state collapses in favor of an emergent metallic state at high pressures as the unit cell shrinks and the electronic bandwidth broadens to fill the insulating energy band gap. Here we report a…

Magnetic insulators are often antiferromagnetic (AFM) and layered AFM compounds usually show low ordering temperature. On the other hand, layered ferromagnetic (FM) insulators with high-TC are very rare although they could be quite useful…

Materials Science · Physics 2018-11-12 Ke Yang , Feng-Ren Fan , Alessandro Stroppa , Hua Wu

We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

Strongly Correlated Electrons · Physics 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

Here, we report an investigation of structural, magnetic and electronic properties in Y-doped layered iridate (Sr$_{1-x}$Y$_x$)$_2$IrO$_4$ ($x$ $\leq$ 0.1). The parent Sr$_2$IrO$_4$ is a well-studied spin-orbit coupling (SOC) induced…

Strongly Correlated Electrons · Physics 2021-03-17 Imtiaz Noor Bhatti , A. K. Pramanik

The layered 5d transition metal oxide Sr2IrO4 has been shown to host a novel Jeff=1/2 Mott spin orbit insulating state with antiferromagnetic ordering, leading to comparisons with the layered cuprates. Here we study the effect of…

Strongly Correlated Electrons · Physics 2015-03-20 S. Calder , G. -X. Cao , M. D. Lumsden , J. W. Kim , Z. Gai , B. C. Sales , D. Mandrus , A. D. Christianson

Sr$_2$IrO$_4$ has attracted a lot of attention due to its structural and electronic similarities to La$_2$CuO$_4$ which is the parent compound of high-T$_c$ superconducting cuprates. It was proposed to be a strong spin-orbit coupled…

Sr2IrO4 exhibits a novel insulating state driven by spin-orbit interactions. We report two novel phenomena, namely a large magnetoresistivity in Sr2IrO4 that is extremely sensitive to the orientation of magnetic field but exhibits no…

Strongly Correlated Electrons · Physics 2015-05-28 M. Ge , T. F. Qi , O. B. Korneta , D. E. De Long , P. Schlottmann , W. P. Crummett , G. Cao

Sr$_2$IrO$_4$ is the archetype of the spin-orbit Mott insulator, but the nature of the metallic states that may emerge from this type of insulator is still not very well known. We study with angle-resolved photoemission the…

Strongly Correlated Electrons · Physics 2018-04-30 Alex Louat , Fabrice Bert , Lise Serrier-Garcia , François Bertran , Patrick Le Fèvre , Julien Rault , Véronique Brouet

BaIrO3 is a magnetic insulator driven by the spin-orbit interaction (SOI), whereas BaRuO3 is a paramagnet and exhibits a crossover from a metallic to an insulating regime. Our investigation of structural, magnetic, transport and thermal…

Strongly Correlated Electrons · Physics 2016-04-26 S. J. Yuan , K. Butrouna , J. Terzic , H. Zheng , S. Aswartham , L. E. DeLong , P. Schlottmann , G. Cao

The orthorhombic perovskite SrIrO3 is a semimetal, an intriguing exception in iridates where the strong spin-orbit interaction coupled with electron correlations tends to impose a novel insulating state. We report results of our…

Strongly Correlated Electrons · Physics 2016-07-06 H. Zheng , J. Terzic , Feng Ye , X. G. Wan , D. Wang , Jinchen Wang , Xiaoping Wang , P. Schlottmann , S. J. Yuan , G. Cao

Sr3Ir2O7 exhibits a novel Jeff=1/2 insulating state that features a splitting between Jeff=1/2 and 3/2 bands due to spin-orbit interaction. We report a metal-insulator transition in Sr3Ir2O7 via either dilute electron doping (La3+ for Sr2+)…

Strongly Correlated Electrons · Physics 2015-06-15 L. Li , P. P. Kong , T. F. Qi , C. Q. Jin , S. J. Yuan , L. E. DeLong , P. Schlottmann , G. Cao

We report structural, magnetic, transport and thermal properties of single-crystal Ca2Ru1-xIrxO4 (0 < x< 0.65). Ca2RuO4 is a structurally-driven Mott insulator with a metal-insulator transition at TMI = 357 K, which is well separated from…

Strongly Correlated Electrons · Physics 2016-04-26 S. J. Yuan , J. Terzic , J. C. Wang , S. Aswartham , W. H. Song , F. Ye , G. Cao
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