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Conical intersections are crossing points or lines between two or more adiabatic electronic potential energy surfaces in the multi-dimensional coordinate space of colliding atoms and molecules. Conical intersections and corresponding…

Atomic Physics · Physics 2023-04-19 Hui Li , Ming Li , Alexander Petrov , Eite Tiesinga , Svetlana Kotochigova

The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…

Light-induced conical intersections (LICIs) can be formed both by standing or by running laser waves. The position of a LICI is determined by the laser frequency while the laser intensity controls the strength of the nonadiabatic coupling.…

Atomic and Molecular Clusters · Physics 2016-07-11 András Csehi , Gábor J. Halász , Lorenz S. Cederbaum , Ágnes Vibók

Recently it has been recognized that electronic conical intersections in molecular systems can be induced by laser light even in diatomics. As is known a direct consequence of these accidental degeneracies is the appearence of nonadiabatic…

Atomic and Molecular Clusters · Physics 2013-10-30 Gábor J. Halász , Ágnes Vibók , Nimrod Moiseyev , Lorenz S. Cederbaum

We show that dressing of diatomic molecules by running laser waves gives rise to conical intersections (CIs). Due to presence of such CIs, the rovibronic molecular motions are strongly coupled. A pronounced impact of the CI on the spectrum…

Atomic Physics · Physics 2015-05-19 Milan Sindelka , Nimrod Moiseyev , Lorenz S. Cederbaum

Nonadiabatic effects are ubiquitous in physics, chemistry and biology. They are strongly amplified by conical intersections (CIs) which are degeneracies between electronic states of triatomic or larger molecules. A few years ago it has been…

Atomic and Molecular Clusters · Physics 2014-11-25 Gábor J. Halász , Ágnes Vibók , Lorenz S. Cederbaum

We theoretically study dissociative ionization of H$_2^+$ exposed to strong linearly polarized few-cycle visible, near-infrared and midinfrared laser pulses. We find rich energy-sharing structures in the combined electron and nuclear…

Atomic Physics · Physics 2016-03-15 Lun Yue , Lars Bojer Madsen

In the presence of linearly varying frequency chirped laser pulses the photodissociation dynamics of D$_2^+$ is studied theoretically after ionization of D$_{2}$ . As a completion of our recent work (J. Chem. Phys. 143, 014305 (2015)) a…

Atomic and Molecular Clusters · Physics 2016-03-23 András Csehi , Gábor J. Halász , Lorenz S. Cederbaum , Ágnes Vibók

We calculate angle-resolved above-threshold ionization spectra for diatomic molecules in linearly polarized laser fields, employing the strong-field approximation. The interference structure resulting from the individual contributions of…

Atomic Physics · Physics 2009-11-13 H. Hetzheim , C. Figueira de Morisson Faria , W. Becker

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

Ionization of atoms and molecules in laser fields can lead to various interesting interference structures in the photoelectron spectrum. For the case of a super-intense extreme ultraviolet laser pulse, we identify a novel petal-like…

Atomic Physics · Physics 2022-03-29 Lei Geng , Hao Liang , K. Krajewska , Liang-You Peng , Qihuang Gong

We use orthogonally polarized two-colour (OTC) laser pulses to separate quantum paths in multiphoton ionization of Ar atoms. Our OTC pulses consist of 400~nm and 800~nm light at a relative intensity ratio of 10:1. We find a hitherto…

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

A fundamental theoretical framework is formulated for the investigation of rovibronic spectra resulting from the coupling of molecules to one mode of the radiation field in an optical cavity. The approach involves the computation of (1)…

Atomic and Molecular Clusters · Physics 2018-08-15 Tamás Szidarovszky , Attila. G. Császár , Gábor J. Halász , Lorenz S. Cederbaum , Ágnes Vibók

Conical intersections (CI) between molecular potential energy surfaces with non-vanishing non-adiabatic couplings generally occur in any molecule consisting of at least three atoms. They play a fundamental role in describing the molecular…

We study the ionization of atomic hydrogen in the direction of polarization due to a linearly polarized XUV pulse in the presence a strong field IR. We describe the photoelectron spectra as an interference problem in the time domain.…

Atomic Physics · Physics 2016-11-15 Ana Alicia Gramajo , Renata Della Picca , Carlos Roberto Garibotti , Diego Arbó

Existence of different types of interference in the spectrum of radiation emitted by a doubly hard scattered electron is demonstrated. The spectrum develops oscillations in two regions: the hard, where the oscillations depend on the…

Accelerator Physics · Physics 2017-04-05 M. V. Bondarenco , N. F. Shul'ga

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

Quantum Physics · Physics 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

In the Kapitza-Dirac effect, atoms, molecules, or swift electrons are diffracted off a standing wave grating of the light intensity created by two counter-propagating laser fields. In ultrafast electron optics, such a coherent beam splitter…

Quantum Physics · Physics 2019-05-03 Nahid Talebi , Christoph Lienau

New experimental data about proton-proton collisions obtained atthe LHC allow to widen strongly the energy interval where one gets some knowledge about the structure of their interaction region. Using the unitarity relation in combination…

High Energy Physics - Phenomenology · Physics 2016-11-25 I. M. Dremin
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